Magic angle (in)stability and mobility edges in disordered Chern insulators
Abstract.
Why do experiments only exhibit one magic angle if the chiral limit of the Bistritzer-MacDonald Hamiltonian suggest a plethora of them? - In this article, we investigate the remarkable stability of the first magic angle in contrast to higher (smaller) magic angles. More precisely, we examine the influence of disorder on magic angles and the Bistritzer-MacDonald Hamiltonian. We establish the existence of a mobility edge near the energy of the flat band for small disorder. We also show that the mobility edges persist even when all global Chern numbers become zero, leveraging the symmetry of the system to demonstrate non-trivial sublattice transport. This effect is robust even beyond the chiral limit and in the vicinity of perfect magic angles, as is expected from experiments.
1. Introduction
Twisted bilayer graphene is a highly tunable material that exhibits approximately flat bands at special twisting angles, the so-called magic angles [TKV19, BiMa11].
In this article, we study the question of why the largest magic angle, as predicted by the chiral model, is more robust than smaller magic angles within the chiral limit. We analyze why the chiral model’s largest magic angle exhibits greater resilience compared to smaller magic angles within the chiral limit. This finding potentially elucidates why, up until now, only the first magic angle has been experimentally observed. We also study the impact of disorder in the chiral limit and its interplay with the flat bands at magic angles. In quantum systems, disorder-induced dynamical localization is a well-known phenomenon, wherein spatially localized wavepackets do not significantly diffuse under time evolution. While the underlying mechanisms behind this phenomenon are relatively well understood, the opposite behavior—diffusive behavior in disordered systems—is only understood in specific cases [AS19, AW13, BH22, GKS07, JSS03].
It is widely believed that large classes of two-dimensional quantum systems, even under minor disorder, exclusively exhibit localization, as conjectured by Problem 2 on Simon’s list of open problems for Schrödinger operators [Si00]. As we will show below, the Hamiltonian describing twisted bilayer graphene at a magic angle or other related materials is an exception. These new classes of materials, so-called Chern insulators, exhibit non-zero Chern numbers in the absence of external magnetic fields [Li21]. In particular, in twisted bilayer graphene, for wavepackets localized sufficiently close to the perturbed flat band at zero energy, the time-evolution is, in a suitable sense, ballistic. Our argument here is an adaptation of an argument by Germinet, Klein, and Schenker showing a form of delocalization for the Landau Hamiltonian [GKS07]. The physical intuition behind this delocalization argument is straightforward: the Landau Hamiltonian exhibits non-zero Hall conductivity at each Landau level. Moreover, as the Hall conductivity, a topological quantity, remains invariant under minor disorder, the existence of substantial spectral gaps between the Landau levels prevents strong localization across the spectrum.
The properties of the flat bands for twisted bilayer graphene are analogous to Landau levels with the crucial difference that no magnetic field is required. At the first magic angle, the two flat bands exhibit only a Chern number zero. However, the two flat bands individually carry non-zero Chern numbers , allowing for an anomalous quantum Hall effect when the TBG substrate is e.g. aligned with hexagonal boron nitride [Li21]. Mathematically, the effect of aligning the substrate with hBN is modeled by adding an effective mass term to the Hamiltonian thereby splitting the two flat bands each carrying a non-zero Chern number. In addition, the flat bands are gapped from the rest of the spectrum.
We also establish a localized regime that rests on the multi-scale analysis framework of Germinet-Klein [GK01, GK03]. Here, the only difficulty is to allow for a sufficiently large class of random perturbations which requires us to extend the estimate on the number of eigenvalues (NE) and thus the Wegner estimate (W).
The chiral limit of the massive continuum model for twisted bilayer graphene, which can also be thought of as a model Hamiltonian for twisted transition metal dichalcogenides (TMDs) [CRQ23], is the Hamiltonian acting on with domain given by the Sobolev space
(1.1) |
where , is an effective parameter that is inversely proportional to the twisting angle and a mass parameter. Let be a triangular lattice with . The tunnelling potentials are -periodic functions satisfying for with , i.e.
(1.2) |
The central object in the one-particle picture of twisted bilayer graphene are the so-called magic angles. We say that is magic if and only if the Bloch-Floquet transformed Hamiltonian, see [Be*22, (2.11)], with mass parameter exhibits a flat band at energy , i.e.
(1.3) |
with denoting the spectrum of the linear operator on the Hilbert space on a suitable dense domain, where The set of under which there exists a flat band at energy is independent of 111Observe that [T92, (5.66)].. In the sequel, we shall suppress the mass parameter in the notation.
For the study of magic angles we also introduce a translation operator
(1.4) |
and a rotation operator We can then define subspaces
(1.5) |
and similarly .
The set of such magic parameters , that we shall denote by is characterized by [Be*22, Theo.]
(1.6) |
with the dual lattice.
We then define the set of generic magic angles. The terminology generic is motivated by [BHZ23, Theo.] which shows that for a generic choice of tunnelling potentials all magic angles are of the following form.
Definition 1.1 (Generic magic angles).
We say that is a simple or two-fold degenerate magic angle if and with , respectively. In the following sections, we will denote the combination of these magic angles as the collection of generic magic angles.
1.1. Magic angle (in)stability
The first aim of this article is to study perturbations of the operator , i.e. for
with bounded linear perturbations . We then obtain in Theorem 6 a bound on the spread of the magic angles under such perturbations. This is a non-trivial result as the operator , whose eigenvalues are the magic angles, is a non-normal operator. In particular, small perturbations in norm can lead to substantial perturbations of the spectrum, see [TE05]. On the other hand, we show that even simple rank -perturbations of exponentially small size in suffice to generate eigenvalues in the spectrum of .
Theorem 1 (Instability).
Let and , then there exists a rank- operator with and independent of such that . Here, characterizes the set of magic parameters as explained in (1.6).
1.2. Anderson model and IDS
One consequence of having a flat band is the occurrence of jump discontinuities in the integrated density of states (IDS). The integrated density of states is defined as follows, see [Sj89] and others:
Definition 1.2.
The integrated density of states (IDS) for energies and is defined by
with and has periodic boundary conditions, i.e.
For ergodic random operators, the almost sure existence of this limit is shown using the subadditive ergodic theorem, see for instance [K89, Sec. 7.3]. Alternatively, one may define for the regularized trace
(1.7) |
By Riesz’s theorem on the representation of positive functionals, one has that
where is the density of states (DOS) measure of This way,
Remark 1.
For Schrödinger operators it is common to consider Dirichlet approximations of the finite-size truncation. It is known that Dirac operators do in general not have any self-adjoint Dirichlet realizations. However, self-adjoint Neumann-type boundary conditions are possible, see [BM87] and for instance the introduction of [SV19] for a mathematical discussion. The independence of the definition of the IDS of the boundary conditions can then be shown using spectral shift function techniques if the operator contains a gap in the spectrum, see for instance the work by Nakamura [N01] on Schrödinger operators.
A periodic Hamiltonian that exhibits a flat band at energy possesses a jump discontinuity in the IDS at . In particular, the Lebesgue decomposition of has a pure point contribution at As a consequence, if we define the associated cumulative distribution function by , then this function is monotonically increasing and right-continuous (càdlàg). At a magic angle, the function for exhibits a jump discontinuity at Indeed, this can easily be seen from the following formula which shows that for a periodic Hamiltonian one just has [Sj89, (1.29)]
Let be a generic magic angle, as in Def. 1.1, then we define the energy gap between the flat bands and the rest of the spectrum
(1.8) |
That this quantity is non-zero by [BHZ22, Theo.] for simple and by [BHZ23, Theo.] for two-fold degenerate magic angles and is illustrated in Figure 1. In particular, the following union of intervals is in the resolvent set of the Hamiltonians
(1.9) |
Let be the orthogonal projection onto a closed subspace . For generic it has been shown in [BHZ22b, Theo. ] and [BHZ23, Theo. ] that the Chern number of the flat band at energy is or more generally (including ) for the Hamiltonian in (1.1)
(1.10) |
The Chern number can be computed from the Hall conductivity , see (4.4), by using that
In particular, the net Chern number of the flat bands for is zero
Assumption 1 (Anderson model).
We introduce the Anderson-type Hamiltonian with alloy-type potentials and (possible) lattice relaxation effects for and
(1.11) |
where and are families of i.i.d. random variables with absolutely continuous bounded densities. For the density is a function with and in case of a density supported within a compact domain where we allow . Random variables model small inhomogeneities of the moiré lattice due to relaxation effects. We assume that either
- (1)
-
(2)
Case : The disorder with and for some .
For normalization purposes, we assume that and for some fixed where and
We emphasize that under assumption (1), the matrix is neither positive nor negative definite. This usually poses an obstruction to proving Wegner estimates as the eigenvalues are not monotone in the noise parameter. We can overcome this obstacle here by using the off-diagonal structure of the Hamiltonian. The probability space is the Polish space with the product measure. Then is an ergodic (with respect to lattice translations) family of self-adjoint operators with continuous dependence Thus, there is closed such that
(1.13) |
see [CFKS87, Pa80]. In addition, using ergodicity arguments, see e.g. [W95], the density of states measure for the random operator, exists almost surely and is almost surely non-random, i.e. is almost surely equal to a non-random measure a.s. with non-random. An extension of our work to unbounded disorder is possible. In the context of Schrödinger operators this extension has been shown for magnetic Landau Hamiltonians [GKS09, GKM09]. Related proofs of localization for Dirac operators under a spectral gap assumption have also been obtained in [BCZ19].
For , the infinitely-degenerate point spectrum of at energy zero, i.e. the flat band, gets non-trivially perturbed and expands in energy. To capture this, we then introduce constants and One thus finds analogously to (1.9) for the disordered Hamiltonian
(1.14) |
where all three intervals are non-trivial for sufficiently small and . We then also define
(1.15) |
When perturbing away from perfect magic angles, we may do so by either using a random potential or perturbing slightly. In both cases, for sufficiently small perturbations, this leaves the spectral gap to the remaining bands open.
Given a finite domain , we introduce the Hamiltonian
with periodic boundary conditions where . In general we shall denote by the restriction of an operator to the domain with periodic boundary conditions in case that is a differential operator.
While the occurrence of a flat band for the unperturbed Hamiltonian (1.1) leads to a jump discontinuity in the IDS, one has that the random Hamiltonian (1.11) has a Lipschitz continuous IDS for all . Since the randomly perturbed Hamiltonian is no longer periodic, it is customary to measure the destruction of the flat band by studying the regularity of the IDS.
Theorem 2 (Continuous IDS).
Consider the Anderson Hamiltonian as in Assumption (1) with and coupling constant with sufficiently small, then the integrated density of states (IDS) is a.s. Hölder continuous in Hausdorff distance for all , i.e.
-
•
Case 1 disorder: for intervals with and
-
•
Case 2 disorder: arbitrary bounded intervals , and If we assume in addition that is globally positive, i.e.
(1.16) then the IDS is a.s. Lipschitz continuous
In particular, the IDS is a.s. differentiable and its Radon-Nikodym derivative, the density of states (DOS), exists a.s. and is a.s. bounded.
The above results follow directly from the following estimate on the number of eigenvalues (NE) that directly lead to Wegner estimates (4.2).
1.3. Mobility edges
In the works of Germinet–Klein [GK01, GK03, GK04] dynamical measures of transport have been introduced. The dynamical localization implies a strong form of decaying eigenfunctions, see Def. 4.1. To measure dynamical localization/delocalization one introduces the following Hilbert-Schmidt norm
(1.17) |
where , for some non-negative with time average
Recall that to see that indicates a time-averaged power scaling of Here, measures the spread of mass in a spectral energy window of the Hamiltonian from the origin under the free Schrödinger evolution.
We shall then show that the random Hamiltonian (1.11) exhibits diffusive behavior in the vicinity of magic angles.
Theorem 3 (Dynamical delocalization).
Let be a generic magic angles as in Definition 1.1. We consider a coupling constant , , mass and sufficiently small . The random Hamiltonian exhibits diffusive behavior for at at least two energies located close to energies , respectively, and at at least one energy for . In particular, for every that equals to one on an open interval containing at least one of and we have for all
We do not have a very precise understanding how close are to . By choosing suitable disorder (of fixed support but rescaled probability), one can show that and can get arbitrarily close, see Theorem 7, at least when is a magic angle, as the bands of the unperturbed Hamiltonian are perfectly flat.
Remark 2.
Transport behavior can also be characterized by the -dependence of the estimate in the previous theorem and using a local transport exponent
The region of dynamical localization is then defined as the open set
(1.18) |
whereas the region of dynamical delocalization is defined as its complement. A mobility edge is an energy It follows from [GK04, Theo. , ] that Theorem 3 implies Theorem 7 then proves the existence of mobility edges for the disordered Hamiltonian.
While Theorem 3 describes the dynamical features of the Hamiltonian, it is equally valid to ask for a spectral theoretic interpretation of transport and localization. The interpretation of the nature of the spectrum in the dynamically localized phase is captured by the concept of SUDEC, see Def. 4.1.
The existence of a dynamical delocalization, in the above sense, does not imply the existence of a.c. or s.c. spectrum. Given that at magic angles the Hamiltonian only exhibits (infinitely degenerate) point spectrum at energies , it is unknown if such phases can occur for our disordered Hamiltonian in a neighborhood of the flat bands. We conjecture that this is not the case.
As we will explain below, see Remark 3, the point spectrum of the Hamiltonian within an energy window, cannot be too localized.
Definition 1.4 (Wannier basis).
Let be an orthogonal projection onto . We say an orthonormal basis for an index set is an -localized generalized Wannier basis for for some if:
-
•
-
•
There exists and a collection of localization centers such that for all
One then has for the random Hamiltonian
Theorem 4 (Slow decay; ).
Under the assumptions of Theorem 3, we define the orthogonal projection on with as in (1.15) for For any and for any with sufficiently small and independent of , does not admit a -localized generalized Wannier basis.
However, the projection admits a -localized generalized Wannier basis for small disorder.
In this article, we have not considered disorder that only perturbs the off-diagonal entries of the Hamiltonian (1.1), since no techniques to show Wegner estimates for such disorder are known on which the multi-scale analysis rests.
Wegner estimates are however not needed to study the decay of Wannier functions and thus we shall consider such perturbations now, by looking at the Hamiltonian
(1.19) |
where is a (possibly random) potential which we assume without loss of generality to satisfy The result of Theorem 4 cannot be directly extended to , since the net Chern number of the Hamiltonian is zero. However, the square of the Hamiltonian (1.19) exhibits a diagonal form
(1.20) |
Thus, to capture the low-lying spectrum, we may study the projections
(1.21) |
separately, where we dropped the , dependence as it does not affect the spectrum apart from a constant shift. We then have
Theorem 5 (Slow decay; ).
We make a few observations related to Theorem 4 and the notion of Wannier bases. First, these theorems imply a lower bound on the uniform decay of eigenfunctions for the random Hamiltonian. In particular, it implies that if the random Hamiltonian exhibits pure point spectrum, then the decay is not too fast in a uniform sense which should be compared with the notion of SUDEC, see Def. 4.1 which one obtains by applying the multiscale analysis. In particular, one has
Remark 3 (Lower bound on uniform eigenfunction decay).
If the Hamiltonian only exhibits point spectrum in the interval , for which the associated spectral projections does not admit a generalized Wannier basis, then we can choose an orthonormal basis of eigenfunctions such that and any sequence of localization centers
In this sense, Theorem 4 gives a lower-bound on the decay of eigenfunctions in case that the random Hamiltonian exhibits only pure point spectrum.
Outline of article.
2. (In)stability of magic angles
In this section, we obtain stability bounds on magic angles with respect to perturbations.
We recall the definition of the compact Birman-Schwinger operator , with , where . This operator is defined by
where
for For scalar functions, we also define spaces where we replace the translation operator by its first component (1.4). As described in (1.6), is magic if and only if One can then show that if and only if see [BHZ22b]. By squaring the operator, we define new compact operators
(2.1) |
Since the operator is compact, it follows that
This implies that for which is well-defined as is a Hilbert-Schmidt operator. In particular, the spectrum of is independent of , see [Be*22, Prop.3.1.] and we have for any The traces of powers of are illustrated in Table 1. We thus have that
where the right-hand side depends only on and the unperturbed operator
1 | |
2 | |
3 | |
4 |
5 | |
6 | |
7 | |
8 |
We then consider a perturbation of the potentials which gives us a new operator
with bounded potentials and where satisfies the same symmetries as , respectively, cf. (1.2). By squaring the operator, similar to (LABEL:eq:Tk), we define
(2.2) |
such that
To describe the spectral (in)-stability of non-normal operators one resorts to the pseudospectrum, see also the book [ET05].
Definition 2.1.
Let be a bounded linear operator. We denote the -pseudospectrum of , for every , by
(2.3) |
with the space of bounded linear operators. It is equivalently characterized by
2.1. Stability of magic angles
In order to study the stability of small magic angles, characterized by the eigenvalues of ( is magic if and only if ), we start with a resolvent bound and recall the definition of the regularized determinant for a Hilbert-Schmidt operator [Si77]
The following estimate is non-trivial, as the operator is non-normal:
Lemma 2.2.
Let be as above, then for such that
Before stating the proof of this lemma we state a perturbation estimate that limits by how much the eigenvalues of can spread. This bound is illustrated in Fig. 2.
Theorem 6.
Let , as in (LABEL:eq:Tk), with the magic angles, and define as in (2.2). The perturbed operator does not have any eigenvalues with as long as the size of the perturbation satisfies
(2.4) |
Before stating the proof of this result, we shall briefly discuss the interpretation of (2.4). The right hand side of (2.4) is small for large , i.e. small twisting angles as well as for close to , i.e. for that are almost magic. This means that for such even small perturbations of the potential may generate eigenvalues of the form of the perturbed operator . This shows that such are inherently unstable, as small perturbations can generate and destroy them. Conversely, for large twisting angles, i.e. small it is in general impossible to generate spectrum of the perturbed operator. In particular, this bound implies a spectral stability for small , i.e. large magic angles, since they cannot move by much. The regularized determinant in (2.4) can be controlled (from above and below) by Lemma 2.3.
Proof of Theo. 6.
We now give the proof of the auxiliary Lemma 2.2.
Proof of Lemma 2.2.
We recall from [Si77, Theo.] that together with for a Hilbert-Schmidt operator and a trace-class operator with
(2.5) |
Assuming is invertible and a finite rank operator, we have for the usual determinant
This shows that
which shows
Using that
(2.6) |
we find the log-derivative of the regularized 2-determinant
By using a density argument it follows that this formula also holds for Hilbert-Schmidt, i.e. we can drop the assumption that is of finite rank. Thus, one finds from (2.6) by specializing to , with and multiplying by
Consequently, if is a magic angle, we can estimate in (2.4) by using [BHZ22b, Lemma ], which in a reduced version states that
Lemma 2.3.
The entire function satisfies for any
with , where
(2.7) |
The first few traces are summarized in Table 1.
2.2. Instability of magic angles
Lower row: 1000 realizations of random perturbations of tunnelling potential with new magic angles (black dots) superimposed on resolvent norm figure. (left) and (right).
We shall now give the proof of Theorem 1. Arbitrary low-lying eigenvalues of , which correspond to large magic angles in the unperturbed case, can be produced by rank perturbations of that are exponentially small in the spectral parameter. Let be one such low-lying eigenvalue of . On the Hamiltonian side, this indicates that zero modes with quasi-momentum and can be generated by rank one perturbations of the Bloch-Floquet Hamiltonian,
Proof of Theo. 1.
We recall that by [Be*22, Theo ] there exists for each an -normalized such that the operator
satisfies with and This implies that there is a constant , which we allow to change throughout this proof, such that Hence, we define the normalized then We recall that
This implies that, since , where denotes the Hausdorff distance
Hence, for the normalized , we have
Thus, we can define with norm such that
∎
3. Integrated DOS and Wegner estimate
In this section we prove Theorem 2 by stating a proof of Prop. 1.3, i.e. study the regularity of the integrated density of states and prove a corresponding estimate on the number of eigenvalues of the disordered Hamiltonian. This then also implies a Wegner estimate by (4.2). We start by giving the proof of Hölder continuity, which uses the spectral shift function, see [CHK07, CHK03, CHN01], and then subsequently explain the modifications to obtain Lipschitz continuity, which uses spectral averaging. In the following, we will write with , , and and often drop subscripts to simplify the notation. Let be a compact operator then denotes the -th Schatten class norm.
3.1. Proof of Prop. 1.3
In this subsection we shall give the proof of Prop. 1.3, up to two crucial estimates that are provided in different subsections, namely the Hölder estimate (3.13) in Subsection 3.2 and the Lipschitz estimate (3.15) in Subsection 3.3.
Proof of Prop. 1.3.
In the proof, we shall focus on Case 1 disorder as Case 2 disorder follows along the same lines but more care is needed since the potential is not positive in Case 1. We shall emphasize the differences of the two cases in our proof. Since the spectrum in Case 1 exhibits a spectral gap, see (1.14), we may focus without loss of generality on the spectrum around . The argument around is analogous. In Case 2, we do not have to restrict ourselves to those neighborhoods. Let for two closed bounded intervals , with of non-empty interior, centered at and . We decompose
(3.1) |
We then write for the second term in (3.1)
(3.2) |
The first term in (3.2) satisfies by Hölder’s inequality and the definition of
We then use the inequality
with . We can then bound (3.2), in terms of
by choosing sufficiently small
(3.3) |
Notice that while we do not have that , at least in case (1), since is not positive, we still have that
(3.4) |
To see this, observe that
(3.5) |
Indeed, since , we have by periodicity of the Hamiltonian that Since the spectrum of is uniformly gapped for small, it follows that the spectral projection is norm-continuous. We conclude from (3.5) that for
(3.6) |
with and continuous. Indeed, applying norms to (3.6), we find by substituting
in (3.6) that, since , there is such that
Rearranging this, we find
which implies that, since
showing (3.6). This then directly implies (3.4), since in the notation of (1.12)
We can easily obtain, along the same lines, an upper bound on the left-hand side of (3.4)
to see that (3.4) holds.
Finally, we have for the first term in (3.1)
(3.7) |
Here, we used in the first line of (3.7) the following identity that we shall verify below
(3.8) |
Since is the unperturbed Hamiltonian, the eigenvectors associated to spectrum in are supported in the first two entries of the wavefunction, cf. (3.5). Let be the projection onto the first two entries.
We can then define another auxiliary potential Thus, one has that . The projection onto the first two components is redundant for case disorder since in that case.
Finally to show (3.8) it suffices to show that
Since is a periodic Hamiltonian with respect to any lattice it suffices by Bloch-Floquet theory to prove the estimate for the Bloch functions of the full Hamiltonian Indeed, let be the Bloch functions associated with the spectral projection where is the set of Bloch eigenvalues inside with quasimomentum , where has a finite subset (in ) of those as eigenvectors. It then suffices to show that is strictly positive definite for all . If not, then there is and with not all zero, such that and by strict positivity of , see (1.12), we find but this implies that by real-analyticity of since is elliptic with real-analytic coefficients, which is a contradiction. Thus is a strictly positive matrix and using continuity in and compactness of , we also see that for all .
For the second term in (3.7) observe that by the boundedness of the potential
where the last term can be estimated using (3.3).
We shall now estimate the third and fourth term at the end of (3.7) for , using Young’s, the Cauchy-Schwarz inequality, and that
and similarly
Inserting the last two estimates into (3.7) and choosing small enough
Inserting this estimate into (3.1) yields
Thus, by choosing sufficiently small in (3.3)
Applying expectation values and using (3.13), which we show below, we find for
(3.9) |
which shows the result by using a partition of small intervals covering . ∎
3.2. Spectral shift function and Hölder continuity
To obtain the Hölder estimate, used to show (3.9), we recall the definition of the spectral shift function, first. Let and be two self-adjoint operator such that is trace-class, then the spectral shift function is defined as, see [Y92, Ch. , Sec. , Theo. ]
In particular for any one has the bound [CHN01, Theorem ]
(3.10) |
where the right-hand side is defined as the generalized Schatten norm
We then start by setting , with sufficiently large, such that is trace-class, with and . Then, we have the Birman-Krein formula, see [Y92, Ch.8, Sec. , Lemma ] stating that for absolutely continuous
Let then we start by defining
and
(3.11) |
We observe that this function satisfies .
Thus, we have for
which implies
Applying the expectation value to this inequality, we find by positivity of , the density of that for the expectation value with respect to all random variables and all apart from
(3.12) |
where is the Hamiltonian with replaced by the constant and Thus, using Hölder’s inequality, we find for any with (3.10) and in the regularization sufficiently large222using we can create, by choosing sufficiently large, arbitrarily large powers of the resolvent. This yields the desired trace-class condition.
(3.13) |
which is the identity used to obtain (3.9).
3.3. Spectral averaging and Lipschitz continuity
We now complete the proof of Lipschitz continuity and follow an argument developed initially by Combes and Hislop [CH94, Corr. ] for Schrödinger operators.
Proof of Theorem 2 (Lipschitz continuity).
Let where then
(3.14) |
where we used that is uniformly bounded in all parameters. Under the assumptions of Case , we know that are strictly positive on thus also which is the necessary condition [CH94, (4.2)] to apply spectral averaging which readily implies together with (3.14) that
(3.15) |
which is the identity (3.9) with for Case disorder. ∎
4. Mobility edge
To prove Theorem 3 we recall Germinet and Klein’s notion of summable uniform decay of correlations (SUDEC), see [GK06].
Definition 4.1 (SUDEC).
The Hamiltonian is said to exhibit a.e. SUDEC in an interval if its spectrum is pure point and for every closed , for an orthonormal set of eigenfunctions of with eigenvalues , we define Then for there is such that
and in addition one has -almost surely
(4.1) |
The strategy to establish delocalization is to show that if the Hamiltonian would exhibit only SUDEC-type localization (SUDEC), then this would contradict the non-vanishing Chern numbers of the flat bands.
4.1. The ingredients to the multi-scale analysis
For the applicability of the multi-scale analysis à la Germinet-Klein we require six ingredients of our Hamiltonian often referred to in their works by the acronyms, as introduced in [GK01],
-
•
Strong generalized eigenfunction expansion SGEE (Lemma 4.2),
-
•
Simon-Lieb inequality SLI and exponential decay inequality EDI (both Lemma 4.3),
- •
-
•
Independence at a distance IAD.
Here, independence at a distance (IAD) just follows from the choice of Anderson-type randomness and means that the disorder of the potentials at a certain distance are independent of each other.
We then start with the strong generalized eigenfunction expansion (SGEE). Therefore, we introduce Hilbert spaces
Lemma 4.2 (SGEE).
Let . The set is dense in and a core of Moreover, for we have
Proof.
The statement about the core is immediate, as is a core, see for instance Theorem 8. The second statement follows as is a uniformly bounded (in ) Hilbert-Schmidt operator. This is easily seen by ∎
The Simon-Lieb inequality (SLI), relating resolvents at different scales, and the eigenfunction decay inequality (EDI), relating decay of finite-volume resolvents to the decay of generalized eigenfunctions and thus Anderson localization, are discussed in the next Lemma. We thus define to be the characteristic function of the belt
For and , we define smooth cut-off functions that are equal to one on and on
Lemma 4.3 (SLI & EDI).
Let be a compact interval. For and with , then -a.s.: If then the Simon-Lieb inequality holds
In addition, we have -a.s. that any , and any generalized eigenfunction , i.e. solving and growing at most polynomially, with one has the eigenfunction decay inequality
Proof.
-
(1)
The proof of the SLI can be streamlined for linear differential operators with disorder of Anderson-type. We start from the following resolvent identity
Using that by assumption we have and find by substituting in the last line above
Since we find by multiplying the previous line by that
Multiplying this equation from the left by and from the right by , the SLI ready follows from the boundedness of and submultiplicativity of the operator norm, as implies that the second term on the right vanishes and
(4.1) -
(2)
For the proof of the EDI, it suffices to choose as in the Lemma and observe the resolvent identity which is easily verified by using that as well as Using then an analogue of (4.1), together with the boundedness of the commutator shows the claim.
∎
We complete our preparations by discussing the estimate on the number of eigenvalues (NE) and the Wegner estimate (W). The estimate on the number of eigenvalues (NE) is the estimate stated in Proposition 1.3. The Wegner estimate is then obtained by applying the estimate in Proposition 1.3 to the last expression in this set of inequalities
(4.2) |
4.2. Dynamical delocalization
In this subsection we prove Theorem 3. To imitate the proof of delocalization in [GKS07], we shall study the third power of the random Hamiltonian (1.11), since , for a two-dimensional compact manifold, is a trace-class embedding333Recall that is the Weyl asymptotics of the negative Laplacian in dimension 2; thus and is bijective, by defining
Let such that encircles the spectrum of the random perturbation of a single flat band, but nothing else (if , then both coincide, we shall explain the modifications of this case at the end of this section). This is possible for sufficiently small noise as the flat band at energies are strictly gapped (1.8) from all higher bands, in the absence of disorder. We then define the -valued spectral projection
(4.3) |
where by we just mean the set of elements in raised to the third power. The delocalization argument rests on the following two pillars:
- •
-
•
The partial Chern numbers of are invariant under disorder as well as small perturbations in away from perfect magic angles.
As a consequence, the Hamiltonian exhibits dynamical delocalization at energies close to . To simplify the notation, we drop the and just focus on , since can be treated analogously.
The central object in this discussion is the Hall conductance. Assuming for a spectral projection and multiplication operators and the Hall conductance is defined by
(4.4) |
Here, is also called the adiabatic curvature with Hall charge transport That is an integer is shown for example in [ASS94, Theorem ] or [BES94, (49),(58)] where it is related to Chern characters and Fredholm indices, respectively, and then [BES94, Theorem ] where this quantity is discussed for periodic and quasi-periodic operators.
Proof of Theo. 3.
Since is a trace-class embedding, for bounded open sets , it follows that there is a universal constant such that for sufficiently small disorder and with as above in trace norm
(4.5) |
Next, we are going to construct an analogue of the Combes-Thomas estimate (CTE) for the operator :
By conjugating the operator with where is some smooth function, we find
where
This implies that for
Thus, for and sufficiently small such that ,
We conclude that for with fixed, we have for all
(CTE) |
as well as
(4.6) |
From the Combes-Thomas estimate (CTE) and (4.3) we find the exponential estimate
(4.7) |
By [GKS07, Lemma ], this implies that
which implies that the Hall conductance is well-defined. In fact, using (4.5) we have
(4.8) |
To obtain the invariance of the Chern number under small disorder, we now define
(4.9) |
then by (4.8) we find
(4.10) |
If the random potential has compact support, i.e. in (1.11) is replaced by
(4.11) |
for some , then by using a partition of unity and (4.5), we find and consequently the traces of all commutators vanish
(4.12) |
So the integer-valued map is constant for small around zero, under the assumption of a compactly supported random potential in (4.11).
It remains now to drop the compact support constraint on the random potential in (4.11). Let , then we define
(4.13) |
where is the corresponding spectral projection associated with By the Combes-Thomas estimates (CTE) and the resolvent identity (4.13), we find
for some , where we used that is zero on Thus, writing the difference of Hall conductivities yields the desired limit
(4.14) |
Here, one uses the strong limit to show the non-vanishing of the first term on the right-hand side in (4.14) and that
with a similar estimate for the last term in (4.14). The last bound converges to zero for by using (4.8) and (4.10), see [GKS07, Lemma 3.1 (i)] for details. Thus, the conductivity derived from is locally constant in and , see (4.12), which shows using (1.10) that Chern numbers stay , for , respectively.
For we repeat the previous computation with our modified (B.3) to arrive at the same conclusion. Thus, if, in the notation of (1.14), then this would contradict the non-vanishing of the (partial) Chern number, see (B.6), in regions of full localization as shown in Prop. B.2.
∎
4.3. Dynamical localization
Working under assumptions (1), we shall now study the localized phase of the Anderson model of the form
(4.15) |
Here we got rid of the parameter but instead consider random variables that are distributed according to a bounded density of compact support in with for and for . Here is a rescaled distribution , with , such that as the mass gets concentrated near zero and , uniformly in , is the normalizing constant.
By (1.13), with probability , the spectrum is independent of Our next theorem shows that the mobility edges can be shown to be located arbitrarily close to the original flat bands, by choosing small, while keeping the support of the disorder fixed, within the interval which is the motivation for our modifications of the Hamiltonian.
Theorem 7 (Mobility edge).
Let be bounded for some and let . Let be as in Assumption 1 with the modification that is incorporated in the rescaled density, as described in (4.15) and small enough. Then for any there exist at least two distinct dynamical mobility edges, denoted by such that
In particular,
where the region of dynamical localization has been defined in (1.18). In the case of the same result holds but with only at least one guaranteed mobility edge.
Proof.
We start by observing that using the bound on , we have for any and
(4.16) |
Thus, for the probability of the low-lying spectrum to be contained in a small interval , we find for fixed
for small enough . We recall that is such that This probability is large, if we choose
(4.17) |
for To prove localization, one chooses large enough, as specified in [GK03, (2.16)] and . We now fix an energy such that with . Then is, with high probability, a distance away from the spectrum of the finite-size Hamiltonian .
In order to show localization, we shall satisfy the finite-size criterion of [GK03, Theorem ]. This will give us another condition aside from (4.17). Indeed, in our setting the finite-size criterion stated in [GK03, Theorem ] takes the following form
(4.18) |
for two constants The term is obtained from [GK03, Theorem ] by choosing (in the notation of [GK03]) , and performing a union bound over a partition of and which accounts for another The in the denominator is due to the scaling of the constant in the Wegner estimate which for us is proportional to the supremum norm of the density, which for us is .
5. Decay of point spectrum and Wannier bases
We now give the proof of Theo. 4 and 5. We shall mainly focus on the first case and only explain the modifications for the second result at the very end.
Proof of Theo.4 & 5.
We first reduce the analysis to By -continuity of the random perturbation, the spectral projections and with as in (1.15)
by using e.g. the resolvent identity and holomorphic functional calculus and the spectral gap of the Hamiltonian. Thus, for small enough there is an isometry [BES94, Lemma ] such that and In particular It then follows that has a Schwartz kernel that is exponentially close to the identity, cf. [CMM19, Lemma ]. By this we mean that there is such that
The Schur test for integral operators implies that is a family of operators uniformly bounded in . This implies that for any
Taking norms, we find, using that by assumption, that
This implies, by choosing for an orthonormal basis of , i.e. is an orthonormal basis of , then , that exhibits a -localized generalized Wannier basis. Since is precisely the projection onto , we deduce that exhibits a non-zero Chern number, see (1.10), and therefore do not possess a -localized Wannier basis, see [LS21] which gives a contradiction.
Conversely, let , where is a sufficiently small circle around zero encircling only the flat band eigenvalue but nothing else in the spectrum of . Then is the spectral projection onto the flat band eigenfunction of . Since is real-analytic, this implies that is real-analytic. Moreover, since with with the spectral projection satisfies the covariance relation
It then follows from [MPPT18, Theo. ] that there exists an associated Wannier basis satisfying for and all for the unperturbed periodic problem. Reversing the argument provided in the first part of the proof, it follows that the randomly perturbed problem also exhibits such a Wannier basis.
To show Theorem 5 one proceeds analogously and notices that correspond to the projections onto and , each one exhibiting a non-zero Chern number. ∎
With this result at hand, we are able to evaluate the quantity (1.17) for the unperturbed Hamiltonian providing a link between the dynamical and spectral theoretic notion of (de)-localization.
Proposition 5.1.
Proof.
We start by observing that for an orthonormal basis of and the standard basis of
Without loss of generality, we shall focus on the first summand. Consider the unitary Bloch-Floquet transform , where has been defined in (1.4), with the convention that and its inverse/adjoint . We then find that
(5.1) |
Since by assumption , we see that
(5.2) |
forms a basis of the space . Indeed, orthonormality just follows from
(5.3) |
and completeness from the completeness of the regular Fourier expansion, i.e. a general element in this subspace is of the form
We then have that Recall the trivial decomposition of given by
We then find for the Hilbert-Schmidt norm using an orthonormal basis of
Since by assumption is a rank projection, we have
This implies that
However, a Wannier basis is obtained from by defining . Indeed, using (5.3) functions are an orthonormal basis of as
and span due to (5.1) and (5.2). Thus, we obtain since is an isometry that
From the non-existence of a -localized Wannier basis and the existence of a Wannier basis, for any , see for instance [MPPT18], we find that for and is finite for
∎
Appendix A Essential self-adjointness
In this appendix, we recall the essential self-adjointness of our Hamiltonian with even possibly unbounded disorder on .
Theorem 8.
The Hamiltonian (1.11) is, under the more general assumptions, with -bounded density for random variables and arbitrary density is almost surely essentially self-adjoint on
Proof.
To see that is essentially self-adjoint, we first observe that it is symmetric on It thus suffices to show that for any -normalized
i.e. the deficiency indices are zero. Elliptic regularity and the assumption that implies that . We then pick a cut-off function with and and find
We conclude that
Since by dominated convergence, we conclude that ∎
Appendix B Partial Chern numbers
Let be an orthogonal projection on such that for some , , and we have
(B.1) |
This condition is satisfied for spectral projections of Hamiltonians under the assumption of (SUDEC), cf. Def. 4.1. Let and . By the definition of the Hilbert-Schmidt norm one finds for all
(B.2) |
We define the new and replace (4.4) by
(B.3) |
which is well-defined for
(B.4) |
Remark 4.
It is convenient to modify rather than in the definition of , since is in general no longer a projection, even for
Since we still have that we find the equivalent formulation of (B.3)
(B.5) |
In particular, if is a finite-rank projection then, we always find , as (B.5) is a commutator of trace-class operators.
To provide further motivation for the above definition (B.3), we shall consider the unperturbed Hamiltonian then and consequently any spectral projection of is also diagonal and thus of the form Thus, we have
where we recall from (1.10) that for a generic magic angle and with
(B.6) |
Thus, while for , we have The definition of captures the non-trivial sublattice Chern numbers of twisted bilayer graphene while the total Chern number vanishes.
One also readily verifies the usual properties of Chern characters, see for instance [GKS07, Lemma 3.1], [BES94]:
Proposition B.1.
Proof.
The second property follows from a direct computation, see [GKS07, Lemma 3.1 (ii)].
We also want to mention reference [ASS94, Sec.6] showing full details on how to obtain the second point and [BES94, Lemma ] for the third point.
The independence of switch functions in Prop. B.1 implies that is an almost surely constant quantity
The purpose of the first and last point in Prop. B.1 is to conclude that in regions of , cf. Definition 4.1, all vanish.
Proposition B.2.
Let exhibit in an interval , then for all closed we have
Proof.
Let be a (finite or infinite) enumeration (counting multiplicities) of all point spectrum of . We can then write the spectral projection as
where are rank one projections. In addition, we have where are defined in (4.1). Using the third item in Prop. B.1 we then have for any
Invoking then the first item in Prop. B.1, we find that as we make arbitrarily large or equal to , if is finite, we obtain ∎
Acknowledgements:. We thank Jie Wang for suggesting the relevance of different disorder types for TBG and Maciej Zworski for initial discussions on the project. M. Vogel was partially funded by the Agence Nationale de la Recherche, through the project ADYCT (ANR-20-CE40-0017). I. Oltman was jointly funded by the National Science Foundation Graduate Research Fellowship under grant DGE-1650114 and by grant DMS-1901462.
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