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Large power dissipation of hot Dirac fermions in twisted bilayer graphene

S. S. Kubakaddi [email protected] Department of Physics, K. L. E. Technological University, Hubballi-580031, Karnataka, India
Abstract

We have carried out a theoretical investigation of hot electron power loss PP, involving electron-acoustic phonon interaction, as a function of twist angle θ\theta, electron temperature TeT_{e} and electron density nsn_{s} in twisted bilayer graphene (tBLG). It is found that as θ\theta decreases closer to magic angle θm\theta_{m}, PP enhances strongly and θ\theta acts as an important tunable parameter, apart from TeT_{e} and nsn_{s}. In the range of TeT_{e} =1-50 K, this enhancement is \sim 250-450 times the PP in monolayer graphene (MLG), which is manifestation of the great suppression of Fermi velocity vF{v_{F}}^{*} of electrons in moiré flat band. As θ\theta increases away from θm\theta_{m}, the impact of θ\theta on PP decreases, tending to that of MLG at θ\theta \sim 3. In the Bloch-Grüneisen (BG) regime, PP \sim Te4{T_{e}}^{4}, ns1/2{n_{s}}^{-1/2} and vF2{v_{F}}^{*-2}. In the higher temperature region (\sim10- 50 K), PP \sim Teδ{T_{e}}^{\delta}, with δ\delta\sim 2.0, and the behavior is still super linear in TeT_{e}, unlike the phonon limited linear-in- TT ( lattice temperature) resistivity ρp\rho_{p}. PP is weakly, decreasing (increasing) with increasing nsn_{s} at lower (higher) TeT_{e}, as found in MLG. The energy relaxation time τe\tau_{e} is also discussed as a function of θ\theta and TeT_{e}. Expressing the power loss P=Fe(Te)Fe(T)P=F_{e}(T_{e})-F_{e}(T), in the BG regime, we have obtained a simple and useful relation Fe(T)μp(T)=(evs2F_{e}(T)\mu_{p}(T)=(e{v_{s}}^{2}/2) i.e. Fe(T)=(nse2vs2/2)ρpFe(T)=(n_{s}e^{2}{v_{s}}^{2}/2)\rho_{p}, where μp\mu_{p} is the acoustic phonon limited mobility and vsv_{s} is the acoustic phonon velocity. The ρp\rho_{p} estimated from this relation using our calculated Fe(T)F_{e}(T) is nearly agreeing with the ρp\rho_{p} of Wu et al (Phys. Rev. B 99, 165112 (2019)).

preprint: APS

I INTRODUCTION

Recent pioneering experimental discoveries in twisted bilayer graphene (tBLG) by Cao et al Cao et al. (2018a, b), have created great interest in the study of their electronic properties and has ushered in a new era in the condensed matter physics Wu et al. (2018); Yankowitz et al. (2019); Lu et al. (2019); Sharpe et al. (2019); Tomarken et al. (2019); Roy and Juričić (2019); Serlin et al. (2020); Polshyn et al. (2019); Cao et al. (2020); Wu et al. (2019); Das Sarma and Wu (2020). Among the discoveries, the existence of correlated insulating phases and superconductivity at low temperatures and a highly resistive linear-in-temperature TT resistivity ρ\rho at high temperature, are remarkable and exciting Cao et al. (2018a, b); Yankowitz et al. (2019). Very recently, the observation of a quantum anomalous Hall effect in twisted bilayer graphene aligned to hexagonal boron nitride has been reported in tBLG Serlin et al. (2020). In tBLG a small twist angle θ\theta, near the magic angle θm\theta_{m}, between the two layers plays the most significant role and acts as one of the tunable parameters, similar to the carrier density nsn_{s} and temperature TT, of the samples in limiting their electronic properties Cao et al. (2018a, b); Yankowitz et al. (2019); Wu et al. (2019); Das Sarma and Wu (2020). The transport results of Cao et al Cao et al. (2020) establish magic angle bilayer graphene as a highly tunable platform to investigate ‘strange metal’ behavior. Because of the twist between the layers the band structure is a moiré flat band with the twist angle dependent suppressed Fermi velocity vF(θ{v_{F}}^{*}(\theta) <vF<v_{F}, the bare Fermi velocity in monolayer graphene, and the large density of states D(Ek)D(E_{k}) near θm\theta_{m} at which vF(θ{v_{F}}^{*}(\theta) = 0 Wu et al. (2019); Das Sarma and Wu (2020); Bistritzer and MacDonald (2011). The strongly enhanced electrical resistivity ρ\rho, near θm\theta_{m}, with linear-in-temperature behavior has been observed for T>T>\sim 5 K Polshyn et al. (2019); Cao et al. (2020).

Theoretically, the electrical resistivity has been investigated in tBLG, at higher temperature and away from the moiré miniband edge, by considering the effect of electron- acoustic phonon (el-ap) interaction Polshyn et al. (2019); Wu et al. (2019); Das Sarma and Wu (2020). It is shown that the phonon limited resistivity ρp\rho_{p} = ρ\rho (T, θ\theta) is strongly enhanced in magnitude, twist-angle dependent and linear-in- TT occurring for T>TLT>T_{L}, where TLT_{L} (on the order of few kelvins) is the temperature above which linearity in ρ(T,θ)\rho(T,\theta) develops. This linear-in- TT is observed for TL=TBG/8T_{L}=T_{BG}/8 Das Sarma and Wu (2020), where TBG=2vskF/kBT_{BG}=2\hbar v_{s}k_{F}/k_{B} is the Bloch- Grüneisen (BG) temperature, vsv_{s} is the acoustic phonon velocity, and kF=πns/2k_{F}=\sqrt{\pi n_{s}/2} is the Fermi wave vector in tBLG. The enhancement in ρ(T,θ)\rho(T,\theta), about three orders of magnitude greater than that in monolayer graphene (MLG) at TT\sim 10 K, is shown to arise from the large increase in the effective el-ap scattering in tBLG due to the suppression of vFv_{F} induced by the moiré flat band. In the metallic regime i.e. for T>Tm(<TL)T>T_{m}(<T_{L}), where TmT_{m} is the metallic temperature, above which dρ(T,θ)/dT>0d\rho(T,\theta)/dT>0, and it is nsn_{s} and θ\theta dependent. The ρ(T,θ\rho(T,\theta) is found to increase with increasing TT as the twist angle θ\theta approaches θm\theta_{m}. The linear dispersion taken for the Dirac fermions in tBLG is an approximation that is valid for Fermi energy near the Dirac point and hence its transport study is limited to the ns1012n_{s}\leq 10^{12} cm-2. Interestingly, it is also shown that the same enhanced el-ap interaction can also produce superconductivity with Tc1KT_{c}\sim 1K in s, p, d and f orbital pairing channels Wu et al. (2018, 2019).

The theory of Wu et al Wu et al. (2019); Das Sarma and Wu (2020) explains the available experimental data of ρ\rho well for T>T> 5K Polshyn et al. (2019); Cao et al. (2020). In their theory, all the effects of disorder, impurities and defects are ignored assuming that the system is extremely clean and the Fermi energy is slightly away from the Dirac point. However, the hot electron relaxation is an important transport property which is controlled by only electron-phonon interaction and independent of disorders and impurities.

The electron system in samples subject to large electric fields or photoexcitation establishes its internal thermal equilibrium at an electron temperature TeT_{e} greater than the lattice temperature TT because electron-electron interaction occurs at the time scale of several femtoseconds which is much smaller than the electron-phonon scattering time. Consequently, the electron system is driven out of equilibrium with the lattice. In steady state, these electrons will relax towards equilibrium with the lattice by dissipating energy with phonons as the cooling channels. The study of hot electron power loss PP is important as it affects thermal dissipation and heat management which are key issues in nanoscale electronics device. Moreover, it is crucial for applications in variety of devices such as calorimeters, bolometers, infrared detectors, ultrafast electronics and high speed communications. Hot electron cooling has been extensively studied theoretically and experimentally in MLG Kubakaddi (2009); Tse and Das Sarma (2009); Bistritzer and MacDonald (2009); Viljas and Heikkilä (2010); Betz et al. (2012); Baker et al. (2012); Low et al. (2012); Baker et al. (2013); Somphonsane et al. (2013); Laitinen et al. (2015) and conventional bilayer graphene (BLG) Viljas and Heikkilä (2010); Katti and Kubakaddi (2013); Bhargavi and Kubakaddi (2014); Huang et al. (2015).

In the present work, we investigate the effect of enhanced el-ap coupling on the power dissipation PP of the hot electrons in moiré flat band in tBLG. It is studied as a function of twist angle, electron temperature and electron density. We show that the twist angle θ\theta acts as one of the strong tunable parameters of PP. Additionally, a relation between power loss and phonon limited mobility μp\mu_{p} is brought out in BG regime.

II Theoretical model

Wu et al Wu et al. (2019) have used the effective Dirac Hamiltonian with a renormalized velocity for electron energy spectrum, in order to obtain their analytical results. In moiré flat band, the electron energy spectrum is assumed to be Dirac dispersion Ek=vF|k|E_{k}=\hbar{v_{F}}^{*}|k|, which is an approximation that is valid for near Dirac point, with an effective Fermi velocity vFvF(θ){v_{F}}^{*}\equiv{v_{F}}^{*}(\theta). Because of this approximation our theory will be limited to the carrier density ns1012n_{s}\leq 10^{12} cm-2. The density of states is D(Ek)=g(Ek)/[2π(vF)2]D(E_{k})=g(E_{k})/[2\pi{(\hbar{v_{F}}^{*})}^{2}] with the degeneracy gg = gsg_{s} gvg_{v} glg_{l}, where gsg_{s}, gvg_{v} and glg_{l} are, respectively, spin, valley and layer degeneracy each with the value of 2. We consider electron-acoustic phonon interaction within the deformation potential approximation with the longitudinal acoustic (LA) phonons of energy ωq\hbar\omega_{q} and wave vector q interacting with the tBLG Dirac electrons in the moiré miniband. The LA phonons in tBLG are assumed to be unaffected by the tBLG structure and are taken to be the same as the MLG phonons. In MLG the experimental observations of electrical conductivity Efetov and Kim (2010) and power loss Betz et al. (2012); Baker et al. (2012, 2013) are very well explained by the electron interaction with only LA phonons, without screening. Wu et al Wu et al. (2019); Das Sarma and Wu (2020) have explained the linear-in-T resistivity data in tBLG with only electron-LA phonon interaction. We use the modified ordinary el-ap matrix element Wu et al. (2019) |M(q)|2=[(D2qF(θ))/(2Aρmvs)][1(q2/4k2)]{|M(q)|}^{2}=[(D^{2}\hbar qF(\theta))/(2A\rho_{m}v_{s})][1-(q^{2}/4k^{2})] where DD is the first-order acoustic deformation potential coupling constant, AA is the area of the tBLG, ρm\rho_{m} is the areal mass density and vsv_{s} is the LA phonon velocity. The detailed tBLG moiré wave function gives rise to the form factor function F(θ)F(\theta) which modifies the el-ap interaction matrix element in tBLG as compared with the MLG Wu et al. (2019). It is shown to be between 0.5 and 1.0 and being nearly parabolic for 1 << θ<\theta< 2 in the neighborhood of a minimum at θ\theta = \sim 1.3 Das Sarma and Wu (2020). Following the Refs. Kubakaddi (2009); Manion et al. (1987); Kaasbjerg et al. (2014), and taking care of additional layer degeneracy, we obtain an expression for the electron power loss in tBLG and it is given by

P=gD2F(θ)4π2nsρm5vs3vF30d(ωq)(ωq)2γ𝑑Ek(Ek+ωq)[1(γ/Ek)2]1/2×G(Eq,Ek)[Nq(Te)Nq(T)][f(Ek)f(Ek+ωq)],P=-\frac{gD^{2}F(\theta)}{4\pi^{2}n_{s}\rho_{m}\hbar^{5}{v_{s}}^{3}{{v_{F}}^{*}}^{3}}\int_{0}^{\infty}d(\hbar\omega_{q}){(\hbar\omega_{q})}^{2}\int_{\gamma}^{\infty}dE_{k}\frac{(E_{k}+\hbar\omega_{q})}{{[1-{(\gamma/E_{k})}^{2}]}^{1/2}}\times G(E_{q},E_{k})[N_{q}(T_{e})-N_{q}(T)][f(E_{k})-f(E_{k}+\hbar\omega_{q})], (1)

where nsn_{s} is the electron density, γ=(Eq/2)\gamma=(E_{q}/2), Eq=vFqE_{q}=\hbar{v_{F}}^{*}q, Nq(T)=[exp(ωq/kBT)1]1N_{q}(T)={[exp(\hbar\omega_{q}/k_{B}T)-1]}^{-1} is the Bose-Einstein distribution at lattice temperature TT and G(Eq,Ek)=[1(γ/Ek)2]G(E_{q},E_{k})=[1-{(\gamma/E_{k})}^{2}], is due to the spinor wave function of the electron in the electron -phonon matrix element, in the quasi-elastic approximation Kubakaddi (2009). By setting F(θ\theta) =1, glg_{l} = 1 and vF(θ)=vF{v_{F}}^{*}(\theta)=v_{F} in Eq.(1), we regain the equation that is applicable to MLG Kubakaddi (2009) and silicene Kubakaddi and Phuc (2020), similar to the acoustic phonon induced resistivity in tBLG Polshyn et al. (2019); Wu et al. (2019). The twist angle dependence of vFvF(θ){v_{F}}^{*}\equiv{v_{F}}^{*}(\theta) is shown to be very well approximated by Polshyn et al. (2019); Das Sarma and Wu (2020)

vF0.5|θθm|vF,{v_{F}}^{*}\approx 0.5|\theta-\theta_{m}|v_{F}, (2)

which clearly indicates that twist angle effect is very large for θ\theta closer to θm\theta_{m}. We use this relation while computing PP for different twist angles.

In the Bloch-Grüneisen (BG) regime TT, TeT_{e} <<TBG<<T_{BG}, q<<q<< 2kFk_{F}, the power loss is given by

P=Σ(Te4T4)/ns1/2,P=\Sigma({T_{e}}^{4}-T^{4})/{n_{s}}^{1/2}, (3)

where Σ=Σ0(D2/vs3)\Sigma=\Sigma_{0}(D^{2}/{v_{s}}^{3}) and Σ0=(gπ5/2kB4F(θ))/(602ρm4vF2)\Sigma_{0}=(g\pi^{5/2}{k_{B}}^{4}F(\theta))/(60\sqrt{2}\rho_{m}\hbar^{4}{{v_{F}}^{*}}^{2}). Hence, in BG regime PT4P\sim T^{4}, ns1/2{n_{s}}^{-1/2} and vF2{{v_{F}}^{*}}^{-2}.

III Results and discussion

We obtain the following numerical results of power loss in tBLG using the parameters Wu et al. (2019); Das Sarma and Wu (2020): ρm=7.6×108\rho_{m}=7.6\times 10^{-8} gm/cm2, θm\theta_{m} = 1.02, vsv_{s} = 2×\times106 cm/s, vFv_{F} = 1×\times108 cm/s and DD = 20 eV Kubakaddi (2009); Bistritzer and MacDonald (2009); Baker et al. (2012); Efetov and Kim (2010); DaSilva et al. (2010); Hwang and Das Sarma (2008), noting that Polshyn et al Polshyn et al. (2019) and Wu et al Wu et al. (2019) have used DD = 25 ± 5 eV. In order to bring out the angular dependence of the power loss, we confine our illustrations for θ\theta =1.1, 1.2 and 1.3 which are closer to magic angle θm\theta_{m} =1.02. For these angles, the effective Fermi velocity vF{v_{F}}^{*} = 4, 9 and 14×\times106 cm/s (>> 1.5 vsv_{s} Wu et al. (2019)), respectively, which are much smaller than the bare vFv_{F}, and the effect of vF{v_{F}}^{*} on the transport coefficients will be very large. For, further increase of θ\theta, vF{v_{F}}^{*} tends to vFv_{F} at about 3.0. The values of the function F(θ)F(\theta) for different θ\theta are taken from figure 3 of Das Sarma et al Das Sarma and Wu (2020), and because of its value between 0.5 and 1, it will have smaller influence on PP than vF{v_{F}}^{*}. We have presented the calculations for lattice temperature TT = 0.1 K, and ns=0.11n0n_{s}=0.1-1n_{0}, with n0n_{0} =1×\times1012 cm-2, which keeps us slightly away from the Dirac point and within the linear region of moiré flat band. For ns=Nn0n_{s}=Nn_{0}, TBG=38.3NT_{BG}=38.3\sqrt{N} which is smaller by a factor of 2\sqrt{2} compared to MLG.

[Uncaptioned image]
[Uncaptioned image]
Refer to caption
Figure 1: Electron temperature TeT_{e} dependence of the power loss PP in tBLG for twist angle θ\theta = 1.1, 1.2 and 1.3. (a) PP vs TeT_{e} for ns = n0, (b) P/Te4P/T_{e}^{4} vs TeT_{e} for nsn_{s} = n0n_{0} and (c) PP vs TeT_{e} for nsn_{s}=0.5n0n_{0}.
Refer to caption
Figure 2: Power loss PP as a function of electron temperature TeT_{e} for nsn_{s} = n0n_{0} in tBLG ( θ\theta = 1.1), MLG and BLG.

First we explore the dependence of power loss PP on electron temperature TeT_{e} for twist angles θ\theta =1.1, 1.2 and 1.3. In figure 1a, PP is presented as a function of TeT_{e} (1-50 K) for ns=n0n_{s}=n_{0}. For all the θ\theta, we observe the generic nature of the behavior, where in at very low TeT_{e} power loss increases rapidly then slows down at higher temperature. For the temperatures TeT_{e} <<<< TBGT_{BG}, the rapid increase may be attributed to the increasing number of phonons as their wave vector qkBTe/vsq\approx k_{B}T_{e}/\hbar v_{s} increases linearly with TeT_{e}. For θ\theta =1.1, the power law PTe4P\sim{T_{e}}^{4} is found to be obeyed for Te<T_{e}<\sim 2.5 K, which is about TBGT_{BG}/15. The exponent 4 of TeT_{e} is manifestation of two-dimensional phonons with unscreened electron-phonon coupling. In order to see the effect of θ\theta on the range of validity of the power law, we have plotted P/Te4P/{T_{e}}^{4} vs TeT_{e} in figure 1b. It is found that, as θ\theta increases the range of TeT_{e} in which power law is obeyed marginally increases. For example, for θ\theta =1.2 and 1.3, power law is found to be satisfied for TeT_{e} up to about 3 and 3.5 K, respectively, although TBGT_{BG} is same. This happens because as θ\theta increases vF{v_{F}}^{*} also increases and tends towards vFv_{F}. In the BG regime, in which PP\sim vF2{{v_{F}}^{*}}^{-2}, we find Σ\Sigma = 2.66×\times10/15N{}^{-15}/\sqrt{N} W/K4-cm, 5.13×\times10-16/N\sqrt{N} W/K4-cm and 2.1×\times10-16 /N\sqrt{N} W/K4, for θ\theta =1.1, 1.2 and 1.3, respectively, as compared to 5.23×1018/N\times 10^{-18}/\sqrt{N} W/K4-cm in MLG. In the higher temperature region of TeT_{e} = 10 - 50 K (30 - 50 K), PTeδP\sim{T_{e}}^{\delta} with δ\delta \sim 2.0 - 2.2 (\sim 1.7 - 2.0), for all θ\thetas, as compared to the resistivity which is found to show linear-in-temperature for temperature \geq TBGT_{BG}/8 Das Sarma and Wu (2020).

In figure 1c, TeT_{e} dependence of PP is shown for nsn_{s} = 0.5 n0n_{0} and the same behavior is observed as in figure 1a. However, for the same θ\theta, in the low temperature region PP is found to be marginally larger (smaller) at lower (higher) TeT_{e} than that for nsn_{s} = n0n_{0}. We observe that the temperature below which the power law PTe4P\sim{T_{e}}^{4} is obeyed shifts to lower side for smaller nsn_{s}. For example, for θ\theta =1.1 power law is obeyed for Te<T_{e}<\sim2 K, which may be attributed to the lower TBGT_{BG} = 27.0 K. More importantly, from the figures 1a and 1c, we find that θ\theta acts as a tunable parameter of power loss, in addition to TeT_{e} and nsn_{s}. The influence of θ\theta on PP is very much large compared to nsn_{s}. For θ\theta =1.1 and 1.3, for the TeT_{e} range considered, PP is in the range 104109\sim 10^{4}-10^{9} eV/s and 103108\sim 10^{3}-10^{8} eV/s, respectively. These values are comparable to those in monolayer MoS2 Kaasbjerg et al. (2014) but about three and four orders of magnitude greater than those in GaAs heterojunction Ma et al. (1991) and Si-inversion layer Fletcher et al. (1997), respectively.

In order to compare the power loss in tBLG with that in MLG and conventional BLG, PP dependence on TeT_{e} is depicted in figure 2, for nsn_{s} = n0n_{0} with PP(tBLG) taken for θ\theta =1.1. We find that the power loss in tBLG is very large (2×1042×109\sim 2\times 10^{4}-2\times 10^{9} eV/s) compared to that in MLG (4×1016×106\sim 4\times 10^{1}-6\times 10^{6} eV/s) and BLG (9×1013×107\sim 9\times 10^{1}-3\times 10^{7} eV/s) Bhargavi and Kubakaddi (2014). Defining a ratio RpR_{p} = PP(tBLG)/ PP(MLG), it is found that RpR_{p} = \sim 450, 260 and 300, respectively, at 1, 10 and 50 K, and RpR_{p} is expected to be smaller for larger θ\theta. This enhancement is attributed to the significantly reduced vF{v_{F}}^{*}. This may be compared with the ρ\rho enhancement in tBLG, which is of three orders of magnitude greater than that in MLG at \sim10 K Wu et al. (2019); Das Sarma and Wu (2020). It is also noticed that the range of TeT_{e} in which power law is obeyed is much larger in MLG than in tBLG.

[Uncaptioned image]
Refer to caption
Figure 3: Power loss PP as a function of electron density nsn_{s} in tBLG for θ\theta = 1.1, 1.2 and 1.3. (a) TeT_{e} = 1 K and (b) TeT_{e} = 5K.

We have presented in figure 3 the electron density (=0.1-1.0 n0n_{0}) dependence of the power dissipation for two electron temperatures TeT_{e} = 1 K (figure 3a) and 5 K (figure 3b). For nsn_{s} = 0.1(1.0) n0n_{0} the TBGT_{BG} = 12.1 (38.3) K. From figure 3a, we see that PP is found to decrease with increasing nsn_{s}, as found in MLG Kubakaddi (2009); Baker et al. (2013), with power law PP \sim ns1/2{n_{s}}^{-1/2} being followed at larger nsn_{s} and small deviation occurring at lower nsn_{s}. This is due to the fact that TBGT_{BG} goes on decreasing with decreasing nsn_{s}. The PP ns1/2\sim{n_{s}}^{-1/2} dependence in tBLG is in contrast to the PP ns3/2\sim{n_{s}}^{-3/2} dependence in conventional BLG Bhargavi and Kubakaddi (2014); Huang et al. (2015). On the other hand for TeT_{e} = 5 K (figure 3b), PP increases (flattens) with increasing nsn_{s} in the low (high) nsn_{s} region, because we are moving away from the TeT_{e} <<<< TBGT_{BG} region.

Refer to caption
Figure 4: Energy relaxation time τe\tau_{e} as a function of electron temperature TeT_{e} for nsn_{s} = n0n_{0} in tBLG (θ\theta = 1.1, 1.2 and 1.3) and MLG.

The energy relaxation time τe\tau_{e} is another important quantity studied in the hot electron relaxation process, as it determines the samples suitability for its applications in optical detectors (bolometer, calorimeter and infrared detectors) and .high speed devices. For a degenerate electron gas it is given by τe\tau_{e} = [(p+1)(πkB)2(Te2T2)/(6EFP)][(p+1){(\pi k_{B})}^{2}({T_{e}}^{2}-T^{2})/(6E_{F}P)], where pp is the exponent of energy in density of states and EFE_{F} is the Fermi energy Baker et al. (2012); Kubakaddi and Biswas (2018). In BG regime, since PP Te4\sim{T_{e}}^{4} and ns1/2{n_{s}}^{-1/2}, we find τe\tau_{e} Te2\sim{T_{e}}^{-2} and independent of nsn_{s} (as EFE_{F} \sim ns1/2{n_{s}}^{1/2}). In figure 4, τe\tau_{e} is presented as a function of TeT_{e}, for θ\theta = 1.1, 1.2 and 1.3, in tBLG along with the τe\tau_{e} in MLG for nsn_{s} = n0n_{0}. In both tBLG and MLG, τe\tau_{e} is found to decrease with increasing TeT_{e} and the decrease is rapid at lower temperature (<<\sim10 K). It is found that τe\tau_{e} in tBLG, for θ\theta =1.1, is an order of magnitude smaller than that in MLG and this difference decreases with increasing θ\theta. The ratio τe\tau_{e} (MLG)/ τe\tau_{e} (tBLG), for θ\theta =1.1, is found to be 10.0, 6.6 and 6.9, respectively, for TeT_{e} = 5, 10 and 20 K. This ratio is not as large as the ratio of PP’s, because of the product EFPE_{F}P in the denominator of the expression for τe\tau_{e}, noting that for the same nsn_{s}, the EFE_{F} in tBLG is much smaller than that in MLG. By increasing θ\theta the τe\tau_{e} increases significantly, indicating that twist angle is an important tunable parameter for τe\tau_{e} also. It may be noted that samples with faster energy relaxation (i.e. smaller τe\tau_{e}) find applications in ultrafast electronics and high speed communications. On the other hand, samples with longer energy relaxation time are preferred in photodetectors and energy harvesting devices like hot carrier solar cells.

Finally, in BG regime, we bring out a simple relation of PP with phonon limited mobility μp\mu_{p} and resistivity ρp\rho_{p} in tBLG. In this regime, PP, μp\mu_{p} and ρp\rho_{p} are sensitive measures of the el-ap coupling. While PP is determined by the energy relaxation through el-ap interaction, μp\mu_{p} and ρp\rho_{p} involve momentum relaxation through the same mechanism. A relation between these measurable properties is expected because of the same underlying mechanism. This kind of relation between PP and μp\mu_{p} is listed for different electron systems in Ref Kubakaddi (2017). In tBLG, the equation ρp(T)=AT4\rho_{p}(T)=AT^{4} for the phonon limited resistivity is obtained from Min et al Min et al. (2011) with suitable replacement of gsgvg_{s}g_{v} by gsgvglg_{s}g_{v}g_{l}, kF=(πns/2)k_{F}=\sqrt{(\pi n_{s}/2)} and inserting F(θ)F(\theta) in the numerator in their Eq. (8) for A. There by, using the relation μp(T)=1/(nseρp(T))\mu_{p}(T)=1/(n_{s}e\rho_{p}(T)), the phonon limited mobility is found to be μp(T)=[15(ge4ρmvs5vF2ns1/2T4)][162π5/2D2kB4F(θ)]\mu_{p}(T)=[15(ge\hbar^{4}\rho_{m}{v_{s}}^{5}{{v_{F}}^{*}}^{2}{n_{s}}^{1/2}T^{-4})][16\sqrt{2}\pi^{5/2}D^{2}{k_{B}}^{4}F(\theta)], where ee is the electron charge. Expressing Eq. (3) as P=Fe(Te)Fe(T)P=F_{e}(T_{e})-F_{e}(T) Kubakaddi (2009); Ma et al. (1991), where Fe(T)=ΣT4/ns1/2F_{e}(T)=\Sigma T^{4}/{n_{s}}^{1/2} and P=Fe(Te)P=F_{e}(T_{e}) for Te>>TT_{e}>>T, we obtain a very simple relation Fe(T)μp(T)=(evs2/2)F_{e}(T)\mu_{p}(T)=(e{v_{s}}^{2}/2), which is exactly same as that of MLG Kubakaddi (2017). This relation is analogous to Herring’s law Herring (1954), which relates phonon-drag thermopower SgS^{g} and μp\mu_{p}. Alternatively, power loss can be related to ρp\rho_{p} by the formula Fe(T)=(nse2vs2/2)ρp(T)F_{e}(T)=(n_{s}e^{2}{v_{s}}^{2}/2)\rho_{p}(T). The advantage of these relations is, if Fe(T)F_{e}(T) is measured then μp(T)\mu_{p}(T) and ρp(T)\rho_{p}(T) can be determined or the vice-versa, and the measurements of power loss may be preferred as it is independent of lattice disorders and impurities. From our calculated value of P=Fe(T)P=F_{e}(T) = 4.45×1014\times 10^{-14} W at 2 K for θ\theta =1.1 and nsn_{s} = n0n_{0}, we estimate ρp(T)\rho_{p}(T) = 0.8 Ω\Omega, which is nearly agreeing with the value obtained by Wu et al (see figure 4a of Wu et al. (2019)), and μp(T)\mu_{p}(T) = 7.5×106\times 10^{6} cm2/V-s.

We would like to make the following remarks. In the literature the values of θm\theta_{m} given are varying between 1.02 to 1.1 Cao et al. (2018a); Roy and Juričić (2019); Wu et al. (2019); Das Sarma and Wu (2020). However, we believe that our findings and analysis with θm\theta_{m} = 1.02 Wu et al. (2019); Das Sarma and Wu (2020) hold good for the θ\theta values closer to any chosen θm\theta_{m}. We want to emphasize that, our analytical results will be of great help to experimental researchers and secondly can be used to determine DD as the measurements of PP are independent of lattice disorder and impurities, unlike resistivity.

IV Conclusions

We have studied the hot electron power loss PP due to the simple acoustic phonon interaction, via deformation potential coupling, in tBLG of low electron density nsn_{s}\leq 1012 cm-2 for small twist angles θ\theta and for TeT_{e} \geq 1 K. For θ\theta closer to the magic angle, PP is enhanced by a few hundred times that in MLG due to the great suppression of the Fermi velocity vF{v_{F}}^{*} leading to the strong el-ap scattering. Consequently, twist angle emerges as an additional important tunable parameter of PP. Although BG regime power law PTe4P\sim{T_{e}}^{4} is obeyed in low TeT_{e} region, PP vs TeT_{e} behavior still remains super linear at higher TeT_{e} where acoustic phonon limited resistivity ρp\rho_{p} is linear-in-temperature. For a given nsn_{s}, although TBGT_{BG} is independent of θ\theta, the range of TeT_{e} in which PTe4P\sim{T_{e}}^{4} is obeyed increases marginally with increasing θ\theta. The energy relaxation time τe\tau_{e}, is found to be smaller by an order of magnitude than in MLG and decreasing with increasing TeT_{e}. As θ\theta approaches θm\theta_{m} the τe\tau_{e} decreases significantly indicating that θ\theta can be used as an important parameter to tune τe\tau_{e} also. Finally, simple and useful relations of PP with μp\mu_{p} and ρp\rho_{p} are obtained in the BG regime. From the relation between PP and ρp\rho_{p}, using our calculated PP, the estimated value is closer to the ρp\rho_{p} of Wu et al Wu et al. (2019). Experimental observations may test the validity of our predictions.

References