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Unveiling NPT bound problem: From Distillability Sets to Inequalities and Multivariable Insights

Si-Yuan Qi CAS Key Laboratory of Quantum Information, University of Science and Technology of China, Hefei, Anhui 230026, P. R. China CAS Center For Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China, Hefei, Anhui 230026, P. R. China    Geni Gupur [email protected] College of Mathematics and Systems Science, Xinjiang University, Urumqi, Xinjiang 830017, People’s Republic of China    Yu-Chun Wu [email protected] CAS Key Laboratory of Quantum Information, University of Science and Technology of China, Hefei, Anhui 230026, P. R. China CAS Center For Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China, Hefei, Anhui 230026, P. R. China Institute of Artificial Intelligence, Hefei Comprehensive National Science Center, Hefei, Anhui 230088, People’s Republic of China    Guo-Ping Guo CAS Key Laboratory of Quantum Information, University of Science and Technology of China, Hefei, Anhui 230026, P. R. China CAS Center For Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China, Hefei, Anhui 230026, P. R. China Institute of Artificial Intelligence, Hefei Comprehensive National Science Center, Hefei, Anhui 230088, People’s Republic of China Origin Quantum Computing Hefei, Anhui 230026, P. R. China
(January 21, 2025)
Abstract

Equivalence between Positive Partial Transpose (PPT) entanglement and bound entanglement is a long-standing open problem in quantum information theory. So far limited progress has been made, even on the seemingly simple case of Werner states bound entanglement. The primary challenge is to give a concise mathematical representation of undistillability. To this end, we propose a decomposition of the N-undistillability verification into log(N)log(N) repeated steps of 1-undistillability verification. For Werner state N-undistillability verification, a bound for N-undistillability is given, which is independent of the dimensionality of Werner states. Equivalent forms of inequalities for both rank one and two matrices are presented, before transforming the two-undistillability case into a matrix analysis problem. A new perspective is also attempted by seeing it as a non-convex multi-variable function, proving its critical points and conjecturing Hessian positivity, which would make them local minimums.

preprint: APS/123-QED

I Introduction

Entanglement [1] is what distinguished the quantum world from classical worlds. Unfortunately, our understanding of it remains quite limited to this day. Entanglement exhibits varying degrees of strength, the highest of which falls into a subclass called “maximal entanglement”. Bell state is one such example. No consensus has yet been reached about what qualifies as a “weak entanglement”. Quantum states with small Schmidt numbers are generally seen as weakly entangled, since quantum states with Schmidt number 1 are separable. Undistillable entanglement is another kind of widely accepted weak entanglement. Relationships between these two kinds of weak entanglements are discussed in [2].

Entanglement distillation [3] is the process of obtaining pure Bell states only by Local Operations and Classical Communication (LOCC) from multiple copies of an entangled bipartite state. If N copies of a given entangled bipartite state can be transformed into pure Bell states through LOCC, then the entangled bipartite state is referred to as N-distillable. If not, then it’s N-undistillable. If a particular entangled bipartite state is N-undistillable for arbitrary N, it is considered undistillable and is also referred to as a bound entangled state.

Another property concerned here is “Positive Partial Transpose” (PPT). PPT refers to a bipartite quantum state whose partial transpose is positive semidefinite. It is established in [4] that Positive Partial Transpose (PPT) entanglement implies bound entanglement, and therefore weakly entangled in terms of distillability. However, the question of whether the converse is true remains an open problem [5]. This problem is usually referred to as the NPT bound problem, or the distillability problem. The popular conjecture regarding this problem is that the converse is not true, and that NPT bound entanglement exists. A number of special circumstances have been worked out in [6, 7, 8, 9, 10]. Indirect approaches to this problem include expansion of distillation operations to k-extendible operations [11], catalysis-assisted distillation [12], and dually non-entangling and PPT-preserving channels [13], linking the problem with squashed entanglement [14] and linear preserver [15], studying the transformation of bound entangled states under certain dynamic process [16], or considering the problem in a broader scenario such as hyperquantum states [17].

In three separate attempts to directly tackle the distillability problem [18], [19] and [20], they each had a subset of quantum states singled out, and proved that for any finite number of copies N, there exist undistillable states in this subset. However, as N approaches infinity, the subset shrinks to emptiness. It has been shown in [21] that N-undistillability does not imply (N+1)-undistillability, by demonstrating a set of distillable-only-by-arbitrarily-large-number-of-copies state, thus ruling out the easy route of concentrating on few-copies distillation.

For the Werner states [22], a family of single-parameter states, the existence of NPT bound states implies existence of NPT bound Werner states [23]. Therefore, it is sufficient to only study Werner states. Due to the inherent complexity of addressing N-copy Werner state distillability, over the last decade, direct attacks on the problem have been primarily fixating on the seemingly straightforward problem of 2-copy Werner state distillability, but so far only limited progress has been made. In an attempt to attack the 2-copy Werner state distillability problem, the special case of 4×44\times 4 bipartite states is considered in [24], in which case the distillability condition can be reduced to a convenient form of “half-property”, and subsequently reformulated the distillability problem into a matrix analysis problem. For a special case where the matrices are normal, a proof was given.

In [25] the problem is reformulated and established that for a d×dd\times d bipartite Werner state, the 2-copy Werner state undistillability problem is equivalent to a certain 2d2×2d22d^{2}\times 2d^{2} matrix being positive semidefinite. Positive definiteness of the block matrices in the upper-left and lower-right corners has been proved.

In this work, we introduce a method that decomposes bound entanglement verification into repeated steps of 1-undistillability verification, before giving a new bound for N-undistillability that is independent of quantum state dimensions dd, and therefore different from that given in [18], [19] and [20]. However, similar to the problem encountered in [18], [19] and [20], our set of N-undistillable states also shrinks to emptiness for NN\to\infty. Also, an equivalent matrix analysis inequality form is presented, which is applicable to all finite dimensionalities, as opposed to the case in [24] when only the d=4d=4 case is considered. Another equivalent version of inequalities regarding only rank-one matrices is also included, which takes on a form reminiscent of Cauchy-Schwartz inequality. Finally, we take on a brand-new perspective of considering it as a multi-variable function problem, finding critical points, proving non-convexity and conjecturing Hessian positivity.

We will be using A\mathcal{H}_{A} and B\mathcal{H}_{B} to denote Hilbert spaces pertaining to A and B subsystems, and XiX_{i} to denote matrices of rank less than or equal to ii. Throughout the paper we will be considering multi-partite quantum states with identical dimensions, i.e. quantum states on AB\mathcal{H}_{A}\otimes\mathcal{H}_{B}, where dim(A)=dim(B)=ddim(\mathcal{H}_{A})=dim(\mathcal{H}_{B})=d. This is justified by noticing that any quantum state of d1×d2d_{1}\times d_{2} can be equivalently transformed into a quantum state of identical dimensions max{d1,d2}×max{d1,d2}max\{d_{1},d_{2}\}\times max\{d_{1},d_{2}\}, with all unnecessary elements set to zero.

The structure of this paper is as follows: In Section II, we introduce a matrix transformation that takes N-distillability problem into a higher dimensional 1-distillability problem. In Section III, the process of NN-undistillability verification is transformed into log(N)log(N) repeated steps of 1-undistillability verification. In Section IV, upper bounds on NN-undistillability are given, yielding a result similar to that of [18], [19] and [20], effectively finding shrinking families of N-undistillable quantum states. In Section V, equivalent partial trace inequalities are presented before turning them into a matrix analysis problem. The rank-two matrix analysis problem is also reduced to a rank-one matrix analysis problem, resulting in a Cauchy-Schwartz inequality look-alike. In Section VI, we take on a new perspective by treating the problem as a multi-variable function, proving critical points, non-convexity and conjecturing positive-semidefinite Hessians.

II Statement of the distillability problem

The open problem of equivalence between PPT entanglement and bound entanglement can be resolved by finding bound entangled NPT states. Since Peres [26] has already shown that NPT is a sufficient condition for entanglement, attention can be limited to the state being both “bound”, which is, N-undistillable for arbitrarily large N, and NPT, which is, having a negative partial transpose. Compared to ascertaining positive semidefiniteness of a certain matrix, the major difficulty usually lies in finding a concise mathematical interpretation for undistillability, and asserting it for two types of arbitrariness: arbitrary LOCC operation and arbitrarily finitely many copies of the entangled state. This will be the main focus of this section, and the analysis of mathematical structure will eventually lead to a transformation that reduces N-undistillability verification to 1-undistillability verification of a transformed state.

Let’s recall the concept of Schmidt decomposition, Schmidt coefficients and Schmidt rank [27]. Schmidt decomposition of a pure state |ψ|\psi\rangle in AB\mathcal{H}_{A}\otimes\mathcal{H}_{B} is:

|ψ=i=1dαi|uivi,|\psi\rangle=\sum_{i=1}^{d}\alpha_{i}|u_{i}v_{i}\rangle, (1)

where A\mathcal{H}_{A} and B\mathcal{H}_{B} are both d-dimensional Hilbert spaces, with {|u1,,|ud}\{|u_{1}\rangle,\cdots,|u_{d}\rangle\} and {|v1,,|vd}\{|v_{1}\rangle,\cdots,|v_{d}\rangle\} as their respective orthonormal bases. Schmidt coefficients αi\alpha_{i} are real, nonnegative and unique up to re-ordering. The number of non-zero Schmidt coefficients is called Schmidt rank of pure state |ψ|\psi\rangle. SR(|ψ)SR(|\psi\rangle) denotes the Schmidt rank of |ψ|\psi\rangle.

A bipartite quantum state is called N-distillable if pure Bell states can be obtained using LOCC, from N-copies of the state. It has been proven in [28] that all entangled 2×22\times 2 bipartite quantum states are distillable, therefore, all we need to do is transform the original quantum state into a 2×22\times 2 entangled state by LOCC. This is demonstrated in the following result: A bipartite quantum state ρ\rho on AB\mathcal{H}_{A}\otimes\mathcal{H}_{B} is N-undistillable iff for any dN×dNd^{N}\times d^{N} bipartite pure state |ψSR2|\psi^{SR\leq 2}\rangle on ANBN\mathcal{H}_{A}^{\otimes N}\otimes\mathcal{H}_{B}^{\otimes N} with Schmidt rank \leq 2, the following holds:

ψSR2|(ρTA)N|ψSR20,\langle\psi^{SR\leq 2}|(\rho^{T_{A}})^{\otimes N}|\psi^{SR\leq 2}\rangle\geq 0, (2)

where ρTA=(TI)ρ\rho^{T_{A}}=(T\otimes I)\rho is the partial transpose of ρ\rho, with TT being the transpose operator. The above expression overlooks the pairing between different subsystems and so an additional operator MNM_{N} from (AB)N(\mathcal{H}_{A}\otimes\mathcal{H}_{B})^{\otimes N} to ANBN\mathcal{H}_{A}^{\otimes N}\otimes\mathcal{H}_{B}^{\otimes N} is introduced to make it meaningful:

Definition II.1.

Operator MN:(AB)NANBNM_{N}:(\mathcal{H}_{A}\otimes\mathcal{H}_{B})^{\otimes N}\to\mathcal{H}_{A}^{\otimes N}\otimes\mathcal{H}_{B}^{\otimes N} is defined as:

MN=|iA1iANiB1iBNiA1iB1iANiBN|,M_{N}=\sum|i_{A_{1}}\dots i_{A_{N}}i_{B_{1}}\dots i_{B_{N}}\rangle\langle i_{A_{1}}i_{B_{1}}\dots i_{A_{N}}i_{B_{N}}|, (3)

where AN=A1A2AN\mathcal{H}_{A}^{\otimes N}=\mathcal{H}_{A_{1}}\otimes\mathcal{H}_{A_{2}}\otimes\cdots\otimes\mathcal{H}_{A_{N}} , BN=B1B2BN\mathcal{H}_{B}^{\otimes N}=\mathcal{H}_{B_{1}}\otimes\mathcal{H}_{B_{2}}\otimes\cdots\otimes\mathcal{H}_{B_{N}}, and iAj,iBji_{A_{j}},i_{B_{j}} stands for the index corresponding to system Aj,BjA_{j},B_{j}.

Operator MNM_{N} then takes the A1B1A2B2ANBNA_{1}B_{1}A_{2}B_{2}\cdots A_{N}B_{N} structure of (ρTA)N(\rho^{T_{A}})^{\otimes N} and merges their A-subsystems and B-subsystems, resulting in a structure of A1A2ANB1B2BNA_{1}A_{2}\cdots A_{N}B_{1}B_{2}\cdots B_{N} that suits the pure quantum state, thus explicitly demonstrating the process of system pairing which is essential to any further calculations derived from this representation of undistillability.

For better representation of undistillability and further use in following sections, we use a certain state-operator isomorphism introduced in [24]. We notice that it is in essence a Choi-Jamiokowski isomorphism followed by a transposition on the resulting matrix. For convenience and consistency with previous works, we stick to this “transposed Choi-Jamiokowski isomorphism” when presenting our findings.

Definition II.2 (State-operator isomorphism [24]).

A state-operator isomorphism Ψ\Psi is one that takes a pure bipartite state |ψ|\psi\rangle of:

|ψ=ijαij|ij,|\psi\rangle=\sum_{ij}\alpha_{ij}|ij\rangle, (4)

to a matrix form of:

Ψ(|ψ)=(α00α01α0,d1α10α11α1,d1αd1,0αd1,1αd1,d1).\Psi(|\psi\rangle)=\begin{pmatrix}\alpha_{00}&\alpha_{01}&\cdots&\alpha_{0,d-1}\\ \alpha_{10}&\alpha_{11}&\cdots&\alpha_{1,d-1}\\ \vdots&\vdots&\ddots&\vdots\\ \alpha_{d-1,0}&\alpha_{d-1,1}&\cdots&\alpha_{d-1,d-1}\\ \end{pmatrix}. (5)

Note that Schmidt decomposition of a pure quantum state |ψ|\psi\rangle is related to the singular value decomposition of Ψ(|ψ)\Psi(|\psi\rangle) through state-operator isomorphism. In fact, Schmidt coefficients of |ψ|\psi\rangle is the same as the singular values of Ψ(|ψ)\Psi(|\psi\rangle), and Schmidt rank of |ψ|\psi\rangle is equal to the rank of Ψ(|ψ)\Psi(|\psi\rangle).

The following is a more concise mathematical representation of N-undistillability: A bipartite quantum state ρ\rho is N-undistillable iff:

[Ψ1(X2)]MN(ρTA)NMNΨ1(X2)0,[\Psi^{-1}(X_{2})]^{\dagger}M_{N}(\rho^{T_{A}})^{\otimes N}M_{N}^{\dagger}\Psi^{-1}(X_{2})\geq 0, (6)

where X2X_{2} is any dN×dNd^{N}\times d^{N} matrix of rank 2\leq 2. Note that Ψ1(X2)\Psi^{-1}(X_{2}) is equivalent to |ψSR2|\psi^{SR\leq 2}\rangle, a pure bipartite quantum state with Schmidt rank no larger than 2. For the case of N=1N=1, 1-undistillability is:

[Ψ1(X2)]ρTAΨ1(X2)=ψSR2|ρTA|ψSR20.[\Psi^{-1}(X_{2})]^{\dagger}\rho^{T_{A}}\Psi^{-1}(X_{2})=\langle\psi^{SR\leq 2}|\rho^{T_{A}}|\psi^{SR\leq 2}\rangle\geq 0. (7)

Effectively, the problem of ρ\rho being N-copy undistillable is equivalent to the problem of MN(ρN)MNM_{N}(\rho^{\otimes N})M_{N}^{\dagger} being 1-undistillable, but on a Hilbert space with higher dimensions AB\mathcal{H^{\prime}}_{A}\otimes\mathcal{H^{\prime}}_{B}, dim(A)=dim(B)=dNdim(\mathcal{H^{\prime}}_{A})=dim(\mathcal{H^{\prime}}_{B})=d^{N}.

Since discussions of 1-copy distillability problem rarely involves specification of finite dimensional Hilbert space dimensionality, and most of the theorems and methods are applicable to arbitrary dimensions, this transformation poses an advantage. In the next section, a specific symmetry of M2NM_{2^{N}} transformations is utilized for decomposing the increasingly complicated structure of M2NM_{2^{N}} into identical steps repeated for NN times. In fact, verification of 2N2^{N}-undistillability is enough to assert bound entanglement.

III N-undistillability problem as repeated steps

From the observation that (N+1)-undistillability implies N-undistillability, we can get the following result which relaxes the N-undistillability requirement for all N to only an infinite sequence of N diverging to infinity:

Proposition III.1.

{gi}\{g_{i}\} is a sequence of positive real numbers diverging to infinity. A bipartite entangled quantum state is gig_{i}-undistillable for arbitrary i, iff the state is bound entangled.

In the 2-copy case, M2M_{2} transformation is simply:

E=M2=|iA1iA2iB1iB2iA1iB1iA2iB2|,E=M_{2}=\sum|i_{A_{1}}i_{A_{2}}i_{B_{1}}i_{B_{2}}\rangle\langle i_{A_{1}}i_{B_{1}}i_{A_{2}}i_{B_{2}}|, (8)

which is merely an exchange of the second and third parts of B1B_{1} and A2A_{2}. From now on we will always refer to the 2-copy case of M2M_{2} as EE, emphasizing that it is only a simple exchange as opposed to complicated MNM_{N} of larger copy numbers.

According to Eq.6, the quantum state ρ\rho is 2-undistillable iff E(ρρ)EE(\rho\otimes\rho)E^{\dagger} is 1-undistillable.

In the 4-copy case, M4M_{4} can actually be decomposed into two steps:

A1B1A2B2A3B3A4B4\displaystyle A_{1}B_{1}A_{2}B_{2}A_{3}B_{3}A_{4}B_{4} (9)
\displaystyle\to A1A2B1B2A3A4B3B4\displaystyle A_{1}A_{2}B_{1}B_{2}A_{3}A_{4}B_{3}B_{4}
\displaystyle\to A1A2A3A4B1B2B3B4.\displaystyle A_{1}A_{2}A_{3}A_{4}B_{1}B_{2}B_{3}B_{4}.

Step 1: do the 2-copy exchange on subsystems 1,2 (A1B1A2B2A1A2B1B2A_{1}B_{1}A_{2}B_{2}\to A_{1}A_{2}B_{1}B_{2}) and subsystems 3,4 (A3B3A4B4A3A4B3B4A_{3}B_{3}A_{4}B_{4}\to A_{3}A_{4}B_{3}B_{4}). This step is no different than in the 2-copy case, except that it is done on two systems simultaneously. Group every neighbouring 2 subsystems(in terms of A,BA,B), so that the eight parts are now seen as four parts (A1A2,B1B2,A3A4,B3B4A_{1}A_{2},B_{1}B_{2},A_{3}A_{4},B_{3}B_{4} to ABABABAB). In order to separate this newly obtained four-part state from 2-copy Werner states, we denote this state ρ(e)ρ(e)\rho(e)\otimes\rho(e), where ρ(e)=E(ρρ)E\rho(e)=E(\rho\otimes\rho)E^{\dagger}.

Step 2: Do the 2-copy exchange EE again, obtaining ρ(e2)=E(ρ(e)ρ(e))E\rho(e^{2})=E(\rho(e)\otimes\rho(e))E^{\dagger}, where EE is taken with regard to the “merged” parts. This step takes once-transformed Werner states into twice-transformed Werner states.

The above steps of repeating the EE transformation twice, is equivalent to doing the M4M_{4} translations directly. The original state ρ\rho is 4-copy undistillable iff ρ(e2)\rho(e^{2}) is one-copy undistillable.

Similarly, in the 2N2^{N}-copy case, E is decomposed into N steps, with each step taking state ρ(ei1)ρ(ei1)\rho(e^{i-1})\otimes\rho(e^{i-1}), producing a state ρ(ei)=E(ρ(ei1)ρ(ei1))E\rho(e^{i})=E(\rho(e^{i-1})\otimes\rho(e^{i-1}))E^{\dagger}, verifying its positivity on Schmidt rank 2\leq 2 states and effectively ascertaining 2i2^{i}-copy undistillability, before passing two copies of this state on, as a starting state for the next step. The following theorem demonstrates the process.

Theorem III.2.

Define ρ(e0)=ρ\rho(e^{0})=\rho to be the initial state, and

ρ(ek)=E(ρ(ek1)ρ(ek1))E,\rho(e^{k})=E(\rho(e^{k-1})\otimes\rho(e^{k-1}))E^{\dagger}, (10)

then ρ(ek)\rho(e^{k}) being 1-undistillable is equivalent to ρ\rho being 2k2^{k}-undistillable.

In other words, we are essentially searching for an infinite sequence of points connected by the operation EE, with the first point being ρ=ρ(e0)\rho=\rho(e^{0}), second point being ρ(e1)=E(ρ(e0)ρ(e0))E\rho(e^{1})=E(\rho(e^{0})\otimes\rho(e^{0}))E^{\dagger}, and the (i+2)(i+2)-th point being ρ(ei+1)=E(ρ(ei)ρ(ei))E\rho(e^{i+1})=E(\rho(e^{i})\otimes\rho(e^{i}))E^{\dagger}. If points of this infinite sequence always fall within the set of 1-undistillability, then we can safely say that the starting point ρ\rho is N-undistillable for arbitrary N, or that it is a bound state.

IV Bounds for Werner state N-undistillability

IV.1 Werner state 1-undistillability and NPT condition

It has been shown in [23] that it is sufficient to only consider Werner states for NPT bound problem, that if an NPT bound state exists, there must be an NPT bound state within the family of Werner states. Necessary and sufficient conditions of Werner state 1-undistillability and partial transpose negativity are obtained in this section.

We first introduce a lemma that would assist further attempts concerning inner product with Schmidt rank 2\leq 2 pure states:

Lemma IV.1.

Let |ψ|\psi\rangle be an arbitrary pure quantum state and sjs_{j} are the Schmidt coefficients of |ψ|\psi\rangle arranged in descending order, then

j=1ksj2=max|ϕSRk|ψ|ϕSRk|2,\;\sum_{j=1}^{k}s_{j}^{2}=max_{|\phi^{SR\leq k}\rangle}|\langle\psi|\phi^{SR\leq k}\rangle|^{2}, (11)

where |ϕSRk|\phi^{SR\leq k}\rangle is an arbitrary quantum pure state with Schimidt rank being less than k, namely, SR(|ϕSRk)kSR(|\phi^{SR\leq k}\rangle)\leq k.

Proof of this lemma is provided in Appendix A.

A Werner state is as follows:

ρw=1d2+βd(I+βF),\rho_{w}=\frac{1}{d^{2}+\beta d}(I+\beta F), (12)

where F=ij|ijji|F=\sum_{ij}|ij\rangle\langle ji|, II is the unnormalized identity matrix, d denote the dimensionality of both parts of the system, and β\beta is a parameter characterizing the “portion” of swap operator FF, ranging in 1β1-1\leq\beta\leq 1.

Its partial transpose is:

ρwTA=1d2+βd(I+βG),\rho_{w}^{T_{A}}=\frac{1}{d^{2}+\beta d}(I+\beta G), (13)

where G=ij|iijj|G=\sum_{ij}|ii\rangle\langle jj|, which is in fact the unnormalized density matrix of a pure maximally entangle state |Φ|\Phi\rangle, namely,

G=d|ΦΦ|,|Φ=i1d|ii.G=d|\Phi\rangle\langle\Phi|,\;|\Phi\rangle=\sum_{i}\frac{1}{\sqrt{d}}|ii\rangle. (14)

When β>0\beta>0, ρwTA\rho_{w}^{T_{A}} is always positive semidefinite, hence we consider β<0\beta<0 case only. Combining Eq.6 and Eq.11, we obtain

ψSR2|ρwTA|ψSR2\displaystyle\langle\psi^{SR\leq 2}|\rho_{w}^{T_{A}}|\psi^{SR\leq 2}\rangle (15)
=1d2+βd(1+βd|Φ|ψSR2|2)L.IV.11+2βd2+βd.\displaystyle=\frac{1}{d^{2}+\beta d}(1+\beta d|\langle\Phi|\psi^{SR\leq 2}\rangle|^{2})\stackrel{{\scriptstyle L.\ref{fact}}}{{\geq}}\frac{1+2\beta}{d^{2}+\beta d}.

A Werner state ρw\rho_{w} is 1-undistillable iff ψSR2|ρwTA|ψSR20\langle\psi^{SR\leq 2}|\rho_{w}^{T_{A}}|\psi^{SR\leq 2}\rangle\geq 0 for any |ψSR2|\psi^{SR\leq 2}\rangle pure bipartite quantum state of Schmidt rank no larger than 2. Therefore, Werner state is 1-undistillable iff β12\beta\geq-\frac{1}{2}.

Furthermore, for arbitrary quantum state |ψ|\psi\rangle, we have

ψ|ρwTA|ψ=1d2+βd(1+βd|Φ|ψ|2)1+βdd2+βd,\langle\psi|\rho_{w}^{T_{A}}|\psi\rangle=\frac{1}{d^{2}+\beta d}(1+\beta d|\langle\Phi|\psi\rangle|^{2})\geq\frac{1+\beta d}{d^{2}+\beta d}, (16)

with the equality achieved when |ψ=|Φ|\psi\rangle=|\Phi\rangle. Therefore, Werner state is NPT iff β<1d\beta<-\frac{1}{d}. Any NPT 1-undistillable Werner state can therefore only be found within the parameter range of 12β<1d-\frac{1}{2}\leq\beta<-\frac{1}{d}, provided d>2d>2.

IV.2 Sufficient conditions for Werner state N-undistillability

We derive new bounds for Werner state N-undistillability in this section. As a result, for any finite N, a set of N-undistillable states can be found, but similar to the circumstances encountered in [18], [19] and [20], the set of N-undistillable states shrinks to emptiness as N approaches infinity.

In the previous section it has been established that Werner state N-undistillability is equivalent to:

ψSR2|MN(ρwTA)NMN|ψSR20,\langle\psi^{SR\leq 2}|M_{N}(\rho_{w}^{T_{A}})^{\otimes N}M_{N}^{\dagger}|\psi^{SR\leq 2}\rangle\geq 0, (17)

where |ψSR2|\psi^{SR\leq 2}\rangle is an arbitrary quantum pure state with Schmidt rank being no larger than 2.

Take the 2-copy case as an example, recalling operation EE defined in Eq.8:

E(ρwTAρwTA)E=(1d2+βd)2(E(II)E\displaystyle E(\rho_{w}^{T_{A}}\otimes\rho_{w}^{T_{A}})E^{\dagger}=(\frac{1}{d^{2}+\beta d})^{2}(E(I\otimes I)E^{\dagger} (18)
+β[E(IG)E+E(GI)E]+β2E(GG)E).\displaystyle+\beta[E(I\otimes G)E^{\dagger}+E(G\otimes I)E^{\dagger}]+\beta^{2}E(G\otimes G)E^{\dagger}).

The normalization factor of (1d2+βd)2(\frac{1}{d^{2}+\beta d})^{2} can be ignored since it doesn’t affect positivity. The first and the last term remains unchanged in the sense that:

E(II)E=E(ijkl|ijklijkl|)E=ijkl|ikjlikjl|\displaystyle E(I\otimes I)E^{\dagger}=E(\sum_{ijkl}|ijkl\rangle\langle ijkl|)E^{\dagger}=\sum_{ijkl}|ikjl\rangle\langle ikjl| (19)
=I(e),\displaystyle=I(e),

with I(e)I(e) still being the identity matrix, only that it exists on a higher dimensionality of d4×d4d^{4}\times d^{4}. Similarly,

E(GG)E=E(ijkl|iikkjjll|)E=ijkl|ikikjljl|\displaystyle E(G\otimes G)E^{\dagger}=E(\sum_{ijkl}|iikk\rangle\langle jjll|)E^{\dagger}=\sum_{ijkl}|ikik\rangle\langle jljl| (20)
=G(e),\displaystyle=G(e),

with G(e)=|Φ(e)Φ(e)|G(e)=|\Phi(e)\rangle\langle\Phi(e)| still being the pure state density matrix of unnormalized |Φ(e)=ij|ijij|\Phi(e)\rangle=\sum_{ij}|ijij\rangle, only that it exists on a higher dimensionality of d4×d4d^{4}\times d^{4}.

Regarding the positivity of the middle part E(IG)E+E(GI)EE(I\otimes G)E^{\dagger}+E(G\otimes I)E^{\dagger} on |ψSR2|\psi^{SR\leq 2}\rangle,

E(IG)E=E(ijkl|ijkkijll|)E=ijkl|ikjkiljl|\displaystyle E(I\otimes G)E^{\dagger}=E(\sum_{ijkl}|ijkk\rangle\langle ijll|)E^{\dagger}=\sum_{ijkl}|ikjk\rangle\langle iljl| (21)
=d(|ψ00s2=s4ψ00s2=s4|++|ψd1,d1s2=s4ψd1,d1s2=s4|)\displaystyle=d(|\psi_{00}^{s_{2}=s_{4}}\rangle\langle\psi_{00}^{s_{2}=s_{4}}|+\dots+|\psi_{d-1,d-1}^{s_{2}=s_{4}}\rangle\langle\psi_{d-1,d-1}^{s_{2}=s_{4}}|)
=dij|ψijs2=s4ψijs2=s4|,\displaystyle=d\sum_{ij}|\psi_{ij}^{s_{2}=s_{4}}\rangle\langle\psi_{ij}^{s_{2}=s_{4}}|,

where|ψijs2=s4=1dk=0d1|ikjk|\psi^{s_{2}=s_{4}}_{ij}\rangle=\frac{1}{\sqrt{d}}\sum_{k=0}^{d-1}|ikjk\rangle is the superposition of all multipartite states with identical states on the second and fourth subsystems, while their first and third subsystems are of states i and j respectively. |ψijs2=s4|\psi^{s_{2}=s_{4}}_{ij}\rangle is a normalized pure state of Schmidt rank d, and all Schmidt coefficients are 1d\frac{1}{\sqrt{d}}. Do a decomposition of |ψSR2|\psi^{SR\leq 2}\rangle in the following way:

|ψSR2=ijpij|ψijSR2,|\psi^{SR\leq 2}\rangle=\sum_{ij}p_{ij}|\psi^{SR\leq 2}_{ij}\rangle, (22)

where |ψijSR2|\psi^{SR\leq 2}_{ij}\rangle represents the normalized extraction of all |ij|i-j-\rangle terms from the state of |ψSR2|\psi^{SR\leq 2}\rangle. More specifically, for state |ψSR2|\psi^{SR\leq 2}\rangle of:

|ψSR2=abcdpabcd|abcd,|\psi^{SR\leq 2}\rangle=\sum_{abcd}p_{abcd}|abcd\rangle, (23)

the corresponding |ψijSR2|\psi^{SR\leq 2}_{ij}\rangle is:

|ψijSR2=1Npabpiajb|iajb,|\psi^{SR\leq 2}_{ij}\rangle=\frac{1}{N_{p}}\sum_{ab}p_{iajb}|iajb\rangle, (24)

where Np=ab|piajb|2N_{p}=\sqrt{\sum_{ab}|p_{iajb}|^{2}}.

It can be proven that the normalized extraction of all |ixjy|ixjy\rangle terms must also have Schmidt rank 2\leq 2. Consider state-operator isomorphism in Def.II.2, the Schmidt rank of |ψ|\psi\rangle is equivalent to the rank of the matrix Ψ(|ψ)\Psi(|\psi\rangle). The normalized extraction of all |ij|i-j-\rangle terms composes a new state of |ψijSR2|\psi^{SR\leq 2}_{ij}\rangle, therefore, its corresponding matrix is a submatrix of Ψ(|ψSR2)\Psi(|\psi^{SR\leq 2}\rangle), composed of rows i×d+xi\times d+x and columns j×d+yj\times d+y, with x,y taking values from {0,,d1}\{0,\dots,d-1\}. Since the rank of a submatrix is never larger than the rank of the whole matrix, |ψijSR2|\psi^{SR\leq 2}_{ij}\rangle must have Schmidt rank less than or equal to that of |ψSR2|\psi^{SR\leq 2}\rangle.

Using Lem.IV.1 again, it is then clear that:

|ψijSR2|ψpqs2=s4|2=|ψijSR2|ψijs2=s4|2δipδjqL.IV.12dδipδjq.|\langle\psi_{ij}^{SR\leq 2}|\psi_{pq}^{s_{2}=s_{4}}\rangle|^{2}=|\langle\psi_{ij}^{SR\leq 2}|\psi_{ij}^{s_{2}=s_{4}}\rangle|^{2}\delta_{ip}\delta_{jq}\stackrel{{\scriptstyle L.\ref{fact}}}{{\leq}}\frac{2}{d}\delta_{ip}\delta_{jq}. (25)

It follows that:

ψSR2|E(IG)E|ψSR2=dij|pij|2|ψijSR2|ψijs2=s4|2\displaystyle\langle\psi^{SR\leq 2}|E(I\otimes G)E^{\dagger}|\psi^{SR\leq 2}\rangle=d\sum_{ij}|p_{ij}|^{2}|\langle\psi_{ij}^{SR\leq 2}|\psi_{ij}^{s_{2}=s_{4}}\rangle|^{2} (26)
2ij|pij|2=2.\displaystyle\leq 2\sum_{ij}|p_{ij}|^{2}=2.

A similar analysis is applied to E(GI)EE(G\otimes I)E^{\dagger}, getting

ψSR2|E(GI)E|ψSR2=dij|qij|2|ϕijSR2|ψijs1=s3|2\displaystyle\langle\psi^{SR\leq 2}|E(G\otimes I)E^{\dagger}|\psi^{SR\leq 2}\rangle=d\sum_{ij}|q_{ij}|^{2}|\langle\phi_{ij}^{SR\leq 2}|\psi_{ij}^{s_{1}=s_{3}}\rangle|^{2} (27)
2ij|qij|2=2.\displaystyle\leq 2\sum_{ij}|q_{ij}|^{2}=2.

A sufficient condition for Werner state 2-undistillability is:

ψSR2|I(e)+β2G(e)+βE(IG+GI)E|ψSR2\displaystyle\langle\psi^{SR\leq 2}|I(e)+\beta^{2}G(e)+\beta E(I\otimes G+G\otimes I)E^{\dagger}|\psi^{SR\leq 2}\rangle (28)
1+β2|Ψ(e)|ψSR2|2+4β1+4β0.\displaystyle\geq 1+\beta^{2}|\langle\Psi(e)|\psi^{SR\leq 2}\rangle|^{2}+4\beta\geq 1+4\beta\geq 0.

Therefore we can conclude that when β14\beta\geq-\frac{1}{4}, ρw\rho_{w} must be 2-undistillable.

A similar process is followed in the arbitrary N case, yielding a lower bound regarding all the odd terms in (1+β)N(1+\beta)^{N}. Since the odd terms in (1+β)N(1+\beta)^{N} can be expressed by (1+β)N(1β)N2\frac{(1+\beta)^{N}-(1-\beta)^{N}}{2}, a lower bound can then be obtained for the N-undistillability case:

Theorem IV.2.

Let β0\beta_{0} be the zero point of 1+(1+β)N(1β)N1+(1+\beta)^{N}-(1-\beta)^{N} within [1,0][-1,0]. When ββ0\beta\geq\beta_{0}, Werner state ρw\rho_{w} is N-undistillable.

Proof of this is presented in Appendix B. By calculating the zero point a lower bound is obtained where the corresponding Werner state is N-undistillable. Note that unlike in previous works, this bound β0\beta_{0} is also independent of dimensionality dd. By subsequently raising the dimensionality of Werner states within the set, thus raising 1d-\frac{1}{d}, we can always obtain a set of Werner states that falls into [β0,1d)[\beta_{0},-\frac{1}{d}), which means that they are both NPT and N-undistillable for any finite N. However, as N increases, higher dimensionality are required for undistillability, and so the subset of N-undistillable NPT states shrinks to zero as N approaches to infinity, which is similar to the circumstances encountered in [18], [19] and [20]. Therefore, this method fails to find a state that is undistillable for arbitrarily many copies, while being NPT at the same time.

V The problem as a partial trace inequality

The problem of Werner state N-undistillability can be equivalently written as inequalities regarding the Frobenius norm of partial traces of a rank-2 matrix.

Take 2-undistillability as an example. ψSR2|E(IG+GI)E|ψSR2\langle\psi^{SR\leq 2}|E(I\otimes G+G\otimes I)E^{\dagger}|\psi^{SR\leq 2}\rangle can be written with regard to the Frobenius norms of two partial traces:

ψSR2|E(IG)E|ψSR2=Tr2(X2(ψ))F2,\langle\psi^{SR\leq 2}|E(I\otimes G)E^{\dagger}|\psi^{SR\leq 2}\rangle=||Tr_{2}(X_{2}(\psi))||_{F}^{2}, (29)
ψSR2|E(GI)E|ψSR2=Tr1(X2(ψ))F2,\langle\psi^{SR\leq 2}|E(G\otimes I)E^{\dagger}|\psi^{SR\leq 2}\rangle=||Tr_{1}(X_{2}(\psi))||_{F}^{2}, (30)

where ||||F||\cdot||_{F} denotes Frobenius norm:

XF=ij|Xij|2=Tr(XX).||X||_{F}=\sqrt{\sum_{ij}|X_{ij}|^{2}}=\sqrt{Tr(X^{\dagger}X)}. (31)

X2(ψ)X_{2}(\psi) is a d2×d2d^{2}\times d^{2} matrix of rank \leq 2, obtained by state-operator isomorphism, from |ψSR2|\psi^{SR\leq 2}\rangle, a pure bipartite d2×d2d^{2}\times d^{2} state with Schmidt rank \leq 2. For simplicity, we will be writing it as X2X_{2} from now on.

The normalization of |ψSR2|\psi^{SR\leq 2}\rangle requires that X2F2=Tr(X2X2)=1||X_{2}||_{F}^{2}=Tr(X_{2}^{\dagger}X_{2})=1. Now the problem of Werner state 2-undistillability is equivalent to: Find a range of β\beta that makes the following inequality always holds for arbitrary X2X_{2} with rank no larger than 2 (The requirement of X2F2=1||X_{2}||_{F}^{2}=1 can be lifted due to homogeneity):

X2F2+β2|Tr(X2)|2\displaystyle||X_{2}||_{F}^{2}+\beta^{2}|Tr(X_{2})|^{2} (32)
+β(Tr1(X2)F2+Tr2(X2)F2)0.\displaystyle+\beta(||Tr_{1}(X_{2})||_{F}^{2}+||Tr_{2}(X_{2})||_{F}^{2})\geq 0.

N-undistillability has a similar form:

Theorem V.1.

Werner state ρw\rho_{w} is N-undistillable iff the following holds for all dN×dNd^{N}\times d^{N} X2X_{2}:

S{1,,N}β|S|TrS(X2)F20,\displaystyle\sum_{S\subset\{1,\cdots,N\}}\beta^{|S|}||Tr_{S}(X_{2})||_{F}^{2}\geq 0, (33)

where TrSTr_{S} takes partial traces of the subsystems in set SS.

The proof of this is presented in Appendix C. A similar result is obtained by [29].

The partial trace inequalities are with regard to a matrix X2X_{2} of rank one or two. From now on we consider the case where β\beta is taken to be 12-\frac{1}{2} according to popular guess. For 2-undistillability problem, The rank one case can be trivially proved by making use of the following lemma:

Lemma V.2.

The inequalities:

Tr1(X1)F2X1F2,Tr2(X1)F2X1F2,||Tr_{1}(X_{1})||_{F}^{2}\leq||X_{1}||_{F}^{2},||Tr_{2}(X_{1})||_{F}^{2}\leq||X_{1}||_{F}^{2}, (34)

hold for any d2×d2d^{2}\times d^{2} square matrix X1X_{1} of rank one.

Proof of this lemma is presented in Appendix E. For X2X_{2} of rank two, the inequality of concern when β=12\beta=-\frac{1}{2} is:

Tr2(X2)F2+Tr1(X2)F212|Tr(X2)|22X2F2=2.||Tr_{2}(X_{2})||_{F}^{2}+||Tr_{1}(X_{2})||_{F}^{2}-\frac{1}{2}|Tr(X_{2})|^{2}\leq 2||X_{2}||_{F}^{2}=2. (35)

For any square matrix X2X_{2} of rank two, the singular decomposition can be applied, decomposing the matrix as the sum of two rank one matrices:

X2=σ1X21+σ2X22=σ1𝐮1𝐯1+σ2𝐮2𝐯2,X_{2}=\sigma_{1}X_{2}^{1}+\sigma_{2}X_{2}^{2}=\sigma_{1}\mathbf{u}^{1}\mathbf{v}^{1\dagger}+\sigma_{2}\mathbf{u}^{2}\mathbf{v}^{2\dagger}, (36)

where σ12+σ22=1\sigma_{1}^{2}+\sigma_{2}^{2}=1, and both σ1\sigma_{1} and σ2\sigma_{2} are positive. We introduce d×dd\times d matrices U1,U2,V1,V2U_{1},U_{2},V_{1},V_{2} that are the result of state-operator isomorphisms, corresponding to 𝐮1,𝐮2,𝐯1,𝐯2\mathbf{u}^{1},\mathbf{u}^{2},\mathbf{v}^{1},\mathbf{v}^{2} respectively.

Eq.35 then becomes:

σ12(Tr(V1U1U1V1)+Tr(U1V1V1U1))\displaystyle\sigma_{1}^{2}(Tr(V_{1}U_{1}^{\dagger}U_{1}V_{1}^{\dagger})+Tr(U_{1}^{\dagger}V_{1}V_{1}^{\dagger}U_{1})) (37)
+σ22(Tr(V2U2U2V2)+Tr(U2V2V2U2))\displaystyle+\sigma_{2}^{2}(Tr(V_{2}U_{2}^{\dagger}U_{2}V_{2}^{\dagger})+Tr(U_{2}^{\dagger}V_{2}V_{2}^{\dagger}U_{2}))
+σ1σ22Re[Tr(V1U1U2V2)+Tr(U1V1V2U2)]\displaystyle+\sigma_{1}\sigma_{2}2Re[Tr(V_{1}U_{1}^{\dagger}U_{2}V_{2}^{\dagger})+Tr(U_{1}^{\dagger}V_{1}V_{2}^{\dagger}U_{2})]
|σ1Tr(U1V1)+σ2Tr(U2V2)|222.\displaystyle-\frac{|\sigma_{1}Tr(U_{1}V_{1}^{\dagger})+\sigma_{2}Tr(U_{2}V_{2}^{\dagger})|^{2}}{2}\leq 2.

For simplicity the above is rewritten as:

σ12P+σ22Q+σ1σ2R2,\sigma_{1}^{2}P+\sigma_{2}^{2}Q+\sigma_{1}\sigma_{2}R\leq 2, (38)

where P,Q,RP,Q,R are:

P=Tr(U1V1V1U1)+Tr(V1U1U1V1)|Tr(U1V1)|22,P=Tr(U_{1}^{\dagger}V_{1}V_{1}^{\dagger}U_{1})+Tr(V_{1}U_{1}^{\dagger}U_{1}V_{1}^{\dagger})-\frac{|Tr(U_{1}V_{1}^{\dagger})|^{2}}{2}, (39)
Q=Tr(U2V2V2U2)+Tr(V2U2U2V2)|Tr(U2V2)|22,Q=Tr(U_{2}^{\dagger}V_{2}V_{2}^{\dagger}U_{2})+Tr(V_{2}U_{2}^{\dagger}U_{2}V_{2}^{\dagger})-\frac{|Tr(U_{2}V_{2}^{\dagger})|^{2}}{2}, (40)
R=2Re[Tr(V1U1U2V2)+Tr(U1V1V2U2)\displaystyle R=2Re[Tr(V_{1}U_{1}^{\dagger}U_{2}V_{2}^{\dagger})+Tr(U_{1}^{\dagger}V_{1}V_{2}^{\dagger}U_{2}) (41)
Tr(U1V1)Tr(U2V2)2].\displaystyle-\frac{Tr^{*}(U_{1}V_{1}^{\dagger})Tr(U_{2}V_{2}^{\dagger})}{2}].

Maximization regarding variables σ1,σ2\sigma_{1},\sigma_{2} reduces the question to proving:

R24(2P)(2Q),R^{2}\leq 4(2-P)(2-Q), (42)

with normalization and orthogonality conditions requiring:

U1F2=V1F2=U2F2=V2F2=1,||U_{1}||_{F}^{2}=||V_{1}||_{F}^{2}=||U_{2}||_{F}^{2}=||V_{2}||_{F}^{2}=1, (43)

and

tr(V2V1)=tr(U2U1)=0.tr(V_{2}^{\dagger}V_{1})=tr(U_{2}^{\dagger}U_{1})=0. (44)

The special case of U1=V1U_{1}=V_{1}, in other words, X2X_{2} being the sum of a normal matrix and a rank-1 matrix, has been proved in [29].

In fact, by a slight change of representation, we can also get an equivalent expression of Werner state N-undistillability inequality, regarding only rank one matrices:

Theorem V.3.

Werner state ρw\rho_{w} is N-undistillable iff

Re[fN(X1,X1)]2fN(X1,X1)fN(X1,X1),Re[f_{N}(X_{1},X^{\prime}_{1})]^{2}\leq f_{N}(X^{\prime}_{1},X^{\prime}_{1})f_{N}(X_{1},X_{1}), (45)

where

fN(X1,X1)=S{1,,N}β|S|Tr[TrS(X1)TrS(X1)]0,\displaystyle f_{N}(X_{1},X^{\prime}_{1})=\sum_{S\subset\{1,\cdots,N\}}\beta^{|S|}Tr[Tr^{\dagger}_{S}(X_{1})Tr_{S}(X^{\prime}_{1})]\geq 0, (46)

where X1=𝐰𝐱,X1=𝐲𝐳X_{1}=\mathbf{w}^{\dagger}\mathbf{x},X^{\prime}_{1}=\mathbf{y}^{\dagger}\mathbf{z} are dN×dNd^{N}\times d^{N} rank one matrices, and their component vectors 𝐰,𝐱,𝐲,𝐳\mathbf{w},\mathbf{x},\mathbf{y},\mathbf{z} satisfy 𝐰𝐲,𝐱𝐳\mathbf{w}\perp\mathbf{y},\mathbf{x}\perp\mathbf{z}.

Proof of this equivalence is presented in Appendix D.

It is then established that N-undistillability problem for arbitrary N can be written as inequalities concerning rank one matrices. Although the above form looks like a Cauchy-Schwartz inequality, fN(X1,X1)f_{N}(X_{1},X^{\prime}_{1}) cannot be seen as an inner product and enable the direct application of Cauchy-Schwartz inequality. fN(X1,X1)f_{N}(X_{1},X^{\prime}_{1}) is obviously conjugate symmetric, and for rank one matrices X1X_{1} and X1X^{\prime}_{1}, positivity of fN(X1,X1)f_{N}(X_{1},X_{1}) and fN(X1,X1)f_{N}(X^{\prime}_{1},X^{\prime}_{1}) can be ascertained. However, rank-one matrices do not compose a vector space, since the sum of two rank-one matrices can be a rank-two matrix. Although arbitrary finite rank matrices do compose a finite dimensional vector space, proving positivity of fN(A,A)f_{N}(A,A) for arbitrary rank matrix AA is both beyond our ability and our need, since proving positivity of fN(X2,X2)f_{N}(X_{2},X_{2}) for arbitrary rank two matrix X2X_{2} is, in fact, equivalent to Eq.33, and is enough for proof of N-undistillability.

VI Conversion to a multi-variable function

We make another attempt at this problem by seeing it as a multi-variable function. For simplicity we consider only the real case of the 2-distillability problem, that is, X1X_{1}, X1X^{\prime}_{1} are d2×d2d^{2}\times d^{2} real matrices. For convenience of expression we use f(C,D)=f2(X1,X1)f(C,D)=f_{2}(X_{1},X^{\prime}_{1}) to denote the function concerned. Thus, the 2-undistillability problem is equivalent to proving the following inequality for all d2×d2d^{2}\times d^{2}-dimensional rank one matrices C,DC,D:

f2(C,D)f(C,C)f(D,D),f^{2}(C,D)\leq f(C,C)f(D,D), (47)

where

f(C,D)=Tr(CTD)\displaystyle f(C,D)=Tr(C^{T}D) (48)
+β(Tr(C1TD1)+Tr(C2TD2))+β2Tr(CT)Tr(D),\displaystyle+\beta(Tr(C_{1}^{T}D_{1})+Tr(C_{2}^{T}D_{2}))+\beta^{2}Tr(C^{T})Tr(D),

where we have used Tr1(C)=C2,Tr2(C)=C1,Tr1(D)=D2,Tr2(D)=D1Tr_{1}(C)=C_{2},Tr_{2}(C)=C_{1},Tr_{1}(D)=D_{2},Tr_{2}(D)=D_{1} for simplicity. A multi-variable function g(C)g(C) is defined if we see DD as a constant D0D_{0}:

g(C)D0=f(C,C)f(D0,D0)f2(C,D0),g(C)_{D_{0}}=f(C,C)f(D_{0},D_{0})-f^{2}(C,D_{0}), (49)

where D0D_{0} is an arbitrary d2×d2d^{2}\times d^{2}-dimensional real matrix of rank 1. Both CC and D0D_{0} can be written as outer products of d2d^{2}-dimensional real vectors 𝐰\mathbf{w}, 𝐱,𝐲,𝐳\mathbf{x},\mathbf{y},\mathbf{z}:

C=𝐰𝐱T,D0=𝐲𝐳T.C=\mathbf{w}\mathbf{x}^{T},D_{0}=\mathbf{y}\mathbf{z}^{T}. (50)

The multi variables of function g(C)g(C) are taken to be the components of vector 𝐰,𝐱\mathbf{w},\mathbf{x}, represented by wij,xijw_{ij},x_{ij}. Indices i and j take their values in [0,1,,d1][0,1,\cdots,d-1], and are combined together to represent the (i×d+j)(i\times d+j)-th component of the vector. The problem is therefore transformed into proving that multi-variable function g(C)D0g(C)_{D_{0}} is always non-negative, for all variables wij,xijw_{ij},x_{ij} and all possible parameters yij,zijy_{ij},z_{ij}. It is clear that when C=D0C=D_{0}, g(D0)D0=f2(D0,D0)f2(D0,D0)=0g(D_{0})_{D_{0}}=f^{2}(D_{0},D_{0})-f^{2}(D_{0},D_{0})=0, and we conjecture that these are global minimums.

We first prove that the gradients at these points are zero regardless of the parameters 𝐲,𝐳\mathbf{y},\mathbf{z} by calculating the Jacobian matrix, therefore showing that the C=D0C=D_{0} points are indeed critical points. Then the Hessian matrix at this point is presented, in particular its three block parts, since the Hessian matrix is Hermitian. We conjecture that it is positive semidefinite. An additional proof of nonconvexity is also given in Appendix.F, thus eliminating the easy case where any local minimum is also a global minimum.

VI.1 The gradient at C=D0C=D_{0} is zero

For simplicity all g(C)D0g(C)_{D_{0}} are written as g(C)g(C) in the following text. Define

h1,ij(w,x)=2wij(pqxpq2)\displaystyle h_{1,ij}(w,x)=2w_{ij}\left(\sum_{pq}x_{pq}^{2}\right) (51)
+2β[pqxpjwiqxpq+pqxiqwpjxpq]\displaystyle+2\beta\left[\sum_{pq}x_{pj}w_{iq}x_{pq}+\sum_{pq}x_{iq}w_{pj}x_{pq}\right]
+2β2xij(pqwpqxpq)\displaystyle+2\beta^{2}x_{ij}\left(\sum_{pq}w_{pq}x_{pq}\right)
h2,ij(y,z,x)=yij(pqxpqzpq)\displaystyle h_{2,ij}(y,z,x)=y_{ij}\left(\sum_{pq}x_{pq}z_{pq}\right) (52)
+β[pqxpjyiqzpq+pqxiqypjzpq]\displaystyle+\beta\left[\sum_{pq}x_{pj}y_{iq}z_{pq}+\sum_{pq}x_{iq}y_{pj}z_{pq}\right]
+β2xij(pqypqzpq)\displaystyle+\beta^{2}x_{ij}\left(\sum_{pq}y_{pq}z_{pq}\right)

The partial derivatives of f(C,C)f(C,C) and f(C,D0)f(C,D_{0}) are:

f(C,C)wij=h1,ij(w,x),f(C,C)xij=h1,ij(x,w)\frac{\partial f(C,C)}{\partial w_{ij}}=h_{1,ij}(w,x),\frac{\partial f(C,C)}{\partial x_{ij}}=h_{1,ij}(x,w) (53)
f(C,D0)wij=h2,ij(y,z,x),f(C,D0)xij=h2,ij(z,y,w)\frac{\partial f(C,D_{0})}{\partial w_{ij}}=h_{2,ij}(y,z,x),\frac{\partial f(C,D_{0})}{\partial x_{ij}}=h_{2,ij}(z,y,w) (54)

Notice that h1,ij(w,x)=2h2,ij(w,x,x),h1,ij(x,w)=2h2,ij(x,w,w)h_{1,ij}(w,x)=2h_{2,ij}(w,x,x),h_{1,ij}(x,w)=2h_{2,ij}(x,w,w).

Therefore, at the critical points where C=D0C=D_{0},

f(C,D0)wij|C=D0=12f(C,C)wij|C=D0,\frac{\partial f(C,D_{0})}{\partial w_{ij}}|_{C=D_{0}}=\frac{1}{2}\frac{\partial f(C,C)}{\partial w_{ij}}|_{C=D_{0}}, (55)
f(C,D0)xij|C=D0=12f(C,C)xij|C=D0.\frac{\partial f(C,D_{0})}{\partial x_{ij}}|_{C=D_{0}}=\frac{1}{2}\frac{\partial f(C,C)}{\partial x_{ij}}|_{C=D_{0}}. (56)

It then follows that the Jacobian at the C=D0C=D_{0} point is zero:

g(C)wij|C=D0=f(D0,D0)f(C,C)wij|C=D0\displaystyle\frac{\partial g(C)}{\partial w_{ij}}|_{C=D_{0}}=f(D_{0},D_{0})\frac{\partial f(C,C)}{\partial w_{ij}}|_{C=D_{0}} (57)
2f(C,D0)wij|C=D0f(D0,D0)=0.\displaystyle-2\frac{\partial f(C,D_{0})}{\partial w_{ij}}|_{C=D_{0}}f(D_{0},D_{0})=0.
g(C)xij|C=D0=f(D0,D0)f(C,C)xij|C=D0\displaystyle\frac{\partial g(C)}{\partial x_{ij}}|_{C=D_{0}}=f(D_{0},D_{0})\frac{\partial f(C,C)}{\partial x_{ij}}|_{C=D_{0}} (58)
2f(C,D0)xij|C=D0f(D0,D0)=0.\displaystyle-2\frac{\partial f(C,D_{0})}{\partial x_{ij}}|_{C=D_{0}}f(D_{0},D_{0})=0.

It is then established that the gradients at the C=D0C=D_{0} points are zero, and the points are indeed critical points.

VI.2 Hessian matrix

Hessian matrices at the critical points are presented. Define:

h3,ijkl(x)=2δikδjl(pqxpq2)\displaystyle h_{3,ijkl}(x)=2\delta_{ik}\delta_{jl}\left(\sum_{pq}x^{2}_{pq}\right) (59)
+2β[δikpxpjxpl+δljqxiqxkq]\displaystyle+2\beta\left[\delta_{ik}\sum_{p}x_{pj}x_{pl}+\delta_{lj}\sum_{q}x_{iq}x_{kq}\right]
+2β2xijxkl\displaystyle+2\beta^{2}x_{ij}x_{kl}
h4,ijkl(w,x)=4wijxkl\displaystyle h_{4,ijkl}(w,x)=4w_{ij}x_{kl} (60)
+β[2δjl(qwiqxkq)+xkjwil+2δik(pwpjxpl)+xilwkj]\displaystyle+\beta\left[2\delta_{jl}(\sum_{q}w_{iq}x_{kq})+x_{kj}w_{il}+2\delta_{ik}(\sum_{p}w_{pj}x_{pl})+x_{il}w_{kj}\right]
+2β2[δikδjl(pqwpqxpq)+xijwkl]\displaystyle+2\beta^{2}\left[\delta_{ik}\delta_{jl}\left(\sum_{pq}w_{pq}x_{pq}\right)+x_{ij}w_{kl}\right]
h5,ijkl(y,z)=yijzkl\displaystyle h_{5,ijkl}(y,z)=y_{ij}z_{kl} (61)
+β[δjl(qyiqzkq)+δik(pypjzpl)]\displaystyle+\beta\left[\delta_{jl}(\sum_{q}y_{iq}z_{kq})+\delta_{ik}(\sum_{p}y_{pj}z_{pl})\right]
+β2δikδjl(pqypqzpq)\displaystyle+\beta^{2}\delta_{ik}\delta_{jl}\left(\sum_{pq}y_{pq}z_{pq}\right)

The Hessian matrices at C=D0C=D_{0} can be explicitly written as:

((2g(C)wijwkl)|C=D0(2g(C)wijxkl)|C=D0(2g(C)xijwkl)|C=D0(2g(C)xijxkl)|C=D0).\begin{pmatrix}(\frac{\partial^{2}g(C)}{\partial w_{ij}\partial w_{kl}})|_{C=D_{0}}&(\frac{\partial^{2}g(C)}{\partial w_{ij}\partial x_{kl}})|_{C=D_{0}}\\ (\frac{\partial^{2}g(C)}{\partial x_{ij}\partial w_{kl}})|_{C=D_{0}}&(\frac{\partial^{2}g(C)}{\partial x_{ij}\partial x_{kl}})|_{C=D_{0}}\\ \end{pmatrix}. (62)

where the three independent parts of Hessian matrix are:

2g(C)wijwkl|C=D0\displaystyle\frac{\partial^{2}g(C)}{\partial w_{ij}\partial w_{kl}}|_{C=D_{0}} (63)
=f(D0,D0)h3,ijkl(x)2h2,ij(w,x,x)h2,kl(w,x,x),\displaystyle=f(D_{0},D_{0})h_{3,ijkl}(x)-2h_{2,ij}(w,x,x)h_{2,kl}(w,x,x),
2g(C)xijxkl|C=D0\displaystyle\frac{\partial^{2}g(C)}{\partial x_{ij}\partial x_{kl}}|_{C=D_{0}} (64)
=f(D0,D0)h3,ijkl(w)2h2,ij(x,w,w)h2,kl(x,w,w),\displaystyle=f(D_{0},D_{0})h_{3,ijkl}(w)-2h_{2,ij}(x,w,w)h_{2,kl}(x,w,w),
2g(C)wijxkl|C=D0=f(D0,D0)h4,ijkl(w,x)\displaystyle\frac{\partial^{2}g(C)}{\partial w_{ij}\partial x_{kl}}|_{C=D_{0}}=f(D_{0},D_{0})h_{4,ijkl}(w,x) (65)
2h5,ijkl(w,x)f(D0,D0)2h2,ij(w,x,w)h2,kl(x,w,w).\displaystyle-2h_{5,ijkl}(w,x)f(D_{0},D_{0})-2h_{2,ij}(w,x,w)h_{2,kl}(x,w,w).

We conjecture that this Hessian matrix is positive semidefinite, thus making the critical points local minimums. In Appendix F we prove that the function is non-convex, which means that further scrutinization is needed for characterization of this function.

Conclusion and Discussion

We’ve broken down the process of verifying bound entanglement into iterative steps of 1-undistillability verifications, by noticing that N-undistillability for arbitrary N is equivalent to 2N2^{N}-undistillability for arbitrary N, and then utilizing specific symmetric properties. In the Werner state case, new bounds for N-undistillability of any finite N are presented, a result similar to that of [18], [19] and [20], but different in the sense that our bounds are unaffected by the dimensionality of Werner states. Alternative expressions for inequalities applicable to both rank two and rank one matrices are given. Subsequently, the problem of two-undistillability is converted into a matrix analysis problem. The multi-variable function treatment is also attempted, as well as proving critical points, non-convexity and conjecturing about Hessian positivity.

Recently, the problem of N-copy Werner state distillability has been reformulated in [29] into a set of partial trace inequalities, which coincided with our Theorem V.1. In the regime of 2-copy Werner state distillability, A special case of the matrix being the sum of a rank-one matrix and a normal matrix is proved.

We believe the new perspectives presented here will assist further attempts at this famous open problem.

Acknowledgements.
We would like to thank Prof. Fedor Sukochev, Dr. Dmitriy Zanin and Prof. Zhi Yin for helpful comments and valuable insights about partial trace inequalities.

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Appendix A Proof of Lemma IV.1

Lemma A.1.

Let |ψ|\psi\rangle be an arbitrary pure quantum state and sjs_{j} are the Schmidt coefficients of |ψ|\psi\rangle arranged in descending order, then

j=1ksj2=max|ϕSRk|ψ|ϕSRk|2,\;\sum_{j=1}^{k}s_{j}^{2}=max_{|\phi^{SR\leq k}\rangle}|\langle\psi|\phi^{SR\leq k}\rangle|^{2}, (66)

where |ϕSRk|\phi^{SR\leq k}\rangle is an arbitrary quantum pure state with Schimidt rank being less than k, namely, SR(|ϕSRk)kSR(|\phi^{SR\leq k}\rangle)\leq k.

Proof.

State-operator isomorphism translates the problem to an equivalent form of proving:

|Tr(AB)|2i=1ksi2(A),|Tr(A^{\dagger}B)|^{2}\leq\sum_{i=1}^{k}s^{2}_{i}(A), (67)

where both AA and BB are d×dd\times d matrices, and as they are the result of state-operator isomorphism from |ψ|\psi\rangle and |ϕSR2|\phi^{SR\leq 2}\rangle, are of Frobenius norm 1 due to normalization conditions, with BB having rank k. We use si(A)s_{i}(A) and |λi(A)||\lambda_{i}(A)| to denote the singular values and absolute values of eigenvalues of AA arranged in descending order.

|Tr(AB)|2(i=1d|λi(AB)|)2(i=1dsi(AB))2\displaystyle|Tr(A^{\dagger}B)|^{2}\leq(\sum_{i=1}^{d}|\lambda_{i}(A^{\dagger}B)|)^{2}\leq(\sum_{i=1}^{d}s_{i}(A^{\dagger}B))^{2} (68)
(i=1ksi(A)si(B))2=(i=1ksi(A)si(B))2,\displaystyle\leq(\sum_{i=1}^{k}s_{i}(A^{\dagger})s_{i}(B))^{2}=(\sum_{i=1}^{k}s_{i}(A)s_{i}(B))^{2},

where the second and third inequality are from Theorem 3.3.13(a) and Theorem 3.3.14(a) in [30], and dkd\to k change of index holds because the rest of BB’s singular values are all zeroes after dd. respectively. Then by Cauchy-Schwartz inequality,

|Tr(AB)|2(i=1ksi(A)si(B))2(i=1ksi2(A))(j=1ksj2(B))\displaystyle|Tr(A^{\dagger}B)|^{2}\leq(\sum_{i=1}^{k}s_{i}(A)s_{i}(B))^{2}\leq(\sum_{i=1}^{k}s^{2}_{i}(A))(\sum_{j=1}^{k}s^{2}_{j}(B)) (69)
=i=1ksi2(A),\displaystyle=\sum_{i=1}^{k}s^{2}_{i}(A),

where the last equality follows from the normalization condition of BB. ∎

Appendix B Proof of Theorem IV.2

Theorem B.1.

Let β0\beta_{0} be the zero point of 1+(1+β)N(1β)N1+(1+\beta)^{N}-(1-\beta)^{N} within [1,0][-1,0]. When ββ0\beta\geq\beta_{0}, Werner state ρw\rho_{w} is N-undistillable.

Proof.

We can overlook the 1d2+βd\frac{1}{d^{2}+\beta d} factor since it doesn’t affect positivity.

(ρwTA)N=IN+m=1Nβmseq(m,N)Gi1Gi2GiN,(\rho_{w}^{T_{A}})^{\otimes N}=I^{\otimes N}+\sum_{m=1}^{N}\beta^{m}\sum_{seq(m,N)}G^{i_{1}}\otimes G^{i_{2}}\otimes\cdots\otimes G^{i_{N}}, (70)

where seq(m,N)seq(m,N) denotes all possible binary i1,,iNi_{1},\dots,i_{N} sequences with mm ones and NmN-m zeros. For convenience denote S0={n|in=0},S1={n|in=1}S_{0}=\{n|i_{n}=0\},S_{1}=\{n|i_{n}=1\}.

MNGi1Gi2GiNMN\displaystyle M_{N}G^{i_{1}}\otimes G^{i_{2}}\otimes\cdots\otimes G^{i_{N}}M_{N}^{\dagger} (71)
=MNj1j2N|j2n1j2ninj2n1+inj2n|MN\displaystyle=M_{N}\sum_{j_{1}\dots j_{2N}}|\cdots j_{2n-1}j_{2n-i_{n}}\cdots\rangle\langle\cdots j_{2n-1+i_{n}}j_{2n}\cdots|M_{N}^{\dagger}
=j1j2N|j2n1,j2ninj2n1+in,j2n|\displaystyle=\sum_{j_{1}\dots j_{2N}}|\cdots j_{2n-1}\cdots,\cdots j_{2n-i_{n}}\cdots\rangle\langle\cdots j_{2n-1+i_{n}}\cdots,\cdots j_{2n}\cdots|
=dmj2n1,j2n,nS0|ψj2n1,j2n,nS0ψj2n1,j2n,nS0|,\displaystyle=d^{m}\sum_{j_{2n-1},j_{2n},n\in S_{0}}|\psi_{j_{2n-1},j_{2n},n\in S_{0}}\rangle\langle\psi_{j_{2n-1},j_{2n},n\in S_{0}}|,

where

|ψj2n1,j2n,nS0\displaystyle|\psi_{j_{2n-1},j_{2n},n\in S_{0}}\rangle (72)
=1dmj2n1,nS1|j2n1,j2nin.\displaystyle=\frac{1}{\sqrt{d^{m}}}\sum_{j_{2n-1},n\in S_{1}}|\dots j_{2n-1}\dots,\dots j_{2n-i_{n}}\dots\rangle.

Any pure quantum state |ψSR2|\psi^{SR\leq 2}\rangle of Schmidt rank no larger than 2 can be decomposed into:

|ψSR2=j2n1,j2n,nS0pj2n1,j2n,nS0|ψj2n1,j2n,nS0SR2,|\psi^{SR\leq 2}\rangle=\sum_{j_{2n-1},j_{2n},n\in S_{0}}p_{j_{2n-1},j_{2n},n\in S_{0}}|\psi_{j_{2n-1},j_{2n},n\in S_{0}}^{SR\leq 2}\rangle, (73)

where |ψj2n1,j2n,nS0SR2|\psi_{j_{2n-1},j_{2n},n\in S_{0}}^{SR\leq 2}\rangle is the normalized extraction of all |j2n1,j2n,nS0|\cdots j_{2n-1}\cdots,\cdots j_{2n}\cdots\rangle,n\in S_{0} terms in |ψSR2|\psi^{SR\leq 2}\rangle, namely, if

|ψSR2=k1,,k2Nck1,,k2N|k1,,k2N,|\psi^{SR\leq 2}\rangle=\sum_{k_{1},\cdots,k_{2N}}c_{k_{1},\cdots,k_{2N}}|k_{1},\cdots,k_{2N}\rangle, (74)

then,

|ψj2n1,j2n,nS0SR2\displaystyle|\psi^{SR\leq 2}_{j_{2n-1},j_{2n},n\in S_{0}}\rangle (75)
=1pj2n1,j2n,nS0\displaystyle=\frac{1}{p_{j_{2n-1},j_{2n},n\in S_{0}}}
j2n1,j2n,nS1cj2n1,j2n|j2n1,j2n,\displaystyle\sum_{j_{2n-1},j_{2n},n\in S_{1}}c_{\cdots j_{2n-1}\cdots,\cdots j_{2n}\cdots}|\cdots j_{2n-1}\cdots,\cdots j_{2n}\cdots\rangle,

where

pj2n1,j2n,nS0=j2n1,j2n,nS1|cj2n1,j2n|2p_{j_{2n-1},j_{2n},n\in S_{0}}=\sqrt{\sum_{j_{2n-1},j_{2n},n\in S_{1}}|c_{\cdots j_{2n-1}\cdots,\cdots j_{2n}\cdots}|^{2}} (76)

It can be proved that |ψj2n1,j2n,nS0SR2|\psi_{j_{2n-1},j_{2n},n\in S_{0}}^{SR\leq 2}\rangle also has Schmidt rank less than or equal to 2. According to state-operator isomorphism, Schmidt rank of a state is equal to rank of the corresponding operator. In fact, the operator corresponding to |ψj2n1,j2n,nS0SR2|\psi_{j_{2n-1},j_{2n},n\in S_{0}}^{SR\leq 2}\rangle is the extraction of dmd^{m} rows j2n1,nS0,\cdots j_{2n-1}\cdots,n\in S_{0}, and dmd^{m} columns j2n,nS0\cdots j_{2n}\cdots,n\in S_{0}. The row and column numbers j2n1\cdots j_{2n-1}\cdots and j2n\cdots j_{2n}\cdots are written in base-d numeral systems. Therefore, operator corresponding to |ψj2n1,j2n,nS0SR2|\psi_{j_{2n-1},j_{2n},n\in S_{0}}^{SR\leq 2}\rangle is a submatrix of the operator corresponding to |ψSR2|\psi^{SR\leq 2}\rangle. The rank of a submatrix is no larger than the rank of the entire matrix, therefore |ψj2n1,j2n,nS0SR2|\psi_{j_{2n-1},j_{2n},n\in S_{0}}^{SR\leq 2}\rangle must have Schmidt rank no larger than 2. Using Lem.IV.1, it is then clear that:

|ψj2n1,j2n,nS0SR2|ψj2n1,j2n,nS0|22dm,|\langle\psi_{j_{2n-1},j_{2n},n\in S_{0}}^{SR\leq 2}|\psi_{j_{2n-1},j_{2n},n\in S_{0}}\rangle|^{2}\leq\frac{2}{d^{m}}, (77)

and so

ψSR2|MNGi1Gi2GiNMN|ψSR2\displaystyle\langle\psi^{SR\leq 2}|M_{N}G^{i_{1}}\otimes G^{i_{2}}\otimes\cdots\otimes G^{i_{N}}M_{N}^{\dagger}|\psi^{SR\leq 2}\rangle (78)
dm2dmj2n1,j2n,nS0|pj2n1,j2n,nS0|2=2.\displaystyle\leq d^{m}\frac{2}{d^{m}}\sum_{j_{2n-1},j_{2n},n\in S_{0}}|p_{j_{2n-1},j_{2n},n\in S_{0}}|^{2}=2.

Considering the fact that all even terms in (ρwTA)N(\rho_{w}^{T_{A}})^{\otimes N} are non-negative and using the above inequality on all odd terms, a lower bound is obtained:

ψSR2|MN(ρwTA)NMN|ψSR2\displaystyle\langle\psi^{SR\leq 2}|M_{N}(\rho_{w}^{T_{A}})^{\otimes N}M_{N}^{\dagger}|\psi^{SR\leq 2}\rangle (79)
1+k=1N22CN2k1β2k1=1+(1+β)N(1β)N\displaystyle\geq 1+\sum_{k=1}^{\lceil\frac{N}{2}\rceil}2C_{N}^{2k-1}\beta^{2k-1}=1+(1+\beta)^{N}-(1-\beta)^{N}

For β(1,0)\beta\in(-1,0), any β\beta greater than the zero point β0\beta_{0} would make 1+(1+β)N(1β)N1+(1+\beta)^{N}-(1-\beta)^{N} greater than zero, thus ensuring the positivity of ψSR2|MN(ρwTA)NMN|ψSR2\langle\psi^{SR\leq 2}|M_{N}(\rho_{w}^{T_{A}})^{\otimes N}M_{N}^{\dagger}|\psi^{SR\leq 2}\rangle.

Appendix C Proof of Theorem V.1

Theorem C.1.

Werner state ρw\rho_{w} is N-undistillable iff the following holds for all dN×dNd^{N}\times d^{N} X2X_{2}:

S{1,,N}β|S|TrS(X2)F20,\displaystyle\sum_{S\subset\{1,\cdots,N\}}\beta^{|S|}||Tr_{S}(X_{2})||_{F}^{2}\geq 0, (80)

where TrSTr_{S} takes partial traces of the subsystems in set SS.

Proof.

We’ve already established that N-undistillability is equivalent to:

ψSR2|MN(ρTA)NMN|ψSR20.\langle\psi^{SR\leq 2}|M_{N}(\rho^{T_{A}})^{\otimes N}M_{N}^{\dagger}|\psi^{SR\leq 2}\rangle\geq 0. (81)

In the previous section it has been established that:

(ρwTA)N=IN+m=1Nβmseq(m,N)Gi1Gi2GiN,(\rho_{w}^{T_{A}})^{\otimes N}=I^{\otimes N}+\sum_{m=1}^{N}\beta^{m}\sum_{seq(m,N)}G^{i_{1}}\otimes G^{i_{2}}\otimes\cdots\otimes G^{i_{N}}, (82)
MNGi1Gi2GiNMN\displaystyle M_{N}G^{i_{1}}\otimes G^{i_{2}}\otimes\cdots\otimes G^{i_{N}}M_{N}^{\dagger} (83)
=dmj2n1,j2n,nS0|ψj2n1,j2n,nS0ψj2n1,j2n,nS0|,\displaystyle=d^{m}\sum_{j_{2n-1},j_{2n},n\in S_{0}}|\psi_{j_{2n-1},j_{2n},n\in S_{0}}\rangle\langle\psi_{j_{2n-1},j_{2n},n\in S_{0}}|,

where

|ψj2n1,j2n,nS0\displaystyle|\psi_{j_{2n-1},j_{2n},n\in S_{0}}\rangle (84)
=1dmj2n1,nS1|j2n1,j2nin.\displaystyle=\frac{1}{\sqrt{d^{m}}}\sum_{j_{2n-1},n\in S_{1}}|\dots j_{2n-1}\dots,\dots j_{2n-i_{n}}\dots\rangle.

For a pure quantum state of the form:

|ψSR2=j1,,jNcj2n1,j2n|j2n1,j2n,|\psi^{SR\leq 2}\rangle=\sum_{j_{1},\cdots,j_{N}}c_{\cdots j_{2n-1}\cdots,\cdots j_{2n}\cdots}|\cdots j_{2n-1}\cdots,\cdots j_{2n}\cdots\rangle, (85)
ψSR2|MNGi1Gi2GiNMN|ψSR2\displaystyle\langle\psi^{SR\leq 2}|M_{N}G^{i_{1}}\otimes G^{i_{2}}\otimes\cdots\otimes G^{i_{N}}M_{N}^{\dagger}|\psi^{SR\leq 2}\rangle (86)
=dmj2n1,j2n,nS0|ψj2n1,j2n,nS0|ψSR2|2\displaystyle=d^{m}\sum_{j_{2n-1},j_{2n},n\in S_{0}}|\langle\psi_{j_{2n-1},j_{2n},n\in S_{0}}|\psi^{SR\leq 2}\rangle|^{2}
=j2n1,j2n,nS0|j2n1,nS1cj2n1,j2nin|2\displaystyle=\sum_{j_{2n-1},j_{2n},n\in S_{0}}|\sum_{j_{2n-1},n\in S_{1}}c_{\cdots j_{2n-1}\cdots,\cdots j_{2n-i_{n}}\cdots}|^{2}
=Tr{in|nS1}(X2)F2.\displaystyle=||Tr_{\{i_{n}|n\in S_{1}\}}(X_{2})||_{F}^{2}.

In the last equality, X2X_{2} is the result of state-operator isomorphism from |ψSR2|\psi^{SR\leq 2}\rangle. Noticing that

ψSR2|MNINMN|ψSR2=1=β0X2F2,\langle\psi^{SR\leq 2}|M_{N}I^{\otimes N}M_{N}^{\dagger}|\psi^{SR\leq 2}\rangle=1=\beta^{0}||X_{2}||_{F}^{2}, (87)

it then follows that

ψSR2|MN(ρTA)NMN|ψSR20,\langle\psi^{SR\leq 2}|M_{N}(\rho^{T_{A}})^{\otimes N}M_{N}^{\dagger}|\psi^{SR\leq 2}\rangle\geq 0, (88)

is equivalent to

S{1,,N}β|S|TrS(X2)F20,\displaystyle\sum_{S\subset\{1,\cdots,N\}}\beta^{|S|}||Tr_{S}(X_{2})||_{F}^{2}\geq 0, (89)

Appendix D Proof of Theorem V.3

Theorem D.1.

Werner state ρw\rho_{w} is N-undistillable iff

Re[fN(X1,X1)]2fN(X1,X1)fN(X1,X1),Re[f_{N}(X_{1},X^{\prime}_{1})]^{2}\leq f_{N}(X^{\prime}_{1},X^{\prime}_{1})f_{N}(X_{1},X_{1}), (90)

where

fN(X1,X1)=S{1,,N}β|S|Tr[TrS(X1)TrS(X1)]0,\displaystyle f_{N}(X_{1},X^{\prime}_{1})=\sum_{S\subset\{1,\cdots,N\}}\beta^{|S|}Tr[Tr^{\dagger}_{S}(X_{1})Tr_{S}(X^{\prime}_{1})]\geq 0, (91)

where X1=𝐰𝐱,X1=𝐲𝐳X_{1}=\mathbf{w}^{\dagger}\mathbf{x},X^{\prime}_{1}=\mathbf{y}^{\dagger}\mathbf{z} are dN×dNd^{N}\times d^{N} rank one matrices, and their component vectors 𝐰,𝐱,𝐲,𝐳\mathbf{w},\mathbf{x},\mathbf{y},\mathbf{z} satisfy 𝐰𝐲,𝐱𝐳\mathbf{w}\perp\mathbf{y},\mathbf{x}\perp\mathbf{z}.

Proof.

It has been proven that N-undistillability is equivalent to:

S{1,,N}β|S|TrS(X2)F20,\displaystyle\sum_{S\subset\{1,\cdots,N\}}\beta^{|S|}||Tr_{S}(X_{2})||_{F}^{2}\geq 0, (92)

Since any rank two matrix can be decomposed via singular value decomposition:

X2=σ1X1+σ2X1,X_{2}=\sigma_{1}X_{1}+\sigma_{2}X^{\prime}_{1}, (93)

Eq.92 can be written as:

S{1,,N}β|S|TrS(X2)F2\displaystyle\sum_{S\subset\{1,\cdots,N\}}\beta^{|S|}||Tr_{S}(X_{2})||_{F}^{2} (94)
=S{1,,N}β|S|[σ12||TrS(X1)||F2+σ22||TrS(X1)||F2\displaystyle=\sum_{S\subset\{1,\cdots,N\}}\beta^{|S|}[\sigma^{2}_{1}||Tr_{S}(X_{1})||_{F}^{2}+\sigma_{2}^{2}||Tr_{S}(X^{\prime}_{1})||_{F}^{2}
+2σ1σ2Re(Tr(TrS(X1)TrS(X1)))]\displaystyle+2\sigma_{1}\sigma_{2}Re(Tr(Tr_{S}(X_{1})^{\dagger}Tr_{S}(X^{\prime}_{1})))]
=σ12fN(X1,X1)+σ22fN(X1,X1)\displaystyle=\sigma_{1}^{2}f_{N}(X_{1},X_{1})+\sigma_{2}^{2}f_{N}(X^{\prime}_{1},X^{\prime}_{1})
+2σ1σ2Re[fN(X1,X1)]\displaystyle+2\sigma_{1}\sigma_{2}Re[f_{N}(X_{1},X^{\prime}_{1})]
0.\displaystyle\geq 0.

The above should hold for all singular values σ1,σ2\sigma_{1},\sigma_{2}, which is then equivalent to:

Re[fN(X1,X1)]2fN(X1,X1)fN(X1,X1),Re[f_{N}(X_{1},X^{\prime}_{1})]^{2}\leq f_{N}(X_{1},X_{1})f_{N}(X^{\prime}_{1},X^{\prime}_{1}), (95)

always holding when X1=𝐰𝐱,X1=𝐲𝐳X_{1}=\mathbf{w}^{\dagger}\mathbf{x},X^{\prime}_{1}=\mathbf{y}^{\dagger}\mathbf{z} are dN×dNd^{N}\times d^{N} rank one matrices, and their component vectors 𝐰,𝐱,𝐲,𝐳\mathbf{w},\mathbf{x},\mathbf{y},\mathbf{z} satisfy 𝐰𝐲,𝐱𝐳\mathbf{w}\perp\mathbf{y},\mathbf{x}\perp\mathbf{z}. ∎

Appendix E Proof of Lem. V.2

Lemma E.1.

The inequalities:

Tr1(X1)F2X1F2,Tr2(X1)F2X1F2,||Tr_{1}(X_{1})||_{F}^{2}\leq||X_{1}||_{F}^{2},||Tr_{2}(X_{1})||_{F}^{2}\leq||X_{1}||_{F}^{2}, (96)

hold for any d2×d2d^{2}\times d^{2} square matrix X1X_{1} of rank one.

Proof.

A rank one matrix X1X_{1} can always be written as the outer product of two vectors: (in this case, bipartite)

(X1)ij,kl=wijxkl.(X_{1})_{ij,kl}=w_{ij}x_{kl}. (97)

Its partial traces can be computed accordingly:

(Tr2(X1))i,k=jwijxkj,(Tr1(X1))j,l=iwijxil.(Tr_{2}(X_{1}))_{i,k}=\sum_{j}w_{ij}x_{kj},(Tr_{1}(X_{1}))_{j,l}=\sum_{i}w_{ij}x_{il}. (98)

A direct calculation and application of Cauchy-Schwartz inequality yields the desired result:

Tr2(X1)F2=ik|jwijxkj|2ikj|wij|2l|xkl|2\displaystyle||Tr_{2}(X_{1})||_{F}^{2}=\sum_{ik}|\sum_{j}w_{ij}x_{kj}|^{2}\leq\sum_{ik}\sum_{j}|w_{ij}|^{2}\sum_{l}|x_{kl}|^{2} (99)
=ijkl|wij|2|xkl|2=X1F2,\displaystyle=\sum_{ijkl}|w_{ij}|^{2}|x_{kl}|^{2}=||X_{1}||_{F}^{2},
Tr1(X1)F2=jl|iwijxil|2jli|wij|2k|xkl|2\displaystyle||Tr_{1}(X_{1})||_{F}^{2}=\sum_{jl}|\sum_{i}w_{ij}x_{il}|^{2}\leq\sum_{jl}\sum_{i}|w_{ij}|^{2}\sum_{k}|x_{kl}|^{2} (100)
=ijkl|wij|2|xkl|2=X1F2.\displaystyle=\sum_{ijkl}|w_{ij}|^{2}|x_{kl}|^{2}=||X_{1}||_{F}^{2}.

Appendix F Proving non-convexity

We now prove that the function of g(C)D0g(C)_{D_{0}} is non-convex, by showing that its local minimum set is not a convex one. For

C=𝐰𝐱T,D0=𝐲𝐳T,C=\mathbf{w}\mathbf{x}^{T},D_{0}=\mathbf{y}\mathbf{z}^{T}, (101)

we set vectors 𝐲\mathbf{y} and 𝐳\mathbf{z} to identical forms of:

yij=zij=δi0δj1y_{ij}=z_{ij}=\delta_{i0}\delta_{j1} (102)

For simplicity we first write the variables 𝐰,𝐱\mathbf{w},\mathbf{x} in a matrix form of:

(w00w01wd1,d1x00x01xd1,d1),\begin{pmatrix}w_{00}&w_{01}&\cdots&w_{d-1,d-1}\\ x_{00}&x_{01}&\cdots&x_{d-1,d-1}\\ \end{pmatrix},

where the two rows correspond to two vectors 𝐰\mathbf{w}, 𝐱\mathbf{x}, respectively. We take the middle point combination of the following two points:

(010010),(100100),\begin{pmatrix}0&1&\cdots 0\\ 0&1&\cdots 0\\ \end{pmatrix},\begin{pmatrix}1&0&\cdots 0\\ 1&0&\cdots 0\\ \end{pmatrix},

both of these points can be proven to have zero Jacobian matrix and positive definite Hessian, effectively making them local minimums.

For a convex function, its local minimum set must be a convex set, so that middle point combination of any two points should stay in the set. Their middle point combination is:

(11001100).\begin{pmatrix}1&1&0&\cdots 0\\ 1&1&0&\cdots 0\\ \end{pmatrix}.

The normalization factor doesn’t change whether the Jacobian matrix is nonzero or not, and therefore is interchangeable and omitted here. At this particular point, the Jacobian matrix is nonzero and proportional to:

[1,1,0,0,0,0,0,0,0,1,1,0,0,0,0,0,0,0],[1,1,0,0,0,0,0,0,0,1,1,0,0,0,0,0,0,0], (103)

which suggests that the middle point is not a local minimum, thus proving the non-convexity of the set of local minimums. It then follows that the function of g(C,D)g(C,D) is non-convex.