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Control the qubit-qubit coupling in the superconducting circuit with double-resonator couplers

Hui Wang [email protected] Shandong Inspur Intelligence Research Institute Co., Ltd., Jinan, China Shandong Yunhai Guochuang Innovative Technology Co., Ltd, Jinan, China    Yan-Jun Zhao zhao˙[email protected] Key Laboratory of Opto-electronic Technology, Ministry of Education, Beijing University of Technology, Beijing, China    Hui-Chen Sun Institute for Quantum Computing and Department of Physics and Astronomy, University of Waterloo, Waterloo, Ontario N2L 3G1, Canada    Xun-Wei Xu Key Laboratory of Low-Dimensional Quantum Structures and Quantum Control of Ministry of Education, Key Laboratory for Matter Microstructure and Function of Hunan Province, Department of Physics and Synergetic Innovation Center for Quantum Effects and Applications, Hunan Normal University, Changsha 410081, China    Yong Li Shandong Inspur Intelligence Research Institute Co., Ltd., Jinan, China Shandong Yunhai Guochuang Innovative Technology Co., Ltd    Yarui Zheng [email protected] Quantum Element Technology (Shen Zhen) Co.,Ltd., Shenzhen 518048, China    Qiang Liu Shandong Inspur Intelligence Research Institute Co., Ltd., Jinan, China Shandong Yunhai Guochuang Innovative Technology Co., Ltd    Rengang Li Shandong Inspur Intelligence Research Institute Co., Ltd., Jinan, China
Abstract

We propose a theoretical scheme of using two-fixed frequency resonator couplers to tune the interaction between two Xmon qubits. The indirect interaction between two qubits induced by two resonators can cancel each other, so the direct qubit-qubit coupling is not essential for the switching off. So we can suppress the static ZZ coupling with the weak direct qubit-qubit coupling and even eliminate the static ZZ coupling through the destructive interferences of the double-path couplers. The cross-kerr resonance can induce additional poles for the static ZZ coupling which should be kept away during the two-qubit gates. The double-resonator couplers scheme could unfreeze some restrictions during the design of superconducting quantum chips and mitigate the static ZZ coupling, which might supply a promising platform for future superconducting quantum chip.

I Introduction

In past several years, the superconducting quantum computing develops quickly, IBM announced 433 qubits superconducting quantum chip at the end of 2022, and plan to launch quantum chip with more than 1000 qubits in 2023. The coherence time of superconducting qubits fabricated with new superconducting materials is greatly enhanced[1, 2, 3, 4, 5], and the introduction of tunable coupler greatly enhances the fidelities of two-qubit gates to above 99.5%99.5\% [6, 7, 8, 9, 12, 10, 11]. The quantum supremacy of random circuit sampling and other multi-body quantum simulation experiments have been conducted on the superconducting quantum chip with more than 50 qubits [14, 15, 13, 4]. But the fidelities of two-qubit gate are still not high enough for the universal quantum computer, and the state leakages and residual coupling are still need to be suppressed in superconducting qunatum chip.

The tunable coupler can switch off the interactions between adjacent qubits, which can isolate qubits from the surrounding environments for local quantum operations. In the single-coupler circuit, the induced indirect qubit-qubit coupling (dispersive type interaction) can not be zero for finite frequency detuning between qubit and coupler, so the direct qubit-qubit interaction is required for switching off. If the direct qubit-qubit coupling is very weak, the switching off frequency should be very high, and this leaves narrow available frequency ranges for readout resonators (or qubits). For the case of strong direct qubit-qubit coupling, the state leakages and crosstalks should be another perplex[6, 7, 8]. So there are many limitations during the design of single-coupler superconducting quantum chip, and the residual coupling and state leakages are still serious troubles[16].

In this article, we propose a theoretical scheme to dynamically tune the qubit-qubit coupling with the double-resonator couplers in the superconducting quantum chip. As theoretically and experimentally demonstrated, the superconducting resonator can function as a coupler[17, 20, 18, 19, 22, 21]. In particular, if the two resonator couplers take the respective maximal and minimal frequencies, the induced indirect qubit-qubit coupling by two resonators are in opposite signs and can cancel each other. So the direct qubit-qubit couplings is not indispensable for switching off in the double-resonator coupler circuit, which can hopefully unfreeze some restrictions on the superconducting quantum chip, such as the qubit-qubit coupling strengths, maximal frequencies of couplers, and so on. The switching off positions can be very close to two-qubit gate regimes in the double-resonator couplers circuit, thus the maximal frequencies of couplers can be smaller. So available frequency ranges for readout resonators or qubits can be wider in double-path coupler circuit, and this should relieve the frequency crowding on the superconducting quantum chip.

We also study the effects of superconducting artificial atom’s high-excited states on qubits’ energy levels and switching off positions. The elimination of the static ZZ coupling through the destructive interferences of double-path couplers are also explored[23, 24, 12, 25]. We find that the cross-kerr resonances through the virtual photon exchange could induce new poles of the static ZZ coupling, which should be kept away from during the two-qubit gates.

The paper is organized as follows: In Sec. II, we first perform Numerical calculation of the circuit energy levels. In Sec. III, we then discuss the Switching off for the qubit-qubit coupling. In Sec. IV, we further study the suppression and cancellation of Static ZZ coupling. Finally, we summarize the results in Sec. V.

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Figure 1: (Color online) (a) Schematic diagram. The double-resonator couplers superconducting circuit consists of two Xmon qubits coupling to two common fixed-frequency resonators. (b) The equivalent circuit. The ωη\omega_{\eta} is the frequency of a qubit or resonator, with η=a,b,x,y\eta=a,b,x,y. The inductive type coupling is neglected, and there are only capacitive type interactions in the superconducting circuit. CηC_{\eta} is the capacitances of a qubit or resonator, and the two-body relative capacitance is CηηC_{\eta\eta^{\prime}}, with Cηη=CηηC_{\eta\eta^{\prime}}=C_{\eta^{\prime}\eta} and ηη\eta\neq\eta^{\prime}. LaL_{a} and LbL_{b} are the respective inductances of resonators a and b, while Φe,x\Phi_{e,x} and Φe,y\Phi_{e,y} are the external magnetic fluxes applying on the superconducting loops of qubits x and y, respectively.

II Circuit Energy levels

In this section, we numerically calculate the energy levels of qubits for the superconducting circuit in Fig. 1 with the QuTiP software [26, 27, 28, 16]. The superconducting circuit consists of two Xmon qubits coupling to two common resonator couplers. The two-body interactions are all assumed as capacitive type, and the direct qubit-qubit and resonator-resonator interactions are very weak. The two-body interactions in the superconducting circuit are all assumed as capacitive type. Because of the small anharmonicities, the high-excited states of superconducting artificial atoms should also make contributions to the energy levels of qubits and couplers. Truncated to the second-excited states of atoms and third-excited states of resonators, the curved surfaces of qubits and resonators’ energy levels are plotted in Appendix A (see Fig. 10).

For simplicity, we focus on the special case that the resonant frequency ωa\omega_{a} of resonator a, resonant frequency ωb\omega_{b} of resonator b , and the transition frequency ωx\omega_{x} of qubit x are fixed, and only the transition frequency ωy\omega_{y} for qubit y is tuned by the external magnetic flux Φe,y\Phi_{e,y}. By setting ωx/(2π)=4.56\omega_{x}/(2\pi)=4.56 GHz, the energy level curves of qubits and resonators’ single and double-excited states are plotted in Figs.2(a) and 2(b), respectively. During the numerical calculations with QuTiP software , the transition frequencies of qubit x and qubit y are respectively chosen as ωx/(2π)=4.56\omega_{x}/(2\pi)=4.56 GHz and ωy/(2π)=5.12\omega_{y}/(2\pi)=5.12 GHz, the resonant frequencies of resonator a and resonator b are ωa/(2π)=4.10\omega_{a}/(2\pi)=4.10 GHz and ωb/(2π)=5.20\omega_{b}/(2\pi)=5.20 GHz, respectively. The coupling strengths between resonator a (or b) and two qubits are gax/(2π)=gay/(2π)=32g_{ax}/(2\pi)=g_{ay}/(2\pi)=32 MHz (or gbx/(2π)=gby/(2π)=30g_{bx}/(2\pi)=g_{by}/(2\pi)=30 MHz), so the qubits and couplers are in the dispersive coupling regimes.

The ket vector of four-body quantum state is defined as |mamxmymb|m_{a}m_{x}m_{y}m_{b}\rangle, and the values of ma,mx,my,mbm_{a},m_{x},m_{y},m_{b} respectively describe quantum numbers of resonator a, qubit x, qubit y, and resonator b. Because of the avoided crossing effect, each curve in Fig. 2 can not describe the whole energy level of a certain quantum state, here we mark each curve with the corresponding state at the zero magnetic flux. In Fig.2(a), the transition frequency of qubit y decreases under magnetic field, and it becomes anticrossing with qubit x at the frequency regimes close to 4.56 GHz and with resonator a at the regimes close to 4.10 GHz. For the double-excited states, the energy levels and avoided crossing gaps can be seen in Fig. 2(b). The energy level structure in Fig.2 is important for analyzing the switching off and the static ZZ coupling on the superconducting quantum chip as shown in the follow sections.

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Figure 2: (Color online) The energy level diagram. The energy level curves for (a) single and (b) double-excited states, here we set the transition frequency of qubit x as ωx/2π=4.56\omega_{x}/2\pi=4.56 GHz. The maximal frequencies of qubits x and y are respective ωx(max)/2π=4.56\omega^{(max)}_{x}/2\pi=4.56 GHz and ωy(max)/2π=5.12\omega^{(max)}_{y}/2\pi=5.12 GHz, their corresponding anharmonicities are αx/2π=175\alpha_{x}/2\pi=-175 MHz and αy/2π=195\alpha_{y}/2\pi=-195 MHz. The resonant frequencies of resonators a and b are ωa/2π=4.10\omega_{a}/2\pi=4.10 GHz and ωb/2π=5.20\omega_{b}/2\pi=5.20 GHz, respectively. The direct qubit-qubit and direct resonator-resonator coupling strengths are gxy/2π=1.0g_{xy}/2\pi=1.0 MHz and the gab/2π=0.1g_{ab}/2\pi=0.1 MHz, respectively. The coupling strengths of qubits with resonator a are gax/2π=gay/2π=32g_{ax}/2\pi=g_{ay}/2\pi=32 MHz, and gbx/2π=gby/2π=30g_{bx}/2\pi=g_{by}/2\pi=30 MHz label the coupling strengths of qubits with resonator b.

III switching off

III.1 Circuit Quantization

Figure 1(a) describes the superconducting circuit consisting of two Xmon qubits coupling to two common fixed frequency resonators, the frequencies of qubits are tunable. Besides the direct interactions, the qubit-resonator couplings can also induce indirect qubit-qubit and resonator-resonator interactions. The resonant frequencies of resonators a and b are respective ωa\omega_{a} and ωb\omega_{b}, while ωx\omega_{x} and ωy\omega_{y} label the transition frequencies of qubits x and y, respectively. In the case of zero magnetic fluxes, the frequencies of qubits and resonators satisfy ωa<ωx<ωy<ωb\omega_{a}<\omega_{x}<\omega_{y}<\omega_{b}. We expect a large distance between two resonators and neglect their inductive coupling, then the interactions are all regarded as capacitive type as shown in Fig. 1(b). The capacitances of resonators should be distributed type and proportional to their lengths, but in the article we simply label the total capacitances of resonators a and b as CaC_{a} and CbC_{b}, respectively.

Inspired by previous work[17, 20], the kinetic energy of superconducting circuit with double-resonator couplers can be written as T=η=a,b,x,yCηϕ˙η2/2+η,η=a,b,x,yηηCηη(ϕ˙ηϕ˙η)2/4T=\sum_{\eta=a,b,x,y}C_{\eta}\dot{\phi}^{2}_{\eta}/2+\sum_{\eta,\eta^{\prime}=a,b,x,y\atop\eta\neq\eta^{\prime}}C_{\eta\eta^{\prime}}\left(\dot{\phi}_{\eta}-\dot{\phi}_{\eta^{\prime}}\right)^{2}/4, where CηC_{\eta} is the capacitance of qubit or resonator, and CηηC_{\eta\eta^{\prime}} (Cηη=CηηC_{\eta\eta^{\prime}}=C_{\eta^{\prime}\eta}) is relative capacitance between arbitrary two devices among qubits and resonators, with η,η=a,b,x,y\eta,\eta^{\prime}=a,b,x,y and ηη\eta\neq\eta^{\prime}. The ϕa\phi_{a} and ϕb\phi_{b} are the respective magnetic fluxes of circuit nodes for resonators a and b, while ϕx\phi_{x} and ϕy\phi_{y} are the respective node fluxes of qubits x and y, and they can be tuned by the external magnetic fluxes Φe,x\Phi_{e,x} and Φe,y\Phi_{e,y}[29, 30, 31]. If we label the LaL_{a} and LbL_{b} as the respective inductances of resonators a and b, thus the potential energy of superconducting circuit can be written as U=λ=a,bϕλ2/(2Lλ)+β=x,yEJβ[1cos(2πϕβ/Φ0)]U=\sum_{\lambda=a,b}\phi^{2}_{\lambda}/(2L_{\lambda})+\sum_{\beta=x,y}E_{J_{\beta}}\left[1-\cos\left(2\pi\phi_{\beta}/\Phi_{0}\right)\right], the subscript λ=a,b\lambda=a,b label the respective variables of resonators a and b, while β=x,y\beta=x,y describe the variables of qubit x and qubit y, respectively. The EJβ=IcβΦ0/(2π)E_{J_{\beta}}=I_{c\beta}\Phi_{0}/(2\pi) is the Josephson energy of qubit β\beta, where the IcβI_{c\beta} is the corresponding critical current, and Φ0=h/2e\Phi_{0}=h/2e is the flux quantum with the planck constant h and an electron charge e.

With the kinetic energy TT and potential energy UU, the Lagrangian of the superconducting circuit in Fig. 1 can be formally written as L=TUL=T-U. If we define the generalized momentum operators as qη=L/ϕ˙η=Cϕ˙ηq_{\eta}=\partial L/\partial\dot{\phi}_{\eta}=C\dot{\phi}_{\eta} (with η=a,b,x,y\eta=a,b,x,y), under the conditions CabCxyCax,Cay,Cbx,CbyCx,CyCa,CbC_{ab}\ll C_{xy}\ll C_{ax},C_{ay},C_{bx},C_{by}\ll C_{x},C_{y}\ll C_{a},C_{b}, we obtain the expression of Hamiltonian (see Appendix B)

H\displaystyle H =\displaystyle= 4λ=a,b[ECλ(nλ)2+ϕλ28Lλ]\displaystyle 4\sum_{\lambda=a,b}\left[E_{C_{\lambda}}(n_{\lambda})^{2}+\frac{\phi^{2}_{\lambda}}{8L_{\lambda}}\right]
+\displaystyle+ β=x,y[ECβ(nβ)2Ejβcos(2πΦ0ϕβ)]\displaystyle\sum_{\beta=x,y}\left[E_{C_{\beta}}(n_{\beta})^{2}-E_{j\beta}\cos\left(\frac{2\pi}{\Phi_{0}}\phi_{\beta}\right)\right]
+\displaystyle+ 8λ=a,bβ=x,yCλβCλCβECλECβ(nλnβ)\displaystyle 8\sum_{\lambda=a,b\atop\beta=x,y}\frac{C_{\lambda\beta}}{\sqrt{C_{\lambda}C_{\beta}}}\sqrt{E_{C_{\lambda}}E_{C_{\beta}}}(n_{\lambda}n_{\beta})
+\displaystyle+ 8(1+CaxCbxCxCab+CayCbyCyCab)CabCaCbECaECb(nanb)\displaystyle 8\left(1+\frac{C_{ax}C_{bx}}{C_{x}C_{ab}}+\frac{C_{ay}C_{by}}{C_{y}C_{ab}}\right)\frac{C_{ab}}{\sqrt{C_{a}C_{b}}}\sqrt{E_{C_{a}}E_{C_{b}}}(n_{a}n_{b})
+\displaystyle+ 8(1+CaxCayCaCxy+CbxCbyCbCxy)CxyCxCyECxECy(nxny),\displaystyle 8\left(1+\frac{C_{ax}C_{ay}}{C_{a}C_{xy}}+\frac{C_{bx}C_{by}}{C_{b}C_{xy}}\right)\frac{C_{xy}}{\sqrt{C_{x}C_{y}}}\sqrt{E_{C_{x}}E_{C_{y}}}(n_{x}n_{y}),

where nη=qη/2en_{\eta}=q_{\eta}/2e is the Cooper-pair number operator of a qubit or resonator, and the corresponding charging energy is ECη=e2/2CηE_{C_{\eta}}=e^{2}/2C_{\eta}. The transition frequencies of resonators and qubits are respectively defined as ωλ=1/CλLλ\omega_{\lambda}=1/\sqrt{C_{\lambda}L_{\lambda}} and ωβ=(8EJβECβECβ)/\omega_{\beta}=(\sqrt{8E_{J_{\beta}}E_{C_{\beta}}}-E_{C_{\beta}})/\hbar, while αβ=ECβ/\alpha_{\beta}=-E_{C_{\beta}}/\hbar labels the anharmonicity of qubit β\beta. As shown in Appendix B, the two-body coupling strengths among qubits and resonators can be defined as

gλβ\displaystyle g_{\lambda\beta} =\displaystyle= 12CλβCλCβωλωβ,\displaystyle\frac{1}{2}\frac{C_{\lambda\beta}}{\sqrt{C_{\lambda}C_{\beta}}}\sqrt{\omega_{\lambda}\omega_{\beta}}, (2)
gab\displaystyle g_{ab} =\displaystyle= 12(1+CaxCbxCxCab+CayCbyCyCab)CabCaCbωaωb,\displaystyle\frac{1}{2}\left(1+\frac{C_{ax}C_{bx}}{C_{x}C_{ab}}+\frac{C_{ay}C_{by}}{C_{y}C_{ab}}\right)\frac{C_{ab}}{\sqrt{C_{a}C_{b}}}\sqrt{\omega_{a}\omega_{b}},\quad (3)
gxy\displaystyle g_{xy} =\displaystyle= 12(1+CaxCayCaCxy+CbxCbyCbCxy)CxyCxCyωxωy.\displaystyle\frac{1}{2}\left(1+\frac{C_{ax}C_{ay}}{C_{a}C_{xy}}+\frac{C_{bx}C_{by}}{C_{b}C_{xy}}\right)\frac{C_{xy}}{\sqrt{C_{x}C_{y}}}\sqrt{\omega_{x}\omega_{y}}. (4)

The two-body interactions are mainly decided by their relative capacitances CηηC_{\eta\eta^{\prime}} with η,η=a,b,x,y\eta,\eta^{\prime}=a,b,x,y and ηη\eta\neq\eta^{\prime}. The qubit-resonator coupling strength gλβg_{\lambda\beta} in Eq.(2) could induce indirect interaction between two qubits, so the Eq. (4) can not describe the complete interaction between two qubits. In the single-coupler superconducting quantum chip, there are many restrictions on the capacitances and frequencies of qubits (or couplers), but these limitations might be unfrozen in the double-coupler circuit as will be discussed in the follow sections.

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Figure 3: (Color online) The decoupled qubit-qubit coupling strengths. The curved surfaces of gxy(d)g^{(d)}_{xy} are plotted in (a) gxy/2π=3g_{xy}/2\pi=3 MHz and (c) gxy/2π=0g_{xy}/2\pi=0 Hz, while (b) and (d) describe the corresponding decoupled frequencies of qubits along the diagonal line direction in the ϕx\phi_{x}-ϕy\phi_{y} plane. The other parameters are the same as in Fig.2.

III.2 Effective coupling

To get the effective qubit-qubit coupling, we try to decouple the qubit-resonator interactions in this section. For the Xmon qubit, the Josephson energy is much larger than its charging energy, EJβ/ECβ1E_{J_{\beta}}/E_{C_{\beta}}\gg 1, and then the ϕβ\phi_{\beta} should be very small and we can use the approximate equation: cos(ϕβ)=1ϕβ2/2+ϕβ4/24\cos(\phi_{\beta})=1-\phi^{2}_{\beta}/2+\phi^{4}_{\beta}/24-.... If we introduce the creation and annihilation operators by the definitions ϕβ=2EC/EJβ4(aβ+aβ)\phi_{\beta}=\sqrt[4]{2E_{C}/E_{J_{\beta}}}(a^{\dagger}_{\beta}+a_{\beta}), and nβ=(i/2)2EC/EJβ4(aβaβ)n_{\beta}=(i/2)\sqrt[4]{2E_{C}/E_{J_{\beta}}}(a^{\dagger}_{\beta}-a_{\beta}), the second-quantization Hamiltonian can be obtained as H=λ=a,bHλ+β=x,yHβ+λ=a,bβ=x,yHλβ+Hab+HxyH=\sum_{\lambda=a,b}{H_{\lambda}}+\sum_{\beta=x,y}{H_{\beta}}+\sum_{\lambda=a,b\atop\beta=x,y}H_{\lambda\beta}+H_{ab}+H_{xy}, with

Hλ/\displaystyle H_{\lambda}/\hbar =\displaystyle= ωλ2cλcλ,\displaystyle\frac{\omega_{\lambda}}{2}c^{\dagger}_{\lambda}c_{\lambda}, (5)
Hβ/\displaystyle H_{\beta}/\hbar =\displaystyle= ωβ2aβaβ+αβ2aβaβaβaβ,\displaystyle\frac{\omega_{\beta}}{2}a^{\dagger}_{\beta}a_{\beta}+\frac{\alpha_{\beta}}{2}a^{\dagger}_{\beta}a^{\dagger}_{\beta}a_{\beta}a_{\beta}, (6)
Hλβ/\displaystyle H_{\lambda\beta}/\hbar =\displaystyle= gλβ(cλaβ+cλaβcλaβcλaβ),\displaystyle g_{\lambda\beta}(c^{\dagger}_{\lambda}a_{\beta}+c_{\lambda}a^{\dagger}_{\beta}-c^{\dagger}_{\lambda}a^{\dagger}_{\beta}-c_{\lambda}a_{\beta}), (7)
Hab/\displaystyle H_{ab}/\hbar =\displaystyle= gab(cacb+cacbcacbcacb),\displaystyle g_{ab}(c^{\dagger}_{a}c_{b}+c_{a}c^{\dagger}_{b}-c^{\dagger}_{a}c^{\dagger}_{b}-c_{a}c_{b}), (8)
Hxy/\displaystyle H_{xy}/\hbar =\displaystyle= gxy(axay+axayaxayaxay).\displaystyle g_{xy}(a^{\dagger}_{x}a_{y}+a_{x}a^{\dagger}_{y}-a^{\dagger}_{x}a^{\dagger}_{y}-a_{x}a_{y}). (9)

We define αβ=ECβ/\alpha_{\beta}=-E_{C_{\beta}}/\hbar to describe anharmonicity of qubit β\beta, and the nonlinear term (αβ/2)aβaβaβaβ(\alpha_{\beta}/2)a^{\dagger}_{\beta}a^{\dagger}_{\beta}a_{\beta}a_{\beta} reflects the effects of high-excited states of superconducting artificial atom. We define the Δλβ=ωβωλ\Delta_{\lambda\beta}=\omega_{\beta}-\omega_{\lambda} to describe the frequency detuning between the qubit β\beta and resonator λ\lambda, while Σλβ=ωβ+ωλ\Sigma_{\lambda\beta}=\omega_{\beta}+\omega_{\lambda} is the frequency summation of qubit β\beta and resonator λ\lambda. Δxy=ωyωx\Delta_{xy}=\omega_{y}-\omega_{x} describes the frequency detuning between two qubits, and Δab=ωbωa\Delta_{ab}=\omega_{b}-\omega_{a} labels the frequency detuning between two resonators.

Separating the Hamiltonian as H=H0+HintH=H_{0}+H_{int}, the free term is defined as H0=λ=a,bHλ+β=x,yHβH_{0}=\sum_{\lambda=a,b}H_{\lambda}+\sum_{\beta=x,y}H_{\beta}, while the interaction term is Hint=Hab+Hxy+λ=a,bβ=x,yHλβH_{int}=H_{ab}+H_{xy}+\sum_{\lambda=a,b\atop\beta=x,y}H_{\lambda\beta}. In the qubit-resonator dispersive coupling regimes gλβ/|Δλβ|1g_{\lambda\beta}/|\Delta_{\lambda\beta}|\ll 1 and gλβ/Σλβ1g_{\lambda\beta}/\Sigma_{\lambda\beta}\ll 1, we define S=λ=a,bβ=x,y[(gλβ/Δλβ)(cλaβcλaβ)(gλβ/Σλβ)(cλaβcλaβ)]S=\sum_{\lambda=a,b\atop\beta=x,y}[(g_{\lambda\beta}/\Delta_{\lambda\beta})(c^{\dagger}_{\lambda}a_{\beta}-c_{\lambda}a^{\dagger}_{\beta})-(g_{\lambda\beta}/\Sigma_{\lambda\beta})(c^{\dagger}_{\lambda}a^{\dagger}_{\beta}-c_{\lambda}a_{\beta})]. Under the Schrieffer–Wolff transformation, if we choose H(d)=exp(S)Hexp(S)H^{(d)}=\exp{(S)}H\exp{(-S)} and Hint+[S,H0]=0H_{int}+[S,H_{0}]=0, thus the decoupled Hamiltonian becomes H(d)=H0(1/2)[Hint,S]+O(Hint3)H^{(d)}=H_{0}-(1/2)[H_{int},S]+O(H_{int}^{3}) (see Appendix C), that is

H(d)\displaystyle\frac{H^{(d)}}{\hbar} =\displaystyle= λ=a,bωλ(d)cλcλ+β=x,y(ωβ(d)aβaβ+α~β2aβaβaβaβ)\displaystyle\sum_{\lambda=a,b}\omega^{(d)}_{\lambda}c^{\dagger}_{\lambda}c_{\lambda}+\sum_{\beta=x,y}\left(\omega^{(d)}_{\beta}a^{\dagger}_{\beta}a_{\beta}+\frac{\tilde{\alpha}_{\beta}}{2}a^{\dagger}_{\beta}a^{\dagger}_{\beta}a_{\beta}a_{\beta}\right) (10)
+\displaystyle+ gxy(d)(axay+ayax)+gab(d)(cacb+cbca).\displaystyle g^{(d)}_{xy}(a^{\dagger}_{x}a_{y}+a^{\dagger}_{y}a_{x})+g^{(d)}_{ab}(c^{\dagger}_{a}c_{b}+c^{\dagger}_{b}c_{a}).

Since gab,gxygλβg_{ab},g_{xy}\ll g_{\lambda\beta}, the contributions of HabH_{ab} and HxyH_{xy} have been neglected. Following the method of previous work[7], we assumed α~βαβ\tilde{\alpha}_{\beta}\approx\alpha_{\beta} during the derivations of Eq.(10), thus the contributions of superconducting artificial atoms’ high-excited states are neglected.

The decoupled frequencies of qubits and resonators can be respectively defined as ωβ(d)=ωβ+λ=a,b(gλβ2/Δλβgλβ2/Σλβ)\omega^{(d)}_{\beta}=\omega_{\beta}+\sum_{\lambda=a,b}(g^{2}_{\lambda\beta}/\Delta_{\lambda\beta}-g^{2}_{\lambda\beta}/\Sigma_{\lambda\beta}) and ωλ(d)=ωλβ=x,y(gλβ2/Δλβgλx2/Σλβ)\omega^{(d)}_{\lambda}=\omega_{\lambda}-\sum_{\beta=x,y}(g^{2}_{\lambda\beta}/\Delta_{\lambda\beta}-g^{2}_{\lambda x}/\Sigma_{\lambda\beta}) (as shown in Appendix C,). And the decoupled qubit-qubit coupling strength can be obtained as

gxy(d)\displaystyle g^{(d)}_{xy} =\displaystyle= 12λ=a,bβ=x,y(gλxgλyΔλβgλxgλyΣλβ)+gxy.\displaystyle\frac{1}{2}\sum_{\lambda=a,b\atop\beta=x,y}\left(\frac{g_{\lambda x}g_{\lambda y}}{\Delta_{\lambda\beta}}-\frac{g_{\lambda x}g_{\lambda y}}{\Sigma_{\lambda\beta}}\right)+g_{xy}. (11)

Since Δλβ\Delta_{\lambda\beta} and Σλβ\Sigma_{\lambda\beta} depend the frequency of qubit β\beta, so the induced qubit-qubit coupling gλ,xy(in)=(1/2)β=x,y(gλxgλy/Δλβgλxgλy/Σλβ)g^{(in)}_{\lambda,xy}=(1/2)\sum_{\atop\beta=x,y}(g_{\lambda x}g_{\lambda y}/\Delta_{\lambda\beta}-g_{\lambda x}g_{\lambda y}/\Sigma_{\lambda\beta}) can be tuned by the external magnetic fluxes Φe,x\Phi_{e,x} and Φe,y\Phi_{e,y}. To switch off the qubit-qubit coupling (gxy(d)/(2π)=0g^{(d)}_{xy}/(2\pi)=0 Hz), we should find parameters to satisfy gxy(in)=gxy-g^{(in)}_{xy}=g_{xy}.

From the expression of gλ,xy(in)g^{(in)}_{\lambda,xy}, both two resonators make contributions to the effective qubit-qubit coupling, and their contributions might cancel each other (ga,xy(in)+gb,xy(in)=0g^{(in)}_{a,xy}+g^{(in)}_{b,xy}=0) if the qubit frequency of qubits satisfy certain conditions. Thus the direct qubit-qubit coupling might be not necessary for the switching off in the double-resonator couplers circuit. The qubits could also induce indirect interactions between the two resonators, and the decoupled resonator-resonator coupling strength can be defined as gab(d)=(1/2)λ=a,bβ=x,y(gaβgbβ/Δλβgaβgbβ/Σλβ)+gabg^{(d)}_{ab}=(1/2)\sum_{\lambda=a,b\atop\beta=x,y}\left(g_{a\beta}g_{b\beta}/\Delta_{\lambda\beta}-g_{a\beta}g_{b\beta}/\Sigma_{\lambda\beta}\right)+g_{ab} (see Appendix C). Because of the large frequency detuning between two resonators (|Δab|gab(d)|\Delta_{ab}|\gg g^{(d)}_{ab}), the effective resonator-resonator interaction makes little effect on the energy levels of qubits and resonators.

With the parameters in Fig. 2, we can get gby/min(|Δby|)1/3g_{by}/\min{(|\Delta_{by}|)}\sim 1/3 and gax/min(|Δax|)1/15g_{ax}/\min{(|\Delta_{ax}|)}\sim 1/15 in the idling states of qubits (without external magnetic field). This means that the qubits and resonators are in the dispersive or weak-dispersive coupling regimes, thus the perturbation method can be used to calculate the effective qubit-qubit coupling . If we choose ωa<ωx<ωy<ωb\omega_{a}<\omega_{x}<\omega_{y}<\omega_{b}, the signs of Δaβ\Delta_{a\beta} and Δbβ\Delta_{b\beta} are opposite. As indicated by gλ,xy(in)g^{(in)}_{\lambda,xy}, the resonator b will induce negative indirect qubit-qubit coupling, and the contributions of resonators a is positive. With Eq. (11), the curved surfaces of gxy(d)g^{(d)}_{xy} are plotted in Figs. 3(a) and 3(c), and the corresponding decoupled frequencies of qubits are shown in Figs. 3(b) and 3(d). The curved surface of gxy(d)g^{(d)}_{xy} has many crossing points with the zero value plane (gxy(d)/(2π)=0g^{(d)}_{xy}/(2\pi)=0 Hz) in Fig. 3(a) (gxy/(2π)=3g_{xy}/(2\pi)=3 MHz), which correspond to switch off positions for the qubit-qubit coupling. The multiple switching off points can be used to optimize the quantum operation parameters and reduce the effects of adjoint qubits. For the case of nonzero direct qubit-qubit coupling (gxy0g_{xy}\neq 0), the distribution of crossing points forms an approximately elliptical curve in ϕx\phi_{x}-ϕy\phi_{y} plane as shown in Fig. 3(a), and this means that the contributions of resonator b to induced qubit-qubit coupling (in amplitudes) is larger than the contributions of resonator a.

In the case of gxy/(2π)=0g_{xy}/(2\pi)=0 Hz, the effective qubit-qubit can also be zero if the indirect qubit-qubit couplings induced by resonators a and b are the same in amplitudes but opposite in signs (ga,xy(in)=gb,xy(in)g^{(in)}_{a,xy}=-g^{(in)}_{b,xy}). As shown in Fig. 3(c), the curved surface of gxy(d)g^{(d)}_{xy} can also cross with the zero values plane (gxy(d)/(2π)=0g^{(d)}_{xy}/(2\pi)=0 Hz) in the case of gxy/(2π)=0g_{xy}/(2\pi)=0 Hz, and this means that the switching off can be realized without the direct qubit-qubit interaction in the double-resonator couplers circuit. The distribution of switching off points approximately forms a circle in ϕx\phi_{x}-ϕy\phi_{y} plane in Fig. 3(c), which indicates the approximate equal contributions (in amplitudes) of two resonators to the effective qubit-qubit couplings. The decoupled frequencies of qubits are plotted in Fig. 3(b) (gxy/(2π)=3g_{xy}/(2\pi)=3 MHz) and Fig. 3(d)(gxy/(2π)=0g_{xy}/(2\pi)=0 Hz), and the effects of direct qubit-qubit coupling to the transition frequencies of qubits seems not very large.

The switching off positions are not totally decided by the direct qubit-qubit coupling in the double-resonator coupler circuit, thus we can take arbitrary small or even zero direct qubit-qubit coupling strength in principally, which might be helpful to suppress the state leakages and crosstalks on the superconducting quantum chips. And the restrictions on the direct qubit-qubit coupling strength and coupler’s frequency can be unfreezed on the double-resonator couplers superconducting quantum chip). If we choose the switching off positions close to two-qubit gate regimes, thus the maximal frequencies of couplers can be smaller, and this might create wider available frequency ranges for the readout resonators and relieve the frequency crowding on the superconducting quantum chip.

III.3 High-excited states corrections

In current theoretical model for tunable coupler circuit, the nonlinear term Hnl,β=(αβ/2)aβaβaβaβH_{nl,\beta}=(\alpha_{\beta}/2)a^{\dagger}_{\beta}a^{\dagger}_{\beta}a_{\beta}a_{\beta} term is regarded as invariant during dynamical decoupling processes for qubit-resonator interactions[7, 16]. This approximation in fact neglects the effects of superconducting artificial atoms’ high-excited states, so the gxy(d)g^{(d)}_{xy} in Eq. (11) does not contain the information of anharmonicity αβ\alpha_{\beta}. Because of the small anharmonicity for Xmon qubit (between 200 MHz and 400 MHz), the interactions between the resonators and high-excited states of superconducting artificial atoms should make corrections to the qubits’ energy levels and effective qubit-qubit coupling.

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Figure 4: (Color online) Corrections by the high-excited states. The black-solid curves in (a) qubit x and (b) qubit y describe the decoupled frequencies ωβ(d)\omega^{(d)}_{\beta}, while the red-dashed curves label the corresponding corrected frequencies ωβ(cr)(=ωβ(d)+Δωβ)\omega^{(cr)}_{\beta}(=\omega^{(d)}_{\beta}+\Delta\omega_{\beta}), and the insert figures show the frequency shifts Δωβ\Delta\omega_{\beta}. The effective qubit-qubit coupling strengths gxy(d)g^{(d)}_{xy} (black-solid curve) and gxy(cr)g^{(cr)}_{xy} (red-dashed curve) are plotted via (c) node phase ϕy\phi_{y} and (d) transition frequency ωy\omega_{y}. Here ωx/2π=4.56\omega_{x}/2\pi=4.56 GHz and gxy/2π=1g_{xy}/2\pi=1 MHz, the other parameters are the same as in Fig.2.

The Bogoliubov transformation has been used to analyze the variations of nonlinear term Hnl,βH_{nl,\beta} during the decoupling processes[40, 39], and the derived self-kerr and cross-kerr resonant terms under the unitary transformation reflect the contributions of superconducting artificial atoms’ high-excited states. To maintain consistency, in this section we continue to use the Schrieffer–Wolff transformation to calculate the effects of the nonlinear term Hnl,βH_{nl,\beta} (see appendix D). In the qubit-resonator dispersive coupling regimes, gλβ/|Δλβ|1g_{\lambda\beta}/|\Delta_{\lambda\beta}|\ll 1 and gλβ/|Σλβ|1g_{\lambda\beta}/|\Sigma_{\lambda\beta}|\ll 1, we define Sλβ=(gλβ/Δλβ)(cλaβcλaβ)(gλβ/Σλβ)(cλaβcλaβ)S_{\lambda\beta}=(g_{\lambda\beta}/\Delta_{\lambda\beta})(c^{\dagger}_{\lambda}a_{\beta}-c_{\lambda}a^{\dagger}_{\beta})-(g_{\lambda\beta}/\Sigma_{\lambda\beta})(c^{\dagger}_{\lambda}a^{\dagger}_{\beta}-c_{\lambda}a_{\beta}) with S=λ=a,bβ=x,ySλβS=\sum_{\lambda=a,b\atop\beta=x,y}S_{\lambda\beta}. Since Hnl,βH_{nl,\beta} is a small quantity, we will separately conduct the Unitary transform Hnl,β=exp(S)Hnl,βexp(S)H^{\prime}_{nl,\beta}=\exp(S)H_{nl,\beta}\exp(-S) to study its contributions to the high-order effects, such as cross-kerr resonance, self-kerr resonance, and so on[40]. With tedious calculations (see Appendix D), up to the second-order perturbation expansion terms, we get

Hnl,β\displaystyle H^{\prime}_{nl,\beta} \displaystyle\approx λ=a,b(gλβ2αβΣλβ2gλβ2αβΔλβ2)aβaβaβaβ\displaystyle\sum_{\lambda=a,b}\left(\frac{g^{2}_{\lambda\beta}\alpha_{\beta}}{\Sigma^{2}_{\lambda\beta}}-\frac{g^{2}_{\lambda\beta}\alpha_{\beta}}{\Delta^{2}_{\lambda\beta}}\right)a^{\dagger}_{\beta}a^{\dagger}_{\beta}a_{\beta}a_{\beta}
+\displaystyle+ λ=a,b[2gλx2αβΔλβ2cλcλaβaβ+2gλβ2αβΣλβ2cλcλaβaβ].\displaystyle\sum_{\lambda=a,b}\left[\frac{2g^{2}_{\lambda x}\alpha_{\beta}}{\Delta^{2}_{\lambda\beta}}c^{\dagger}_{\lambda}c_{\lambda}a^{\dagger}_{\beta}a_{\beta}+\frac{2g^{2}_{\lambda\beta}\alpha_{\beta}}{\Sigma^{2}_{\lambda\beta}}c_{\lambda}c^{\dagger}_{\lambda}a^{\dagger}_{\beta}a_{\beta}\right].

Since gxy,gabgλβg_{xy},g_{ab}\ll g_{\lambda\beta}, the indirect interaction induced by the weakly direct qubit-qubit and resonator-resonator interactions have been neglected. The first and second lines in the right side of Eq.(12) respectively describe the self-kerr and cross-kerr resonance terms, and the complete calculation results can be seen in Appendix D. There are no external pump fields for resonator couplers, so the cavity photon numbers should be very small (nλ=aλaλ1n_{\lambda}=a^{\dagger}_{\lambda}a_{\lambda}\ll 1). Thus we can get the approximate frequency shift for qubit β{\beta} induced by the nonlinear terms,

Δωβ=λ=a,b(gλβ2Δλβ2+gλβ2Σλβ2)αβ.\displaystyle\Delta\omega_{\beta}=\sum_{\lambda=a,b}\left(\frac{g^{2}_{\lambda\beta}}{\Delta^{2}_{\lambda\beta}}+\frac{g^{2}_{\lambda\beta}}{\Sigma^{2}_{\lambda\beta}}\right)\alpha_{\beta}. (13)

We can see that the frequency shift Δωβ\Delta\omega_{\beta} for qubit β\beta is proportional to the qubit’s anharmonicity αβ\alpha_{\beta}, which reflects the effects of the second-excited state of superconducting artificial atoms. Adding the frequency shift induced by the nonlinear term Hnl,βH_{nl,\beta}, we can approximately get the corrected frequency ωβ(cr)\omega^{(cr)}_{\beta} of qubit β\beta in decoupled coordinate frame

ωβ(cr)\displaystyle\omega^{(cr)}_{\beta} =\displaystyle= ωβ+λ=a,b(gλβ2Δλβgλβ2Σλβ)\displaystyle\omega_{\beta}+\sum_{\lambda=a,b}\left(\frac{g^{2}_{\lambda\beta}}{\Delta_{\lambda\beta}}-\frac{g^{2}_{\lambda\beta}}{\Sigma_{\lambda\beta}}\right)
+λ=a,b(gλβ2Δλβ2+gλβ2Σλβ2)αβ.\displaystyle+\sum_{\lambda=a,b}\left(\frac{g^{2}_{\lambda\beta}}{\Delta^{2}_{\lambda\beta}}+\frac{g^{2}_{\lambda\beta}}{\Sigma^{2}_{\lambda\beta}}\right)\alpha_{\beta}.

The transition frequency of qubit x in decoupled coordinate is plotted in Fig. 4(a), the deviation between ωx(cr)\omega^{(cr)}_{x} and ωx(d)\omega^{(d)}_{x} is larger at the regimes far from the zero magnetic flux points, which coincides with the curve of Δωx\Delta\omega_{x} in insert figure. On the contrary, the maximal deviation between ωy(cr)\omega^{(cr)}_{y} and ωy(d)\omega^{(d)}_{y} appears at the regime close to the zero magnetic flux (Φe,y0\Phi_{e,y}\rightarrow 0 or ϕy0\phi_{y}\rightarrow 0) in Fig. 4(b), this also coincides with the curve of Δωy\Delta\omega_{y} in the insert figure.

If we replace the ωβ(d)\omega^{(d)}_{\beta} with ωβ(cr)\omega^{(cr)}_{\beta} in Eq.(11), we can get the corrected effective qubit-qubit coupling gxy(cr)g^{(cr)}_{xy}. The resonators’ resonant frequencies ωa\omega_{a} and ωb\omega_{b} are fixed in this article, so the effective qubit-qubit coupling are mainly tuned by the qubits’ transition frequencies ωx\omega_{x} and ωy\omega_{y}. By setting ωx/(2π)=4.56\omega_{x}/(2\pi)=4.56 GHz, we plot the curves of effective qubit-qubit coupling gxy(cr)g^{(cr)}_{xy} and gxy(d)g^{(d)}_{xy} on the respective ϕy\phi_{y} and ωy\omega_{y} in Figs. 4(c) and  4(d), the points satisfying gxy(cr)/(2π)=0g^{(cr)}_{xy}/(2\pi)=0 Hz or gxy(d)/(2π)=0g^{(d)}_{xy}/(2\pi)=0 Hz corresponds to the switching off position for the qubit-qubit interaction. The zero value points of gxy(cr)g^{(cr)}_{xy} and gxy(cr)g^{(cr)}_{xy} are different, which reflects the effects of the nonlinear term HnlH_{nl} ( also the second-excited state of superconducting artificial atom) on the switching off positions. The calculation results of the corrections to qubits’ frequencies and effective qubit-qubit coupling strength can help to accurately design the superconducting quantum chip.

III.4 Switching off the qubit-qubit coupling

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Figure 5: (Color online) Switching off the interaction between two qubits. The effects of (a) direct qubit-qubit coupling strengths and (b) qubits’ anharmoncities on the switching off positions. (a) The three types of line styles correspond to different direct qubit-qubit coupling strengths: (1) gxy/2π=0g_{xy}/2\pi=0 Hz for blue-solid curves; (2) gxy/2π=0.5g_{xy}/2\pi=0.5 MHz for black-dashed curves; (3) gxy/2π=1g_{xy}/2\pi=1 MHz red-dotted curves. The ωx/2π=4.56\omega_{x}/2\pi=4.56 GHz for the curves without markers, while ωx/2π=4.53\omega_{x}/2\pi=4.53 GHz for the curves with star markers. (b) The three curves correspond to different anharmonicities: (1) αy/2π=190\alpha_{y}/2\pi=-190 MHz for the blue-solid curve; (2) αy/2π=195\alpha_{y}/2\pi=-195 MHz for the black-dashed curve; (3) αy/2π=200\alpha_{y}/2\pi=-200 MHz for the red-dotted curve. The variation of ωy\omega_{y} on the node phase ϕy\phi_{y} is shown in the insert figure. We choose ωx/2π=4.56\omega_{x}/2\pi=4.56 GHz and gxy/2π=0.5g_{xy}/2\pi=0.5 MHz in (b). The other parameters of (a) and (b) are the same as in Fig.2.

In this section, we study the effects of direct qubit-qubit coupling gxyg_{xy} and qubit’s anharmonicitiy αβ\alpha_{\beta} on the effective qubit-qubit coupling gxy(cr)g^{(cr)}_{xy} and the switching off position. If we take the parameters of Fig. 2, we can get gby/min(|Δby|)1/3g_{by}/\min{(|\Delta_{by}|)}\sim 1/3 and gax/min(|Δax|)1/15g_{ax}/\min{(|\Delta_{ax}|)}\sim 1/15 in the idling states of qubits (without external magnetic field), so the qubits and resonators are in the dispersive or weak-dispersive coupling regimes. To see clearer the working mechanism of switching-off processes in the double-resonator couplers circuit, we plot the one-dimensional curves of effective qubit-qubit coupling gxy(cr)g^{(cr)}_{xy} with the variation of qubit transition frequency ωy\omega_{y} in Fig. 5(a). By fixing ωx/(2π)=4.56\omega_{x}/(2\pi)=4.56 GHz, the three curves without markers in Fig. 5(a) correspond to different direct qubit-qubit coupling strengths: gxy/(2π)=0g_{xy}/(2\pi)=0 Hz in the blue-solid curve, gxy/(2π)=0.5g_{xy}/(2\pi)=0.5 MHz in black-dashed curve, and gxy/(2π)=1g_{xy}/(2\pi)=1 MHz in the red-dotted curve. The crossing points of three curves with zero value line ( gxy(cr)/(2π)=0g^{(cr)}_{xy}/(2\pi)=0 Hz) are different, this means that the direct qubit-qubit coupling could affect the switching off positions. If we set ωx/(2π)=4.53\omega_{x}/(2\pi)=4.53 GHz, the switching off points in the three marked curves show considerable shifts relative to the corresponding same color curves without markers.

In Fig. 5(b), we plot the curves of effective qubit-qubit coupling gxy(cr)g^{(cr)}_{xy} on the node phase ϕy\phi_{y} with ωx/(2π)=4.56\omega_{x}/(2\pi)=4.56 GHz. For the same ranges of node phase ϕy\phi_{y}, the qubit’s maximal frequencies ωy(max)\omega^{(max)}_{y} are not the same for different anharmonicities αy\alpha_{y} as shown in the insert figure. For different anhamonicities αy\alpha_{y}, the shifts of switching off positions on three curves reflect the effects of superconducting artificial atom’s second-excited states.

The frequency of qubit y should be tuned close to ωyωx\omega_{y}\approx\omega_{x} for the iSWAP gate and ωy+αyωx\omega_{y}+\alpha_{y}\approx\omega_{x} for the Controlled-Z gate. For the single-path coupler circuit, the switching off point is usually close to the idling coupler frequency (usually about 6.0 GHz) which is far from the two-qubit gate regimes (usually below 5.0 GHz). In the double-resonator couplers circuit, the switching off positions can be very close to the two-qubit gate regimes as shown in Fig. 5(a). So the maximal frequencies of couplers can be smaller in the double-resonator couplers superconducting circuit, this leaves wider available ranges for readout resonators (or qubits) and might relieve the frequency crowding on superconducting quantum chip.

IV Static ZZ coupling

The tunable coupler could isolate the qubits from surrounding environments for local quantum operations and reduce the accumulated phases for the quantum state preparations, and this can greatly enhance the fidelity of two-qubit gate[9, 12, 10, 11, 14, 15, 13, 4]. Because of the small anharmonicity of the Xmon qubit and the high-order quantum state exchanges (originating from the qubit-qubit and qubit-coupler interactions), the quantum state leakages and the Parasitic crosstalks are still important obstructions for the further enhancement the fidelity of two-qubit gate[16]. Suppressing the residual coupling and the Parasitic crosstalks among neighbour qubits are the leading tasks for enhancing the quality of superconducting quantum chip[17, 32, 33, 34, 35].

The residual ZZ coupling consists the static type ZZ coupling and the dynamic type ZZ coupling, but the dynamic ZZ coupling is usually suppressed by optimizing the microwave pulse shapes and not the interest of this article[16, 34]. In the section, we mainly focus on the Static ZZ coupling which can be mitigated by the designing structures and working parameters of qubits and tunable couplers[23, 17, 25, 24, 32, 33, 12, 34, 35, 36, 37, 38]. In the double-coupler superconducting quantum circuit, the direct qubit-qubit coupling can be arbitrarily small in principally, and this should be helpful for suppressing the static ZZ coupling. And the destructively interferences between double-path couplers might eliminate the static ZZ coupling [23, 24, 12, 25].

IV.1 Analytic calculations

In Figs. 2(a)-2(b), we have numerically calculated the energy level curves of states |0100|0100\rangle, |0010|0010\rangle, and |0110|0110\rangle, in principally the static ZZ coupling can be easily calculated through the definition ξZZ=ω|0110ω|0100ω|0010+ω|0000\xi_{ZZ}=\omega_{|0110\rangle}-\omega_{|0100\rangle}-\omega_{|0010\rangle}+\omega_{|0000\rangle}. In practically, it is difficult to accurately fit the energy level curves of qubits because the avoided crossing gaps are affected by multi-body interactions. By setting ωx/(2π)=4.56\omega_{x}/(2\pi)=4.56 GHz, if we tune the frequency of qubit y to be near resonant with qubit x (ωyωx\omega_{y}\approx\omega_{x}), thus we can get gby/|Δby|gbx/|Δbx|1/20g_{by}/|\Delta_{by}|\approx g_{bx}/|\Delta_{bx}|\sim 1/20 and gax/|Δax|gay/|Δay|1/15g_{ax}/|\Delta_{ax}|\approx g_{ay}/|\Delta_{ay}|\sim 1/15. Thus the qubit-resonator are dispersive coupling regimes, and the perturbation method can be used to analyze the static ZZ coupling close to the two-qubit gate regimes.

For convenience and consistency, we still use ωβ\omega_{\beta} to describe the energy levels of first-excited state of qubit β\beta in this section, and the energy level for second-excited state is 2ωβ+αβ2\omega_{\beta}+\alpha_{\beta}, where the αβ\alpha_{\beta} is the qubit’s anharmoncity . If we temporarily disregard the weak direct qubit-qubit and direct resonator-resonator interactions, up to the fourth-order perturbation theory the effective Hamiltonian on the qubits’ eigenstates space can be obtained as [40, 39]

Hm/=λ=a,bωλcλcλ\displaystyle H^{\prime}_{m}/\hbar=\sum_{\lambda=a,b}\omega_{\lambda}c^{\dagger}_{\lambda}c_{\lambda}
+β=x,yλ=a,bjβ=0,1,2,(ωjβ+κλ,jβ+χλ,jβcλcλ)|jβjβ|\displaystyle+\sum_{\beta=x,y}\sum_{\lambda=a,b\atop j_{\beta}=0,1,2,...}(\omega_{j_{\beta}}+\kappa_{\lambda,j_{\beta}}+\chi_{\lambda,j_{\beta}}c^{\dagger}_{\lambda}c_{\lambda})|j_{\beta}\rangle\langle j_{\beta}|
+β=x,yjβ=0,1,2,[λ=a,bμλ,jβ(cλcλ)2\displaystyle+\sum_{\beta=x,y}\sum_{j_{\beta}=0,1,2,...}\bigg{[}\sum_{\lambda=a,b}\mu_{\lambda,j_{\beta}}(c^{\dagger}_{\lambda}c_{\lambda})^{2}
+νab,jβcacacbcb+νba,jβcbcbcaca]|jβjβ|,\displaystyle+\nu_{ab,j_{\beta}}c^{\dagger}_{a}c_{a}c^{\dagger}_{b}c_{b}+\nu_{ba,j_{\beta}}c^{\dagger}_{b}c_{b}c^{\dagger}_{a}c_{a}\bigg{]}|j_{\beta}\rangle\langle j_{\beta}|, (15)

The ket vector |jβ|j_{\beta}\rangle describes the jβj_{\beta}-th excited state of qubit β\beta, with jβ,jβ=0,1,2,j_{\beta},j^{\prime}_{\beta}=0,1,2,.... We define gλjβjβg^{j_{\beta}j^{\prime}_{\beta}}_{\lambda} as the coupling strength between resonator λ\lambda and the transition |jβ|jβ|j_{\beta}\rangle\leftrightarrow|j^{\prime}_{\beta}\rangle of qubit β\beta. Considering the selection rule, the resonator λ\lambda can only interact with the neighbour quantum states of qubit β\beta: gλjβjβ=0g^{j_{\beta}j^{\prime}_{\beta}}_{\lambda}=0 for jβjβ±1j^{\prime}_{\beta}\neq j_{\beta}\pm 1. In this section, we neglect the small differences for the coupling strengths between resonator λ\lambda and different neighbour state transitions of qubit β\beta , then gλjβ1,jβ=gλjβ,jβ+1=gλβg^{j_{\beta}-1,j_{\beta}}_{\lambda}=g^{j_{\beta},j_{\beta}+1}_{\lambda}=g_{\lambda\beta} ( jβ=1,2,j_{\beta}=1,2,...). Defines χλjβ1,jβ=jβgλβ/[Δλβ+(jβ1)αβ]\chi^{j_{\beta}-1,j_{\beta}}_{\lambda}=j_{\beta}g_{\lambda\beta}/[\Delta_{\lambda\beta}+(j_{\beta}-1)\alpha_{\beta}], the κλ,jβ=χλjβ1,jβ\kappa_{\lambda,j_{\beta}}=\chi^{j_{\beta}-1,j_{\beta}}_{\lambda} describes the level shifts of Lamb type for the quantum state |jβ|j_{\beta}\rangle which is induced by the interaction between resonator λ\lambda and qubit β\beta ( |jβ1|jβ|j_{\beta}-1\rangle\leftrightarrow|j_{\beta}\rangle and |jβ|jβ+1|j_{\beta}\rangle\leftrightarrow|j_{\beta}+1\rangle), while χλ,jβ=χλjβ1,jβχλjβ,jβ+1\chi_{\lambda,j_{\beta}}=\chi^{j_{\beta}-1,j_{\beta}}_{\lambda}-\chi^{j_{\beta},j_{\beta}+1}_{\lambda} describes the corresponding ac-stark type dispersive shifts for the quantum state |jβ|j_{\beta}\rangle (χλ,0β=χ0β,0β+1=gλβ2/(2Δλβ)\chi_{\lambda,0_{\beta}}=-\chi^{0_{\beta},0_{\beta}+1}=-g^{2}_{\lambda\beta}/(2\Delta_{\lambda\beta}))[39, 40]. If we add the contributions of second-excited states of superconducting artificial atoms, besides the self-kerr resonant term μλ,jβ(cλcλ)2\mu_{\lambda,j_{\beta}}(c^{\dagger}_{\lambda}c_{\lambda})^{2}, the cross-kerr resonant terms νab,jβcacacbcb\nu_{ab,j_{\beta}}c^{\dagger}_{a}c_{a}c^{\dagger}_{b}c_{b} and νba,jβcbcbcaca\nu_{ba,j_{\beta}}c^{\dagger}_{b}c_{b}c^{\dagger}_{a}c_{a} should also make contributions to the static ZZ coupling(as will be discussed in follow sections)[39, 40, 41].

If we temporarily disregard the cross-kerr resonant terms, after adding the contributions of weak direct qubit-qubit coupling, and then the static ZZ coupling in qubit-resonator dispersive coupling regimes can be obtained as [8, 17, 16, 25],

ξZZ(2)\displaystyle\xi^{(2)}_{ZZ} =\displaystyle= 2(gxy)2(αx+αy)(Δxy+αy)(Δxyαx),\displaystyle\frac{2(g_{xy})^{2}(\alpha_{x}+\alpha_{y})}{(\Delta_{xy}+\alpha_{y})(\Delta_{xy}-\alpha_{x})}, (16)
ξZZ,λ(3)\displaystyle\xi^{(3)}_{ZZ,\lambda} =\displaystyle= 2gxygλxgλy[1Δλy(1Δxy2Δxy+αy)\displaystyle 2g_{xy}g_{\lambda x}g_{\lambda y}\bigg{[}\frac{1}{\Delta_{\lambda y}}\left(\frac{1}{\Delta_{xy}}-\frac{2}{\Delta_{xy}+\alpha_{y}}\right) (17)
\displaystyle- 1Δλy(1Δxy2Δxyαx)],\displaystyle\frac{1}{\Delta_{\lambda y}}\left(\frac{1}{\Delta_{xy}}-\frac{2}{\Delta_{xy}-\alpha_{x}}\right)\bigg{]},
ξZZ,λ(4s)\displaystyle\xi^{(4s)}_{ZZ,\lambda} =\displaystyle= 2(gλy)2(gλx)2Δλy+Δλxαλ(1Δλy+1Δλx)2\displaystyle\frac{2(g_{\lambda y})^{2}(g_{\lambda x})^{2}}{\Delta_{\lambda y}+\Delta_{\lambda x}-\alpha_{\lambda}}\left(\frac{1}{\Delta_{\lambda y}}+\frac{1}{\Delta_{\lambda x}}\right)^{2} (18)
\displaystyle- (gλy)2(gλx)2Δλy2(1Δxy+1Δλx2Δxyαx)\displaystyle\frac{(g_{\lambda y})^{2}(g_{\lambda x})^{2}}{\Delta^{2}_{\lambda y}}\left(\frac{1}{\Delta_{xy}}+\frac{1}{\Delta_{\lambda x}}-\frac{2}{\Delta_{xy}-\alpha_{x}}\right)
\displaystyle- (gλy)2(gλx)2Δλx2(2Δxy+αy1Δxy+1Δλy).\displaystyle\frac{(g_{\lambda y})^{2}(g_{\lambda x})^{2}}{\Delta^{2}_{\lambda x}}\left(\frac{2}{\Delta_{xy}+\alpha_{y}}-\frac{1}{\Delta_{xy}}+\frac{1}{\Delta_{\lambda y}}\right).\qquad

The ξZZ(2)\xi^{(2)}_{ZZ} is the second-order static ZZ coupling between two qubits, and ξZZ,λ(3)\xi^{(3)}_{ZZ,\lambda} describes the third-order static ZZ coupling between two qubits intermediated by the resonator λ\lambda. We use ξZZ,λ(4s)\xi^{(4s)}_{ZZ,\lambda} to label fourth-order static ZZ coupling contributed by the self-kerr resonance intermediated by the resonator λ\lambda, and the ξZZ,λ(4c)\xi^{(4c)}_{ZZ,\lambda} describe the static ZZ coupling induced by the cross-kerr resonance.

Even being listed together, the second-order ξZZ(2)\xi^{(2)}_{ZZ}, third-order ξZZ(3)=λ=a,bξZZ,λ(3)\xi^{(3)}_{ZZ}=\sum_{\lambda=a,b}\xi^{(3)}_{ZZ,\lambda}, and fourth-order (self-kerr) ξZZ(4s)=λ=a,bξZZ,λ(4s)\xi^{(4s)}_{ZZ}=\sum_{\lambda=a,b}\xi^{(4s)}_{ZZ,\lambda} static ZZ coupling terms come from different sources. As shown in Eqs.(16) and (17), the second-order term ξZZ(2)\xi^{(2)}_{ZZ} originates from the direct qubit-qubit coupling [6, 7, 8, 17], and the fourth-order term ξZZ(4s)\xi^{(4s)}_{ZZ} results from the perturbation expansion of qubit-resonator dispersive coupling[39, 41], while the third-order term ξZZ(3)\xi^{(3)}_{ZZ} is joint effects of direct qubit-qubit coupling and qubit-resonator interaction. Here αλ=β=x,yαβ(gλβ/Δλβ)4\alpha_{\lambda}=\sum_{\beta=x,y}\alpha_{\beta}(g_{\lambda\beta}/\Delta_{\lambda\beta})^{4} describes the nonlinearity of resonator λ\lambda induced by the qubit-resonator dispersive coupling[40]. Since gxy,gabgλβg_{xy},g_{ab}\ll g_{\lambda\beta}, the contributions of direct qubit-qubit and resonator-resonator couplings to fourth-order static ZZ coupling are neglected.

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Figure 6: (Color online) Suppression of the static ZZ coupling. The (a) effective qubit-qubit coupling and (b) static ZZ coupling are plotted for different direct qubit-qubit coupling strengths: (1) gxy/2π=0g_{xy}/2\pi=0 Hz (red-solid curve); (2) gxy/2π=0.5g_{xy}/2\pi=0.5 MHz (blue-dashed curve); (3) gxy/2π=1g_{xy}/2\pi=1 MHz (green-dotted curve); (4) gxy/2π=1.5g_{xy}/2\pi=1.5 MHz (black-dashed-dot curve). The insert figures are the partial enlarged drawing. The ξZZ(2)\xi^{(2)}_{ZZ}, ξZZ(3)(=λ=a,bξZZ,λ(3))\xi^{(3)}_{ZZ}(=\sum_{\lambda=a,b}\xi^{(3)}_{ZZ,\lambda}) and ξZZ(4s)(=λ=a,bξZZ,λ(4s))\xi^{(4s)}_{ZZ}(=\sum_{\lambda=a,b}\xi^{(4s)}_{ZZ,\lambda}) are plotted in (c) and (d), they respectively take the parameters of blue-dashed and black dashed-dot curves in (b). The frequency of qubit x is fixed at ωx/2π=4.52\omega_{x}/2\pi=4.52 GHz, and the other parameters of (a)-(d) are the same as in Fig.2.

IV.2 Suppression of the Static ZZ coupling

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Figure 7: (Color online) Cancellation of the Static ZZ coupling. The effective qubit-qubit coupling and the Static ZZ coupling are respectively plotted in (a) and (b) in the case of ωx/2π=4.0\omega_{x}/2\pi=4.0 GHz, the corresponding result for ωx/2π=3.95\omega_{x}/2\pi=3.95 GHz are shown in (c) and (d). The four curves in each figure of (a)-(d) correspond to different direct qubit-qubit coupling strengths: (1) gxy/2π=0.9g_{xy}/2\pi=0.9 MHz (red-solid curves); (2) gxy/2π=1.0g_{xy}/2\pi=1.0 MHz (blue-dashed curves); (3) gxy/2π=1.2g_{xy}/2\pi=1.2 MHz (green-dotted curves); (4) gxy/2π=1.6g_{xy}/2\pi=1.6 MHz (black dash-dotted curves). The ξZZ(2)\xi^{(2)}_{ZZ}, ξZZ(3)\xi^{(3)}_{ZZ} and ξZZ(4s)\xi^{(4s)}_{ZZ} are plotted in (e) and (f), they respectively take the parameters of blue-dashed and green-dotted curves of (b). The other parameters of (a)-(f) are the same as in Fig.2.

In this section, we try to suppress the Static ZZ coupling with the direct qubit-qubit coupling which can be arbitrary small in the double-coupler superconducting circuit. By setting ωx/(2π)=4.52\omega_{x}/(2\pi)=4.52 GHz, the curves of static ZZ coupling ξZZ=ξZZ(2)+ξZZ(3)+ξZZ(4s)\xi_{ZZ}=\xi^{(2)}_{ZZ}+\xi^{(3)}_{ZZ}+\xi^{(4s)}_{ZZ} are plotted in Fig. 6(b) according to Eqs.(16)-(18). The four curves correspond to different direct qubit-qubit coupling strengths. In the regimes suitable for the two-qubit gates, the values of static ZZ coupling are apparently suppressed by the weaker direct qubit-qubit coupling as shown in the insert figure. And the values of ξZZ(3)\xi^{(3)}_{ZZ} and ξZZ(4s)\xi^{(4s)}_{ZZ} are obviously suppressed by weaker direct qubit-qubit coupling in Fig. 6(c) (gxy/(2π)=0.5g_{xy}/(2\pi)=0.5 MHz) compared with the results in Fig. 6(d) (gxy/(2π)=1.0g_{xy}/(2\pi)=1.0 MHz). As shown in Fig. 6(b)-6(f), the static ZZ coupling can be suppressed below Sub-MHz in double-resonator coupler circuit, which is the similar level with transmon-based coupler circuit[7, 16].

For each static ZZ coupling curve in Fig. 6(b), two poles appear at Δxy=αx\Delta_{xy}=\alpha_{x} and Δxy=αy\Delta_{xy}=-\alpha_{y} which originate from resonant state exchanges between the state |0200|0110|0200\rangle\leftrightarrow|0110\rangle and |0020|0110|0020\rangle\leftrightarrow|0110\rangle, respectively. There is also a pole locating at ωy=ωx\omega_{y}=\omega_{x} in each curve of static ZZ coupling in Fig. 6(b), and the poles also appears in the dashed curves (third-order static ZZ coupling) and dotted curve (fourth-order self-kerr resonance static ZZ coupling) in Figs. 6(c) and  6(d), so it should originate the qubit-qubit resonance state exchanges as indicated by the term 1/Δxy1/\Delta_{xy} containing in Eqs.(17)-(18). As shown in Fig. 6(a), the switching off positions in double-resonator couplers circuit can be below 5 GHz which is very close to the regimes of two-qubit gate. If the frequency of qubit y is tuned away from the switching off positions, the effective qubit-qubit coupling quickly increase to above 5 MHz for the two-qubit gates.

IV.3 Cancellation of the Static ZZ coupling

The nonzero residual coupling leads to unnecessary always-on quantum gates and additional accumulated phases, which are the dominant obstructions for the further enhancement of two-qubit gate fidelities. Recently, some work announce to eliminate the static ZZ coupling in the superconducting quantum chip[25, 35, 36], and it might also be removed in our proposed scheme through the destructive interferences of double-path couplers.

When we tune frequencies of qubit x to satisfy ωx<ωa\omega_{x}<\omega_{a}, and then the static ZZ coupling ξZZ\xi_{ZZ} can be zeroes at some points as shown in Figs. 7(b) and 7(d), thus the static ZZ coupling are eliminated in the double-resonator coupler circuit. The signs of second-order ξZZ(2)\xi^{(2)}_{ZZ}, third-order ξZZ(3)\xi^{(3)}_{ZZ} and fourth-order ξZZ(4s)\xi^{(4s)}_{ZZ} (self-kerr resonance) static ZZ coupling are different in Figs. 7(e) and  7(f), and they cancel each other and eliminate the static ZZ coupling at certain points. It should be mentioned that the pole at ωy=ωx\omega_{y}=\omega_{x} in Figs. 6 do not appear in Figs. 7(b) just because they are outside the scope of drawing.

As shown in Fig. 7(a) (or Fig. 7(c)) and Fig.7(b) (or Fig. 7(d)), the static ZZ coupling are not switched off together with the effective qubit-qubit coupling. This result is not difficult to understand for the perturbation calculation methods[25, 16], because the effective qubit-qubit coupling is calculated only up to the second-order dispersive interaction (ac-Stark/Lamb Shifts), but static ZZ coupling contains some the high-order effects, such as self-kerr resonance, cross-kerr resonance, the high-excited states corrections, and so on. The intervals between zero value positions of static ZZ coupling and effective qubit-qubit coupling change for different direct qubit-qubit coupling strengths, and the black-dash-dotted curves (gxy/(2π)=1.6g_{xy}/(2\pi)=1.6 MHz) get the smallest interval in Figs. 7(a) and 7(b). When we set ωx/(2π)=3.95\omega_{x}/(2\pi)=3.95 GHz, the blue-dashed curves (gxy/(2π)=1.0g_{xy}/(2\pi)=1.0 MHz) get the smallest interval in Figs. 7(c) and 7(d). So the interval between the switching off and zero static ZZ coupling points can be tuned by the direct qubit-qubit coupling and the frequencies of qubits, and it is possible to conduct the switching off and two-qubit gates both at the Zero static ZZ coupling regimes in the double-coupler superconducting circuit.

IV.4 Corrections to Static ZZ coupling

If we incorporate the variations of nonlinear term (αβ/2)aβaβaβaβ(\alpha_{\beta}/2)a^{\dagger}_{\beta}a^{\dagger}_{\beta}a_{\beta}a_{\beta} during the decoupling processes of the qubit-resonator interactions, and then the cross-kerr resonances will contribute to the ZZ coupling[39, 40, 41]. The resonator couplers are not pumped by external fields, the average cavity photon number is much smaller than one, so the single virtual photon exchanges will dominate the cross-kerr resonance processes. The cross-kerr resonance terms νab,jβcacacbcb\nu_{ab,j_{\beta}}c^{\dagger}_{a}c_{a}c^{\dagger}_{b}c_{b} and νba,jβcbcbcaca\nu_{ba,j_{\beta}}c^{\dagger}_{b}c_{b}c^{\dagger}_{a}c_{a} in Eq.(15) describe the physical processes of virtual photon exchange between a qubit and two resonators, we plot the energy-level diagrams of single-virtual photon exchange process of cross-kerr resonance for qubit x in Fig. 8. For simplicity, only three lowest energy levels of superconducting artificial atoms are considered. The virtual photon exchange processes of cross-kerr resonance for qubit y can be obtained by replacing the x with y in Fig. 8 .

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Figure 8: (Color online) Energy-level diagrams of cross-kerr resonances. The virtual photon exchange among qubit x, resonator a, and resonator b with the qubit x initially in (a) the ground state and (b) the first-excited state. The VλxV^{-}_{\lambda x} (or Vλx+V^{+}_{\lambda x}) describe the virtual photon annihilation (or creation) process through the interaction between qubit x and resonator λ\lambda, and Vλx=(Vλx+)V^{-}_{\lambda x}=(V^{+}_{\lambda x})^{\dagger}. The energy-level diagram of cross-kerr resonances for qubit y can be obtained by replacing the qubit x with qubit y.
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Figure 9: (Color online) The static ZZ coupling corrected by the cross-kerr resonances. We plot (a) the effective qubit-qubit coupling and (b) the static ZZ coupling ξZZ(t)=ξZZ(2)+ξZZ(3)+ξZZ(4s)+ξZZ(4c,0)ξZZ(4c,1)\xi^{(t)}_{ZZ}=\xi^{(2)}_{ZZ}+\xi^{(3)}_{ZZ}+\xi^{(4s)}_{ZZ}+\xi^{(4c,0)}_{ZZ}-\xi^{(4c,1)}_{ZZ} at different direct qubit-qubit coupling strengths: (1) gxy/2π=0.2g_{xy}/2\pi=0.2 MHz (red-solid curve); (2) gxy/2π=1.4g_{xy}/2\pi=1.4 MHz (green-dashed curve); (3) gxy/2π=2g_{xy}/2\pi=2 MHz (black-dotted curve). The ξZZ(2)\xi^{(2)}_{ZZ} (red-solid curve), ξZZ(3)=λ=a,bξZZ,λ(3)\xi^{(3)}_{ZZ}=\sum_{\lambda=a,b}\xi^{(3)}_{ZZ,\lambda} (blue-dashed curve), ξZZ(4s)=λ=a,bξZZ,λ(4s)\xi^{(4s)}_{ZZ}=\sum_{\lambda=a,b}\xi^{(4s)}_{ZZ,\lambda} (green-dotted curve), ξZZ(4c,0)=β=x,yξZZ,β(4c,0)\xi^{(4c,0)}_{ZZ}=\sum_{\beta=x,y}\xi^{(4c,0)}_{ZZ,\beta} (black-dashed-dot curve), and ξZZ(4c,1)=β=x,yξZZ,β(4c,1)\xi^{(4c,1)}_{ZZ}=\sum_{\beta=x,y}\xi^{(4c,1)}_{ZZ,\beta} (marked purple-solid curve) are plotted with (c) gxy/2π=0.2g_{xy}/2\pi=0.2 MHz and (d) gxy/2π=1.4g_{xy}/2\pi=1.4 MHz. The parameters of four figures are the same as in Fig.2 except for ωx/2π=4.52\omega_{x}/2\pi=4.52 GHz.

When qubit x is initially in the ground states, the Energy-level diagrams of cross-kerr resonance among qubit x, resonator a, and resonator b are shown in Fig. 8(a). The six cross-kerr resonances are attributed as three types of virtual photon exchange processes among qubit x, resonator a, and resonator b [39]. The first type: the qubit x absorbs a virtual photon from resonator a (or b) and transits to the first-excited states from the ground state, and it immediately returns the virtual photon to resonator a (or b) and decays to the ground state. Subsequently the qubit x jumps to the first-excited state again by getting another virtual photon from resonator b (or a), and finally it emits the virtual photon to resonator b (or a) and decays to the ground state. The second type: the qubit x transits to the first-excited state from the ground state by absorbing a virtual photon from resonator a (or b) and immediately jumps to the second-excited state by taking another virtual photon from resonator b (or a). Subsequently the qubit jumps to the first-excited state by emitting a virtual photon to the resonator b (or a), and finally decays to the ground state by emitting another virtual photon to resonator a (or b). The third type: the first two transition processes are the same as the second type, but the qubit firstly returns a virtual photon to resonator a (or b) in the third transition process and transits to the first-excited state, and finally decays to the ground state by emitting another photon to resonator b (or a). The virtual photon exchange processes for cross-kerr resonances among qubit y, resonator a, and resonator b can be obtained by replacing the qubit x with qubit y in Fig. 8(a). Adding together the contributions of the six type cross-kerr resonant processes, and we can obtain the energy level corrections to the ground state of qubit β\beta [39],

ξZZ,β(4c,0)|0β0β|=gaβ2gbβ2[2ΔaβΔbβωβ\displaystyle\xi^{(4c,0)}_{ZZ,\beta}|0_{\beta}\rangle\langle 0_{\beta}|=g^{2}_{a\beta}g^{2}_{b\beta}\bigg{[}\frac{2}{\Delta_{a\beta}\Delta_{b\beta}\omega_{\beta}} (19)
+12ωβ+αβωaωb(2ωβωaωbΔaβΔbβ)2]|0β0β|.\displaystyle~{}~{}+\frac{1}{2\omega_{\beta}+\alpha_{\beta}-\omega_{a}-\omega_{b}}\bigg{(}\frac{2\omega_{\beta}-\omega_{a}-\omega_{b}}{\Delta_{a\beta}\Delta_{b\beta}}\bigg{)}^{2}\bigg{]}|0_{\beta}\rangle\langle 0_{\beta}|.

For simplicity, we have neglected the small differences on the interactions of a resonator with different energy levels of superconducting artificial atom, that is gλjβ,jβ=gλβg^{j_{\beta},j^{\prime}_{\beta}}_{\lambda}=g_{\lambda\beta}.

When the qubit x is the initially in the first-excited state, the Energy-level diagrams of cross-kerr resonance among qubit x, resonator a, and resonator b are shown in Fig. 8(b). The four cross-kerr resonances are attributed as two types of virtual photon exchange processes. The first type: the qubit x in the first-excited state absorbs a virtual photon from resonator a (or b) and transits to the second-excited state, and it immediately returns the photon to resonator a (or b) and jumps to the first-excited state. Subsequently the qubit jumps to the second-excited state again by getting another virtual photon from resonator b (or a) and finally it emits the photon to resonator b (or a) and jumps to the first-excited state. The second type: the qubit xx (in the first-excited state) emits a virtual photon to resonator a (or b) and decays to the ground state and immediately transits to the first-excited state by absorbing a virtual photon from resonator a (or b). Subsequently the qubit emits a virtual photon to resonator b (or a) and decays to the ground state and immediately absorbs another virtual photon from resonator b (or a) and finally jumps to the first-excited state. The virtual photon exchange processes for cross-kerr resonances among qubit y, resonator a, and resonator b can be obtained by replacing the qubit x with qubit y in Fig. 8(b). Adding together the contributions of the four type cross-kerr resonant processes, and we can obtain the energy level corrections to the first-excited state of qubit β\beta [39],

ξZZ,β(4c,1)|1β1β|\displaystyle\xi^{(4c,1)}_{ZZ,\beta}|1_{\beta}\rangle\langle 1_{\beta}| =\displaystyle= 2gaβ2gbβ2ωβ(Δaβ+αβ)(Δbβ+αβ)|1β1β|\displaystyle\frac{2g^{2}_{a\beta}g^{2}_{b\beta}}{\omega_{\beta}(\Delta_{a\beta}+\alpha_{\beta})(\Delta_{b\beta}+\alpha_{\beta})}|1_{\beta}\rangle\langle 1_{\beta}| (20)
+\displaystyle+ 2gaβ2gbβ2ωβΔaβΔbβ|1β1β|.\displaystyle\frac{2g^{2}_{a\beta}g^{2}_{b\beta}}{\omega_{\beta}\Delta_{a\beta}\Delta_{b\beta}}|1_{\beta}\rangle\langle 1_{\beta}|.

Adding the corrections by the cross-kerr resonances, the total ZZ coupling can be defined as ξZZ(t)=ξZZ(2)+ξZZ(3)+ξZZ(4s)+ξZZ(4c,0)ξZZ(4c,1)\xi^{(t)}_{ZZ}=\xi^{(2)}_{ZZ}+\xi^{(3)}_{ZZ}+\xi^{(4s)}_{ZZ}+\xi^{(4c,0)}_{ZZ}-\xi^{(4c,1)}_{ZZ}, with ξZZ(3)=λ=a,bξZZ,λ(3)\xi^{(3)}_{ZZ}=\sum_{\lambda=a,b}\xi^{(3)}_{ZZ,\lambda}, ξZZ(4s)=λ=a,bξZZ,λ(4s)\xi^{(4s)}_{ZZ}=\sum_{\lambda=a,b}\xi^{(4s)}_{ZZ,\lambda}, ξZZ(4c,0)=β=x,yξZZ,β(4c,0)\xi^{(4c,0)}_{ZZ}=\sum_{\beta=x,y}\xi^{(4c,0)}_{ZZ,\beta}, and ξZZ(4c,1)=β=x,yξZZ,β(4c,1)\xi^{(4c,1)}_{ZZ}=\sum_{\beta=x,y}\xi^{(4c,1)}_{ZZ,\beta}. We plot the second-order ξZZ(2)\xi^{(2)}_{ZZ} (red-solid curves), third-order ξZZ(3)\xi^{(3)}_{ZZ} (blue-dashed curves), and fourth-order (self-kerr resonance) ξZZ(4s)\xi^{(4s)}_{ZZ} (green-dotted curves) static ZZ coupling in Fig. 9(c) (gxy/(2π)=0.2g_{xy}/(2\pi)=0.2 MHz) and Fig. 9(d) (gxy/(2π)=1.4g_{xy}/(2\pi)=1.4 MHz). By reducing the direct qubit-qubit coupling strengths, the values of static ZZ coupling curves are apparently suppressed in Fig. 9(c) (gxy/(2π)=0.2g_{xy}/(2\pi)=0.2 MHz) compared with the result in Fig. 9(d) (gxy/(2π)=1.4g_{xy}/(2\pi)=1.4 MHz). The energy level corrections to qubit’s ground state (ξZZ(4c,0)\xi^{(4c,0)}_{ZZ}) and first-excited state (ξZZ(4c,1)\xi^{(4c,1)}_{ZZ}) by the cross-kerr resonances are respectively plotted in the black dashed-dot curves and marked purple-solid curves in Figs. 9(c) and  9(d).

The curves of effective qubit-qubit coupling are plotted in Fig. 9(a), and values of direct qubit-qubit coupling affect switching off positions. Similar with Fig. 6(b), the two poles locating at Δxy=αx\Delta_{xy}=\alpha_{x} and Δxy=αy\Delta_{xy}=-\alpha_{y} also appear in each curve of static ZZ coupling ξZZ(t)\xi^{(t)}_{ZZ} in Fig. 9(b). But there are two new poles in each curve of static ZZ coupling ξZZ(t)\xi^{(t)}_{ZZ} in Fig. 9(b) which should originate from the cross-kerr resonance[39, 40]. As indicated by Eqs.(19) and (20), the cross-kerr resonances through virtual photon exchanges induces additional poles for the static ZZ coupling at the point: 2ωβ+αβ=ωa+ωb2\omega_{\beta}+\alpha_{\beta}=\omega_{a}+\omega_{b} (from Eq.(19)), ωβ+αβ=ωa\omega_{\beta}+\alpha_{\beta}=\omega_{a} (from Eq.(20)), and ωβ+αβ=ωb\omega_{\beta}+\alpha_{\beta}=\omega_{b} (from Eq.(20)). So we can see two new poles at ωy+αy=ωa\omega_{y}+\alpha_{y}=\omega_{a} and 2ωy+αy=ωa+ωb2\omega_{y}+\alpha_{y}=\omega_{a}+\omega_{b} in each curve of Fig. 9(b). Another pole (ωy+αy=ωb\omega_{y}+\alpha_{y}=\omega_{b}) is out of the scope of the drawing. As shown in Figs. 9(c) and  9(d), the pole at 2ωy+αy=ωa+ωb2\omega_{y}+\alpha_{y}=\omega_{a}+\omega_{b} only appears on the black dash-dotted curves which correspond to the level correction to qubits’ ground states by the cross-kerr resonance ξZZ(4c,0)\xi^{(4c,0)}_{ZZ}. While the pole at ωy+αy=ωa\omega_{y}+\alpha_{y}=\omega_{a} only appears in the marked purple-solid curve which describes the level correction to qubits’ first-excited states by the cross-kerr resonance ξZZ(4c,1)\xi^{(4c,1)}_{ZZ}. In this article, we neglect the level corrections of cross-kerr resonances to the double-excited state |01x1y0|01_{x}1_{y}0\rangle, which should correspond to more complex physical processes.

V Conclusions

In conclusion, we have studied the mechanism of the switching off in the superconducting circuit consisting of two fixed-frequency resonator couplers. The induced indirect qubit-qubit coupling by two resonators can be cancelled, so the switching off can be realized without the direct qubit-qubit coupling. The frequencies of couplers can be much smaller than the single transmon-based coupler circuit, and this leaves wider available frequency spaces for couplers (or qubits), thus the frequency crowding on the superconducting chip might be relieved.

The weak direct qubit-qubit coupling can be used to suppress the static ZZ coupling in the double-coupler circuit, and the destructive interferences between double-path couplers can eliminate the static ZZ coupling, thus the quality of superconducting quantum chip might be enhanced. Our proposed double-resonator couplers scheme can unfreeze some restrictions on the superconducting quantum chip, mitigate the static ZZ coupling, and also save the dilution refrigerator lines, which might be a promising platform for superconducting quantum chip.

VI ACKNOWLEDGMENTS

H.W. is supported by the Natural Science Foundation of Shandong Province under Grant No. ZR2023LZH002 and the Inspur artificial intelligence research institute. Y.J.Z. is supported by Beijing Natural Science Foundation under Grant No. 4222064 and NSFC under Grant No. 11904013. X.-W.X. is supported by the National Natural Science Foundation of China under Grant No. 12064010, and Natural Science Foundation of Hunan Province of China under Grant No. 2021JJ20036.

Appendix A: The numerical calculation of the energy levels

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Figure 10: (Color online) The two-dimensional surfaces of energy levels. The curved surfaces for single-excited state in the circuit are shown in (a)-(d), and (e)-(s) describe the energy level curved surfaces of double-excited states. The maximal frequencies of two qubits are: ωx(max)/2π=4.56\omega^{(max)}_{x}/2\pi=4.56 GHz, and ωy(max)/2π=5.12\omega^{(max)}_{y}/2\pi=5.12 GHz. The other parameters are : gxy/2π=1g_{xy}/2\pi=1 MHz, gab/2π=0.1g_{ab}/2\pi=0.1 MHz, ωa/2π=4.10\omega_{a}/2\pi=4.10 GHz, ωb/2π=5.20\omega_{b}/2\pi=5.20 GHz, αx/2π=175\alpha_{x}/2\pi=-175 MHz, αy/2π=195\alpha_{y}/2\pi=-195 MHz, gax/2π=gay/2π=32g_{ax}/2\pi=g_{ay}/2\pi=32 MHz, and gbx/2π=gby/2π=30g_{bx}/2\pi=g_{by}/2\pi=30 MHz.

In this section, we use the numerical method to calculate the two-dimensional energy level curved surfaces of the double-resonator couplers circuit (Fig. 1). Since the anharmonicities of Xmon qubit is very small, we regard the superconducting artificial atom as a multi-energy levels system in this section[39, 16]. The Hamiltonian for the circuit in Fig. 1 can be written as

Hm/=λ=a,bωλcλcλ\displaystyle H_{m}/\hbar=\sum_{\lambda=a,b}\omega_{\lambda}c^{\dagger}_{\lambda}c_{\lambda}
+\displaystyle+ jβωjβjβJjβjβz+gab(cacb+cbca)\displaystyle\sum_{j_{\beta}}\omega_{j_{\beta}j^{\prime}_{\beta}}J^{z}_{j_{\beta}j^{\prime}_{\beta}}+g_{ab}\left(c^{\dagger}_{a}c_{b}+c^{\dagger}_{b}c_{a}\right)
+\displaystyle+ λ=a,b;β=x,yjβ,jβ=0,1,2,gλjβ,jβ(Jjβjβ++Jjβjβ)(cλ+cλ)\displaystyle\sum_{\lambda=a,b;\beta=x,y\atop j_{\beta},j^{\prime}_{\beta}=0,1,2,...}g^{j_{\beta},j^{\prime}_{\beta}}_{\lambda}\left(J^{+}_{j^{\prime}_{\beta}j_{\beta}}+J^{-}_{j_{\beta}j^{\prime}_{\beta}}\right)\left(c_{\lambda}+c^{\dagger}_{\lambda}\right)
+\displaystyle+ jx,jx,jy′′,jy′′′=0,1,2,gxyjxjx,jy′′jy′′′(Jjxjx+Jjy′′jy′′′+Jjy′′′jy′′+Jjxjx),\displaystyle\sum_{j_{x},j^{\prime}_{x},j^{\prime\prime}_{y},j^{\prime\prime\prime}_{y}\atop=0,1,2,...}g^{j_{x}j^{\prime}_{x},j^{\prime\prime}_{y}j^{\prime\prime\prime}_{y}}_{xy}\left(J^{+}_{j^{\prime}_{x}j_{x}}J^{-}_{j^{\prime\prime}_{y}j^{\prime\prime\prime}_{y}}+J^{+}_{j^{\prime\prime\prime}_{y}j^{\prime\prime}_{y}}J^{-}_{j_{x}j^{\prime}_{x}}\right),

where jβ,jβ,jβ′′,jβ′′′=0,1,2,3j_{\beta},j^{\prime}_{\beta},j^{\prime\prime}_{\beta},j^{\prime\prime\prime}_{\beta}=0,1,2,3\cdot\cdot\cdot, and they respectively label the jβj_{\beta}-th, jβj^{\prime}_{\beta}-th, jβ′′j^{\prime\prime}_{\beta}-th, and jβ′′′j^{\prime\prime\prime}_{\beta}-th quantum states of qubit β\beta, with jβ′′′>jβ′′j^{\prime\prime\prime}_{\beta}>j^{\prime\prime}_{\beta} and jβ>jβj^{\prime}_{\beta}>j_{\beta}. Between the quantum states |jβ|j_{\beta}\rangle and |jβ|j^{\prime}_{\beta}\rangle, we define the angular momentum operators as Jjβjβ=[Jjβjβx,Jjβjβy,Jjβjβz]\vec{J}_{j_{\beta}j^{\prime}_{\beta}}=[J^{x}_{j_{\beta}j^{\prime}_{\beta}},J^{y}_{j_{\beta}j^{\prime}_{\beta}},J^{z}_{j_{\beta}j^{\prime}_{\beta}}]. The ladder operators can be introduced by Jjβjβ+=|jβjβ|J^{+}_{j_{\beta}j^{\prime}_{\beta}}=|j^{\prime}_{\beta}\rangle\langle j_{\beta}| and Jjβjβ=|jβjβ|J^{-}_{j_{\beta}j^{\prime}_{\beta}}=|j_{\beta}\rangle\langle j^{\prime}_{\beta}|, thus we can get Jjβjβz=|jβjβ||jβjβ|J^{z}_{j_{\beta}j^{\prime}_{\beta}}=|j^{\prime}_{\beta}\rangle\langle j^{\prime}_{\beta}|-|j_{\beta}\rangle\langle j_{\beta}|, Jjβjβx=(Jjβjβ++Jjβjβ)/2J^{x}_{j_{\beta}j^{\prime}_{\beta}}=(J^{+}_{j_{\beta}j^{\prime}_{\beta}}+J^{-}_{j_{\beta}j^{\prime}_{\beta}})/2, and Jjβjβy=(Jjβjβ+Jjβjβ)/(2i)J^{y}_{j_{\beta}j^{\prime}_{\beta}}=(J^{+}_{j_{\beta}j^{\prime}_{\beta}}-J^{-}_{j_{\beta}j^{\prime}_{\beta}})/(2i). The corresponding transition frequency between states |jβ|j_{\beta}\rangle and |jβ|j^{\prime}_{\beta}\rangle is defined as ωjβjβ\omega_{j_{\beta}j^{\prime}_{\beta}}, the gλjβ,jβg^{j_{\beta},j^{\prime}_{\beta}}_{\lambda} describe the corresponding coupling strengths with resonator coupler λ\lambda. The gxyjxjx,jy′′jy′′′g^{j_{x}j^{\prime}_{x},j^{\prime\prime}_{y}j^{\prime\prime\prime}_{y}}_{xy} describes the direct coupling strengths between the transition processes of |jx|jx|j^{\prime}_{x}\rangle\leftrightarrow|j_{x}\rangle for qubits x and |jy′′′|jy′′′′|j^{\prime\prime\prime}_{y}\rangle\leftrightarrow|j^{\prime\prime\prime\prime}_{y}\rangle for qubit y.

With the QuTiP software, we calculate the two-dimensional curved surfaces for the energy level of single-excited (Figs. 10(a)-10(d)) and double-excited (Figs. 10(e)-10(s)) states. During the numerical calculations with the QuTiP software, we truncate to the second excited states of qubits and assume gλjβ,jβ=gλjβ,jβ=gλβg^{j_{\beta},j^{\prime}_{\beta}}_{\lambda}=g^{j^{\prime}_{\beta},j_{\beta}}_{\lambda}=g_{\lambda\beta} and gyxjxjx,jy′′jy′′′=gxyjyjy,jx′′′jx′′=gxyg^{j_{x}j^{\prime}_{x},j^{\prime\prime}_{y}j^{\prime\prime\prime}_{y}}_{yx}=g^{j^{\prime}_{y}j_{y},j^{\prime\prime\prime}_{x}j^{\prime\prime}_{x}}_{xy}=g_{xy}. Because of the anti-crossing effects, each curved surface in Fig. 10 can not describe a total energy level of certain quantum state, and we label the Z-axis of each figure by the corresponding state at zero magnetic flux.

Appendix B: Circuit Quantization

In this section, we conduct the quantization for the superconducting circuit in Fig. 1. The kinetic energy of the superconducting circuit can be obtained as [17, 20]

T\displaystyle T =\displaystyle= 12(Caϕ˙a2+Cbϕ˙b2+Cxϕ˙x2+Cyϕ˙y2)\displaystyle\frac{1}{2}\left(C_{a}\dot{\phi}^{2}_{a}+C_{b}\dot{\phi}^{2}_{b}+C_{x}\dot{\phi}^{2}_{x}+C_{y}\dot{\phi}^{2}_{y}\right) (B.1)
+\displaystyle+ 12Cab(ϕ˙aϕ˙b)2+12Cxy(ϕ˙xϕ˙y)2\displaystyle\frac{1}{2}C_{ab}\left(\dot{\phi}_{a}-\dot{\phi}_{b}\right)^{2}+\frac{1}{2}C_{xy}\left(\dot{\phi}_{x}-\dot{\phi}_{y}\right)^{2}
+\displaystyle+ 12Cax(ϕ˙aϕ˙x)2+12Cay(ϕ˙aϕ˙y)2\displaystyle\frac{1}{2}C_{ax}\left(\dot{\phi}_{a}-\dot{\phi}_{x}\right)^{2}+\frac{1}{2}C_{ay}\left(\dot{\phi}_{a}-\dot{\phi}_{y}\right)^{2}
+\displaystyle+ 12Cbx(ϕ˙bϕ˙x)2+12Cby(ϕ˙bϕ˙y)2.\displaystyle\frac{1}{2}C_{bx}\left(\dot{\phi}_{b}-\dot{\phi}_{x}\right)^{2}+\frac{1}{2}C_{by}\left(\dot{\phi}_{b}-\dot{\phi}_{y}\right)^{2}.

As indicated by Fig. 1(b), the self-capacitances of the qubits and resonators is CηC_{\eta} , and the relative capacitance between arbitrary two devices is defined as CηηC_{\eta\eta^{\prime}} ( Cηη=CηηC_{\eta\eta^{\prime}}=C_{\eta^{\prime}\eta}), here η,η=a,b,x,y\eta,\eta^{\prime}=a,b,x,y with ηη\eta\neq\eta^{\prime}. Here ϕa\phi_{a} and ϕb\phi_{b} are the respective magnetic fluxes of the circuit nodes of resonators a and b, while ϕx\phi_{x} and ϕy\phi_{y} are respective node fluxes of qubits x and y. If we define the vector ϕ=[ϕa,ϕb,ϕx,ϕy]\vec{\phi}=[\phi_{a},\phi_{b},\phi_{x},\phi_{y}], thus the kinetic energy in Eq.(B.1) can be written as T=12ϕ˙TCϕ˙T=\frac{1}{2}\dot{\vec{\phi}}^{T}C\dot{\vec{\phi}}, with

C\displaystyle C =\displaystyle= (C11CabCaxCayCabC22CbxCbyCaxCbxC33CxyCayCbyCxyC44.),\displaystyle\left(\begin{array}[]{cccc}C_{11}&-C_{ab}&-C_{ax}&-C_{ay}\\ -C_{ab}&C_{22}&-C_{bx}&-C_{by}\\ -C_{ax}&-C_{bx}&C_{33}&-C_{xy}\\ -C_{ay}&-C_{by}&-C_{xy}&C_{44}.\\ \end{array}\right), (B.6)

where we have defined the coefficients: C11=Ca+Cab+Cax+CayC_{11}=C_{a}+C_{ab}+C_{ax}+C_{ay}, C22=Cab+Cb+Cbx+CbyC_{22}=C_{ab}+C_{b}+C_{bx}+C_{by}, C33=Cax+Cbx+Cx+CxyC_{33}=C_{ax}+C_{bx}+C_{x}+C_{xy}, and C44=Cay+Cby+Cxy+CyC_{44}=C_{ay}+C_{by}+C_{xy}+C_{y}.

The potential energy for the superconducting circuit can be written as

U\displaystyle U =\displaystyle= ϕa22La+ϕb22Lb+EJx[1cos(2πΦ0ϕx)]\displaystyle\frac{\phi^{2}_{a}}{2L_{a}}+\frac{\phi^{2}_{b}}{2L_{b}}+E_{J_{x}}\left[1-\cos\left(\frac{2\pi}{\Phi_{0}}\phi_{x}\right)\right] (B.7)
+\displaystyle+ EJy[1cos(2πΦ0ϕy)],\displaystyle E_{J_{y}}\left[1-\cos\left(\frac{2\pi}{\Phi_{0}}\phi_{y}\right)\right],

where EJβ=IcβΦ0/2πE_{J_{\beta}}=I_{c\beta}\Phi_{0}/2\pi is the Josephson energy of qubit β\beta, IcβI_{c\beta} is the corresponding critical current, and Φ0=h/2e\Phi_{0}=h/2e is the flux quantum.

The Lagrangian of the superconducting circuit can be obtained by the definition L=TUL=T-U, thus the generalized momentum can be defined as qη=L/ϕ˙ηq_{\eta}=\partial L/\partial\dot{\phi}_{\eta} (η=a,b,x,y\eta=a,b,x,y), and it can be written in the vector form as q=[qa,qb,qx,qy]\vec{q}=[q_{a},q_{b},q_{x},q_{y}]. Thus the Hamiltonian of superconducting circuit can be written as H=qϕ˙L=12qTC1q+UH=\vec{q}\cdot\dot{\vec{\phi}}-L=\frac{1}{2}\vec{q}^{T}C^{-1}\vec{q}+U, the inverse matrix is defined as

C1\displaystyle C^{-1} =\displaystyle= A|C|=1C(A11A21A31A41A12A22A32A42A13A23A33A43A14A24A34A44.).\displaystyle\frac{A^{\ast}}{|C|}=\frac{1}{||C||}\left(\begin{array}[]{cccc}A_{11}&A_{21}&A_{31}&A_{41}\\ A_{12}&A_{22}&A_{32}&A_{42}\\ A_{13}&A_{23}&A_{33}&A_{43}\\ A_{14}&A_{24}&A_{34}&A_{44}.\\ \end{array}\right). (B.12)

where AA^{\ast} is the adjugate matrix of AA. With the conditions CabCxyCax,Cay,Cbx,CbyCx,CyCa,CbC_{ab}\ll C_{xy}\ll C_{ax},C_{ay},C_{bx},C_{by}\ll C_{x},C_{y}\ll C_{a},C_{b}, thus CCaCbCxCy\|C\|\approx C_{a}C_{b}C_{x}C_{y}, we get approximate expressions for the elements in AA^{\ast} as

A11\displaystyle A_{11} =\displaystyle= C22(C33C44Cxy2)+Cbx(CbxC44CxyCby)\displaystyle C_{22}(C_{33}C_{44}-C^{2}_{xy})+C_{bx}(-C_{bx}C_{44}-C_{xy}C_{by})
\displaystyle- Cby(CbxCxy+C33Cby)CbCxCy,\displaystyle C_{by}(C_{bx}C_{xy}+C_{33}C_{by})\approx C_{b}C_{x}C_{y},
A12\displaystyle A_{12} =\displaystyle= Cab(C33C44Cxy2)Cbx(CaxC44CxyCay)\displaystyle C_{ab}(C_{33}C_{44}-C^{2}_{xy})-C_{bx}(-C_{ax}C_{44}-C_{xy}C_{ay})
+\displaystyle+ Cby(CaxCxy+C33Cay)\displaystyle C_{by}(C_{ax}C_{xy}+C_{33}C_{ay})
\displaystyle\approx CabCxCy+CaxCbxCy+CayCbyCx,\displaystyle C_{ab}C_{x}C_{y}+C_{ax}C_{bx}C_{y}+C_{ay}C_{by}C_{x},
A13\displaystyle A_{13} =\displaystyle= Cab(CbxC44+CbyCxy)+C22(CaxC44+CxyCay)\displaystyle C_{ab}(C_{bx}C_{44}+C_{by}C_{xy})+C_{22}(C_{ax}C_{44}+C_{xy}C_{ay})
\displaystyle- Cby(CaxCbyCbxCay)CbCyCax,\displaystyle C_{by}(C_{ax}C_{by}-C_{bx}C_{ay})\approx C_{b}C_{y}C_{ax},
A14\displaystyle A_{14} =\displaystyle= Cab(CbxCxy+C33Cby)+C22(Caxcxy+C33Cay)\displaystyle C_{ab}(C_{bx}C_{xy}+C_{33}C_{by})+C_{22}(C_{ax}c_{xy}+C_{33}C_{ay}) (B.13)
+\displaystyle+ Cbx(CaxCbyCbxCay)CbCxCay,\displaystyle C_{bx}(C_{ax}C_{by}-C_{bx}C_{ay})\approx C_{b}C_{x}C_{ay},
A21\displaystyle A_{21} =\displaystyle= Cab(C33C44Cxy2)+Cax(CbxC44+CxyCby)\displaystyle C_{ab}(C_{33}C_{44}-C^{2}_{xy})+C_{ax}(C_{bx}C_{44}+C_{xy}C_{by})
+\displaystyle+ Cay(CbxCxy+C33Cby)\displaystyle C_{ay}(C_{bx}C_{xy}+C_{33}C_{by})
\displaystyle\approx CabCxCy+CaxCbxCy+CayCbyCx,\displaystyle C_{ab}C_{x}C_{y}+C_{ax}C_{bx}C_{y}+C_{ay}C_{by}C_{x},
A22\displaystyle A_{22} =\displaystyle= C11(C33C44Cxy2)Cax(CaxC44+CxyCay)\displaystyle C_{11}(C_{33}C_{44}-C^{2}_{xy})-C_{ax}(C_{ax}C_{44}+C_{xy}C_{ay})
\displaystyle- Cay(CaxCxy+C33Cay)CaCxCy,\displaystyle C_{ay}(C_{ax}C_{xy}+C_{33}C_{ay})\approx C_{a}C_{x}C_{y},
A23\displaystyle A_{23} =\displaystyle= C11(CbxC44+CxyCby)+Cab(CaxC44+CxyCay)\displaystyle C_{11}(C_{bx}C_{44}+C_{xy}C_{by})+C_{ab}(C_{ax}C_{44}+C_{xy}C_{ay})
+\displaystyle+ Cay(CaxCbyCbxCay)CbxCaCy,\displaystyle C_{ay}(C_{ax}C_{by}-C_{bx}C_{ay})\approx C_{bx}C_{a}C_{y},
A24\displaystyle A_{24} =\displaystyle= C11(CbxCxy+C33Cby)+Cab(CaxCxy+C33Cay)\displaystyle C_{11}(C_{bx}C_{xy}+C_{33}C_{by})+C_{ab}(C_{ax}C_{xy}+C_{33}C_{ay})
\displaystyle- Cax(CaxCbyCbxCay)CaCxCby,\displaystyle C_{ax}(C_{ax}C_{by}-C_{bx}C_{ay})\approx C_{a}C_{x}C_{by},
A31\displaystyle A_{31} =\displaystyle= Cab(CbxC44CbyCxy)+Cax(C22C44Cby2)\displaystyle-C_{ab}(-C_{bx}C_{44}-C_{by}C_{xy})+C_{ax}(C_{22}C_{44}-C^{2}_{by})
\displaystyle- Cay(C22CxyCbxCby)CaxCbcy,\displaystyle C_{ay}(-C_{22}C_{xy}-C_{bx}C_{by})\approx C_{ax}C_{b}c_{y},
A32\displaystyle A_{32} =\displaystyle= C11(CbxC44+CbyCxy)+Cax(CabC44+CayCby)\displaystyle C_{11}(C_{bx}C_{44}+C_{by}C_{xy})+C_{ax}(C_{ab}C_{44}+C_{ay}C_{by})
+\displaystyle+ Cay(CabCxyCbxCby)CbxCaCy,\displaystyle C_{ay}(C_{ab}C_{xy}-C_{bx}C_{by})\approx C_{bx}C_{a}C_{y},
A33\displaystyle A_{33} =\displaystyle= C11(C22C44Cby2)+Cab(CabC44CayCby)\displaystyle C_{11}(C_{22}C_{44}-C^{2}_{by})+C_{ab}(-C_{ab}C_{44}-C_{ay}C_{by})
\displaystyle- Cay(CabCby+C22Cay)CaCbCy,\displaystyle C_{ay}(C_{ab}C_{by}+C_{22}C_{ay})\approx C_{a}C_{b}C_{y},
A34\displaystyle A_{34} =\displaystyle= C11(C22Cxy+CbxCby)Cab(CabCxyCbxCay)\displaystyle C_{11}(C_{22}C_{xy}+C_{bx}C_{by})-C_{ab}(C_{ab}C_{xy}-C_{bx}C_{ay})
+\displaystyle+ Cax(CabCby+C22Cay)\displaystyle C_{ax}(C_{ab}C_{by}+C_{22}C_{ay})
\displaystyle\approx CxyCaCb+CaCbxCby+CbCaxCay,\displaystyle C_{xy}C_{a}C_{b}+C_{a}C_{bx}C_{by}+C_{b}C_{ax}C_{ay},
A41\displaystyle A_{41} =\displaystyle= Cab(CbxCxy+CbyC33)+Cax(C22Cxy+CbxCby)\displaystyle C_{ab}(C_{bx}C_{xy}+C_{by}C_{33})+C_{ax}(C_{22}C_{xy}+C_{bx}C_{by})
+\displaystyle+ Cay(C22C33Cbx2)CayCbCx,\displaystyle C_{ay}(C_{22}C_{33}-C^{2}_{bx})\approx C_{ay}C_{b}C_{x},
A42\displaystyle A_{42} =\displaystyle= C11(CbxCxy+CbyC33)+Cax(CabCxyCaxCby)\displaystyle C_{11}(C_{bx}C_{xy}+C_{by}C_{33})+C_{ax}(C_{ab}C_{xy}-C_{ax}C_{by})
\displaystyle- Cay(CabC33CaxCbx)CaCxCby,\displaystyle C_{ay}(-C_{ab}C_{33}-C_{ax}C_{bx})\approx C_{a}C_{x}C_{by},
A43\displaystyle A_{43} =\displaystyle= C11(C22Cxy+CbxCby)+Cab(CabCxy+CaxCby)\displaystyle C_{11}(C_{22}C_{xy}+C_{bx}C_{by})+C_{ab}(C_{ab}C_{xy}+C_{ax}C_{by})
+\displaystyle+ Cay(CabCbx+C22Cax)\displaystyle C_{ay}(C_{ab}C_{bx}+C_{22}C_{ax})
\displaystyle\approx CxyCaCb+CaCbxCby+CbCaxCay,\displaystyle C_{xy}C_{a}C_{b}+C_{a}C_{bx}C_{by}+C_{b}C_{ax}C_{ay},
A44\displaystyle A_{44} =\displaystyle= C11(C22C33Cbx2)+Cab(Caxc33CaxCbx)\displaystyle C_{11}(C_{22}C_{33}-C^{2}_{bx})+C_{ab}(-C_{ax}c_{33}-C_{ax}C_{bx})
\displaystyle- Cax(CaxCbx+C22Cax)CaCbCx.\displaystyle C_{ax}(C_{ax}C_{bx}+C_{22}C_{ax})\approx C_{a}C_{b}C_{x}.

Thus the Hamiltonian of double-resonator couplers circuit can be expressed as

H\displaystyle H =\displaystyle= 4ECa(na)2+4ECb(nb)2+4ECx(nx)2+4ECy(ny)2\displaystyle 4E_{C_{a}}(n_{a})^{2}+4E_{C_{b}}(n_{b})^{2}+4E_{C_{x}}(n_{x})^{2}+4E_{C_{y}}(n_{y})^{2}
+\displaystyle+ ϕa22La+ϕb22LbEJxcos(2πΦ0ϕx)EJycos(2πΦ0ϕy)\displaystyle\frac{\phi^{2}_{a}}{2L_{a}}+\frac{\phi^{2}_{b}}{2L_{b}}-E_{J_{x}}\cos\left(\frac{2\pi}{\Phi_{0}}\phi_{x}\right)-E_{J_{y}}\cos\left(\frac{2\pi}{\Phi_{0}}\phi_{y}\right)
+\displaystyle+ 8CaxCaCxECaECx(nanx)\displaystyle 8\frac{C_{ax}}{\sqrt{C_{a}C_{x}}}\sqrt{E_{C_{a}}E_{C_{x}}}(n_{a}n_{x})
+\displaystyle+ 8CayCaCyECaECy(nany)\displaystyle 8\frac{C_{ay}}{\sqrt{C_{a}C_{y}}}\sqrt{E_{C_{a}}E_{C_{y}}}(n_{a}n_{y})
+\displaystyle+ 8CbxCbCxECbECx(nbnx)\displaystyle 8\frac{C_{bx}}{\sqrt{C_{b}C_{x}}}\sqrt{E_{C_{b}}E_{C_{x}}}(n_{b}n_{x})
+\displaystyle+ 8CbyCbCyECbECy(nbny)\displaystyle 8\frac{C_{by}}{\sqrt{C_{b}C_{y}}}\sqrt{E_{C_{b}}E_{C_{y}}}(n_{b}n_{y})
+\displaystyle+ 8(1+CaxCbxCxCab+CayCbyCyCab)CabCaCbECaECb(nanb)\displaystyle 8\left(1+\frac{C_{ax}C_{bx}}{C_{x}C_{ab}}+\frac{C_{ay}C_{by}}{C_{y}C_{ab}}\right)\frac{C_{ab}}{\sqrt{C_{a}C_{b}}}\sqrt{E_{C_{a}}E_{C_{b}}}(n_{a}n_{b})
+\displaystyle+ 8(1+CaxCayCaCxy+CbxCbyCbCxy)CxyCxCyECxECy(nxny).\displaystyle 8\left(1+\frac{C_{ax}C_{ay}}{C_{a}C_{xy}}+\frac{C_{bx}C_{by}}{C_{b}C_{xy}}\right)\frac{C_{xy}}{\sqrt{C_{x}C_{y}}}\sqrt{E_{C_{x}}E_{C_{y}}}(n_{x}n_{y}).

The two-body coupling strengths can be defined as

gλβ\displaystyle g_{\lambda\beta} =\displaystyle= 12CλβCλCβωλωβ,\displaystyle\frac{1}{2}\frac{C_{\lambda\beta}}{\sqrt{C_{\lambda}C_{\beta}}}\sqrt{\omega_{\lambda}\omega_{\beta}}, (B.15)
gab\displaystyle g_{ab} =\displaystyle= 12(1+CaxCbxCxCab+CayCbyCyCab)CabCaCbωaωb,\displaystyle\frac{1}{2}\left(1+\frac{C_{ax}C_{bx}}{C_{x}C_{ab}}+\frac{C_{ay}C_{by}}{C_{y}C_{ab}}\right)\frac{C_{ab}}{\sqrt{C_{a}C_{b}}}\sqrt{\omega_{a}\omega_{b}},\qquad (B.16)
gxy\displaystyle g_{xy} =\displaystyle= 12(1+CaxCayCaCxy+CbxCbyCbCxy)CxyCxCyωxωy.\displaystyle\frac{1}{2}\left(1+\frac{C_{ax}C_{ay}}{C_{a}C_{xy}}+\frac{C_{bx}C_{by}}{C_{b}C_{xy}}\right)\frac{C_{xy}}{\sqrt{C_{x}C_{y}}}\sqrt{\omega_{x}\omega_{y}}.\qquad (B.17)

The qubit-resonator interaction terms gλβg_{\lambda\beta} in Eq.(B.9) could induce indirect coupling between two qubits, which should be decoupled to obtained the effective qubit-qubit coupling.

Appendix C: Decoupling processes

The Josephson energy of Xmon qubit is much larger than its capacitance energy, EJβ/ECβ1E_{J_{\beta}}/E_{C_{\beta}}\gg 1, and then we can approximately get cos(ϕβ)=1ϕβ2/2+ϕβ4/24\cos(\phi_{\beta})=1-\phi^{2}_{\beta}/2+\phi^{4}_{\beta}/24-.... If we introduce the creation and annihilation operators by the definitions: ϕβ=(2EC/EJβ)4(aβ+aβ)\phi_{\beta}=\sqrt[4]{(2E_{C}/E_{J_{\beta}})}(a^{\dagger}_{\beta}+a_{\beta}) and nβ=(i/2)(2EC/EJβ)4(aβaβ)n_{\beta}=(i/2)\sqrt[4]{(2E_{C}/E_{J_{\beta}})}(a^{\dagger}_{\beta}-a_{\beta}), then second-quantized Hamiltonian can be obtained as Htot=λ=a,bHλ+β=x,yHβ+λ=a,bβ=x,yHλβ+Hab(r)+Hxy(q)H_{tot}=\sum_{\lambda=a,b}{H_{\lambda}}+\sum_{\beta=x,y}{H_{\beta}}+\sum_{\lambda=a,b\atop\beta=x,y}H_{\lambda\beta}+H^{(r)}_{ab}+H^{(q)}_{xy}, with

Hλ\displaystyle H_{\lambda} =\displaystyle= 12ωλcλcλ,\displaystyle\frac{1}{2}\hbar\omega_{\lambda}c^{\dagger}_{\lambda}c_{\lambda}, (C.1)
Hβ\displaystyle H_{\beta} =\displaystyle= 12ωβaβaβ+αβ2aβaβaβaβ,\displaystyle\frac{1}{2}\hbar\omega_{\beta}a^{\dagger}_{\beta}a_{\beta}+\frac{\alpha_{\beta}}{2}a^{\dagger}_{\beta}a^{\dagger}_{\beta}a_{\beta}a_{\beta}, (C.2)
Hλβ\displaystyle H_{\lambda\beta} =\displaystyle= gλβ(cλaβ+cλaβcλaβcλaβ),\displaystyle\hbar g_{\lambda\beta}(c^{\dagger}_{\lambda}a_{\beta}+c_{\lambda}a^{\dagger}_{\beta}-c^{\dagger}_{\lambda}a^{\dagger}_{\beta}-c_{\lambda}a_{\beta}), (C.3)
Hab(r)\displaystyle H^{(r)}_{ab} =\displaystyle= gab(cacb+cacbcacbcacb),\displaystyle\hbar g_{ab}(c^{\dagger}_{a}c_{b}+c_{a}c^{\dagger}_{b}-c^{\dagger}_{a}c^{\dagger}_{b}-c_{a}c_{b}), (C.4)
Hxy(q)\displaystyle H^{(q)}_{xy} =\displaystyle= gxy(axay+axayaxayaxay).\displaystyle\hbar g_{xy}(a^{\dagger}_{x}a_{y}+a_{x}a^{\dagger}_{y}-a^{\dagger}_{x}a^{\dagger}_{y}-a_{x}a_{y}). (C.5)

The transition frequencies of resonators and qubits are respectively defined as ωλ=1/CλLλ\omega_{\lambda}=1/\sqrt{C_{\lambda}L_{\lambda}} and ωβ=(8EJβECβECβ)/\omega_{\beta}=(\sqrt{8E_{J_{\beta}}E_{C_{\beta}}}-E_{C_{\beta}})/\hbar, while the αβ=ECβ/\alpha_{\beta}=-E_{C_{\beta}}/\hbar describe the anharmonicity of qubit β\beta.

In the qubit-resonator dispersive coupling regimes, gλβ/|Δλβ|1g_{\lambda\beta}/|\Delta_{\lambda\beta}|\ll 1, we can use the Schrieffer-Wolf transformation to decouple the variables of qubits and resonators. Since the resonator couplers are not pumped by the external fields, and the average cavity photon number should be much smaller than one, so the virtual photon exchanges will dominate the cross-kerr resonances. We define S=λ=a,bβ=x,y[(gλβ/Δλβ)(cλaβcλaβ)(gλβ/Σλβ)(cλaβcλaβ)]S=\sum_{\lambda=a,b\atop\beta=x,y}[(g_{\lambda\beta}/\Delta_{\lambda\beta})(c^{\dagger}_{\lambda}a_{\beta}-c_{\lambda}a^{\dagger}_{\beta})-(g_{\lambda\beta}/\Sigma_{\lambda\beta})(c^{\dagger}_{\lambda}a^{\dagger}_{\beta}-c_{\lambda}a_{\beta})]. Under the Unitary transformation H(d)=exp(S)Hexp(S)H^{(d)}=\exp(-S)H\exp(S), if we choose Hλβ+[H0,S]=0H_{\lambda\beta}+[H_{0},S]=0, thus the decoupled Hamiltonian can be obtained as

H(d)\displaystyle H^{(d)} =\displaystyle= ωa(d)caca+ωb(d)cbcb+ωx(d)axax+ωy(d)ayay\displaystyle\hbar\omega^{(d)}_{a}c^{\dagger}_{a}c_{a}+\hbar\omega^{(d)}_{b}c^{\dagger}_{b}c_{b}+\hbar\omega^{(d)}_{x}a^{\dagger}_{x}a_{x}+\hbar\omega^{(d)}_{y}a^{\dagger}_{y}a_{y} (C.6)
+\displaystyle+ α~x2axaxaxax+α~y2ayayayay\displaystyle\frac{\hbar\tilde{\alpha}_{x}}{2}a^{\dagger}_{x}a^{\dagger}_{x}a_{x}a_{x}+\frac{\hbar\tilde{\alpha}_{y}}{2}a^{\dagger}_{y}a^{\dagger}_{y}a_{y}a_{y}
+\displaystyle+ gxy(d)(axay+ayax)+gab(d)(cacb+cbca).\displaystyle\hbar g^{(d)}_{xy}(a^{\dagger}_{x}a_{y}+a^{\dagger}_{y}a_{x})+\hbar g^{(d)}_{ab}(c^{\dagger}_{a}c_{b}+c^{\dagger}_{b}c_{a}).

The rotating wave approximation has been used to derive the above formula, and the constant terms were neglected. We also neglected the effects of small quantities (HxyH_{xy} and HabH_{ab}). The anharmonicities of qubits are considered as invariant during Unitary transformation ( α~βαβ\tilde{\alpha}_{\beta}\approx\alpha_{\beta}), so some high-order effects relating to high-excited states of superconducting artificial atoms are neglected.

The transition frequencies of qubits, the resonant frequencies of resonators, the qubit-qubit coupling strength, and the resonator-resonator coupling strength in decoupled coordinate are obtained as

ωx(d)\displaystyle\omega^{(d)}_{x} =\displaystyle= ωx+(gax2Δax+gbx2Δbxgax2Σaxgbx2Σbx),\displaystyle\omega_{x}+\left(\frac{g^{2}_{ax}}{\Delta_{ax}}+\frac{g^{2}_{bx}}{\Delta_{bx}}-\frac{g^{2}_{ax}}{\Sigma_{ax}}-\frac{g^{2}_{bx}}{\Sigma_{bx}}\right), (C.7)
ωy(d)\displaystyle\omega^{(d)}_{y} =\displaystyle= ωy+(gay2Δay+gby2Δbygay2Σaygby2Σby),\displaystyle\omega_{y}+\left(\frac{g^{2}_{ay}}{\Delta_{ay}}+\frac{g^{2}_{by}}{\Delta_{by}}-\frac{g^{2}_{ay}}{\Sigma_{ay}}-\frac{g^{2}_{by}}{\Sigma_{by}}\right), (C.8)
ωa(d)\displaystyle\omega^{(d)}_{a} =\displaystyle= ωa(gax2Δax+gay2Δaygax2Σaxgay2Σay),\displaystyle\omega_{a}-\left(\frac{g^{2}_{ax}}{\Delta_{ax}}+\frac{g^{2}_{ay}}{\Delta_{ay}}-\frac{g^{2}_{ax}}{\Sigma_{ax}}-\frac{g^{2}_{ay}}{\Sigma_{ay}}\right), (C.9)
ωb(d)\displaystyle\omega^{(d)}_{b} =\displaystyle= ωb(gbx2Δbx+gby2Δbygbx2Σbxgby2Σby),\displaystyle\omega_{b}-\left(\frac{g^{2}_{bx}}{\Delta_{bx}}+\frac{g^{2}_{by}}{\Delta_{by}}-\frac{g^{2}_{bx}}{\Sigma_{bx}}-\frac{g^{2}_{by}}{\Sigma_{by}}\right), (C.10)
gxy(d)\displaystyle g^{(d)}_{xy} =\displaystyle= 12(gaxgayΔay+gbxgbyΔby+gaygaxΔax+gbygbxΔbx\displaystyle\frac{1}{2}\bigg{(}\frac{g_{ax}g_{ay}}{\Delta_{ay}}+\frac{g_{bx}g_{by}}{\Delta_{by}}+\frac{g_{ay}g_{ax}}{\Delta_{ax}}+\frac{g_{by}g_{bx}}{\Delta_{bx}}
\displaystyle- gaxgayΣaygbxgbyΣbygaygaxΣaxgbygbxΣbx)+gxy,\displaystyle\frac{g_{ax}g_{ay}}{\Sigma_{ay}}-\frac{g_{bx}g_{by}}{\Sigma_{by}}-\frac{g_{ay}g_{ax}}{\Sigma_{ax}}-\frac{g_{by}g_{bx}}{\Sigma_{bx}}\bigg{)}+g_{xy},
gab(d)\displaystyle g^{(d)}_{ab} =\displaystyle= 12(gaxgbxΔbx+gaygbyΔby+gbxgaxΔax+gbygayΔay\displaystyle\frac{1}{2}\bigg{(}\frac{g_{ax}g_{bx}}{\Delta_{bx}}+\frac{g_{ay}g_{by}}{\Delta_{by}}+\frac{g_{bx}g_{ax}}{\Delta_{ax}}+\frac{g_{by}g_{ay}}{\Delta_{ay}}
\displaystyle- gaxgbxΣbxgaygbyΣbygbxgaxΣaxgbygayΣay)+gab.\displaystyle\frac{g_{ax}g_{bx}}{\Sigma_{bx}}-\frac{g_{ay}g_{by}}{\Sigma_{by}}-\frac{g_{bx}g_{ax}}{\Sigma_{ax}}-\frac{g_{by}g_{ay}}{\Sigma_{ay}}\bigg{)}+g_{ab}.

The gxy(d)g^{(d)}_{xy} is the decoupled qubit-qubit coupling strength which can be used to analyze the switching off. The gab(d)g^{(d)}_{ab} is the decoupled resonator-resonator and much smaller than the frequency detuning between two resonators (gab(d)|Δxy|g^{(d)}_{ab}\ll|\Delta_{xy}|), thus its contributions are neglected in this article.

Appendix D:Calculations of High-energy level corrections

In the current theoretical model, the kerr-nonlinear terms Hnl,β=(αβ/2)aβaβaβaβH_{nl,\beta}=(\alpha_{\beta}/2)a^{\dagger}_{\beta}a^{\dagger}_{\beta}a_{\beta}a_{\beta} term are assumed bo be invariant (α~βαβ\tilde{\alpha}_{\beta}\approx\alpha_{\beta}) during the derivations of Eqs.(C.6). This means that some high-order effects and the contributions of high excited state of superconducting artificial atom are neglected, so the decoupled frequency and effective qubit-qubit coupling in Eqs.(C.7)-(C.12) contain no information of qubits’ anharmoncities. But anharmoncity of Xmon qubit is very small, thus the resonator can couple to the high-excited states of atoms, which should affect the transition frequencies of qubits and the effective qubit-qubit coupling strengths. As discussed by some theoretical work, the anharmonicity could induced fourth-order self-kerr and cross-kerr resonances, these effects could create corrections to the qubit’s energy levels[40, 39].

Bogoliubov transformation is used to analyze the higher-order effect during the decoupling processes for the qubit-resonator interactions[40]. To maintain consistency, in this article we still use the Schrieffer-Wolf transformation to analyze the contributions of the kerr-nonlinear terms Hnl,βH_{nl,\beta} during the decoupling process. In the qubit-resonator dispersive coupling regimes, (gλβ/Δλβ)1(g_{\lambda\beta}/\Delta_{\lambda\beta})\ll 1 and (gλβ/Σλβ)1(g_{\lambda\beta}/\Sigma_{\lambda\beta})\ll 1, we define Sλβ=(gλβ/Δλβ)(cλaβcλaβ)(gλβ/Σλβ)(cλaβcλaβ)S_{\lambda\beta}=(g_{\lambda\beta}/\Delta_{\lambda\beta})(c^{\dagger}_{\lambda}a_{\beta}-c_{\lambda}a^{\dagger}_{\beta})-(g_{\lambda\beta}/\Sigma_{\lambda\beta})(c^{\dagger}_{\lambda}a^{\dagger}_{\beta}-c_{\lambda}a_{\beta}), here S=λ=a,bβ=x,ySλβS=\sum_{\lambda=a,b\atop\beta=x,y}S_{\lambda\beta}. Since Hnl,βH_{nl,\beta} is a small quantity, we can separately conduct the Unitary transform Hnl,β=exp(S)Hnl,βexp(S)H^{\prime}_{nl,\beta}=\exp(S)H_{nl,\beta}\exp(-S) [40], thus we get

Hnl,β\displaystyle H^{\prime}_{nl,\beta} =\displaystyle= Hnl,β+[S,Hnl,β]+12![S,[S,Hnl,β]]\displaystyle H_{nl,\beta}+[S,H_{nl,\beta}]+\frac{1}{2!}[S,[S,H_{nl,\beta}]] (D.1)
+\displaystyle+ 13![S[S,[S,Hnl,β]]]+.\displaystyle\frac{1}{3!}[S[S,[S,H_{nl,\beta}]]]+....

The commutation relation for the first-order expansion term,

[Sλβ,Hnl,β]\displaystyle[S_{\lambda\beta},H_{nl,\beta}] (D.2)
=\displaystyle= [gλβΔλβ(cλaβcλaβ)gλβΣλβ(cλaβcλaβ),αβ2aβaβaβaβ]\displaystyle\left[\frac{g_{\lambda\beta}}{\Delta_{\lambda\beta}}(c^{\dagger}_{\lambda}a_{\beta}-c_{\lambda}a^{\dagger}_{\beta})-\frac{g_{\lambda\beta}}{\Sigma_{\lambda\beta}}(c^{\dagger}_{\lambda}a^{\dagger}_{\beta}-c_{\lambda}a_{\beta}),\frac{\alpha_{\beta}}{2}a^{\dagger}_{\beta}a^{\dagger}_{\beta}a_{\beta}a_{\beta}\right]
=\displaystyle= gλβαβΔλβ(cλaβaβaβ+cλaβaβaβ)\displaystyle\frac{g_{\lambda\beta}\alpha_{\beta}}{\Delta_{\lambda\beta}}\left(c^{\dagger}_{\lambda}a^{\dagger}_{\beta}a_{\beta}a_{\beta}+c_{\lambda}a^{\dagger}_{\beta}a^{\dagger}_{\beta}a_{\beta}\right)
+\displaystyle+ gλβαβΣλβ(cλaβaβaβ+cλaβaβaβ).\displaystyle\frac{g_{\lambda\beta}\alpha_{\beta}}{\Sigma_{\lambda\beta}}\left(c^{\dagger}_{\lambda}a^{\dagger}_{\beta}a^{\dagger}_{\beta}a_{\beta}+c_{\lambda}a^{\dagger}_{\beta}a_{\beta}a_{\beta}\right).

Since gxy,gabgλβg_{xy},g_{ab}\ll g_{\lambda\beta}, we have neglected the effects of the weak direct qubit-qubit and resonator-resonator interactions.

The commutation relation for the second-order expansion term,

[Sλβ,[Sλβ,Hnl,β]]\displaystyle[S_{\lambda\beta},[S_{\lambda\beta},H_{nl,\beta}]] (D.3)
=\displaystyle= [4gλx2αβΔλβ2cλcλaβaβ+4gλβ2αβΣλβ2cλcλaβaβ]\displaystyle\left[\frac{4g^{2}_{\lambda x}\alpha_{\beta}}{\Delta^{2}_{\lambda\beta}}c^{\dagger}_{\lambda}c_{\lambda}a^{\dagger}_{\beta}a_{\beta}+\frac{4g^{2}_{\lambda\beta}\alpha_{\beta}}{\Sigma^{2}_{\lambda\beta}}c_{\lambda}c^{\dagger}_{\lambda}a^{\dagger}_{\beta}a_{\beta}\right]
+\displaystyle+ (2gλβ2αβΣλβ22gλβ2αβΔλβ2)aβaβaβaβ\displaystyle\left(\frac{2g^{2}_{\lambda\beta}\alpha_{\beta}}{\Sigma^{2}_{\lambda\beta}}-\frac{2g^{2}_{\lambda\beta}\alpha_{\beta}}{\Delta^{2}_{\lambda\beta}}\right)a^{\dagger}_{\beta}a^{\dagger}_{\beta}a_{\beta}a_{\beta}
+\displaystyle+ gλβ2αβΔλβ2cλcλaβaβ+gλβ2αβΔλβ2cλcλaβaβ\displaystyle\frac{g^{2}_{\lambda\beta}\alpha_{\beta}}{\Delta^{2}_{\lambda\beta}}c^{\dagger}_{\lambda}c^{\dagger}_{\lambda}a_{\beta}a_{\beta}+\frac{g^{2}_{\lambda\beta}\alpha_{\beta}}{\Delta^{2}_{\lambda\beta}}c_{\lambda}c_{\lambda}a^{\dagger}_{\beta}a^{\dagger}_{\beta}
+\displaystyle+ gλβ2αβΣλβ2cλcλaβaβ+gλβ2αβΣλβ2cλcλaβaβ\displaystyle\frac{g^{2}_{\lambda\beta}\alpha_{\beta}}{\Sigma^{2}_{\lambda\beta}}c^{\dagger}_{\lambda}c^{\dagger}_{\lambda}a^{\dagger}_{\beta}a^{\dagger}_{\beta}+\frac{g^{2}_{\lambda\beta}\alpha_{\beta}}{\Sigma^{2}_{\lambda\beta}}c_{\lambda}c_{\lambda}a_{\beta}a_{\beta}
+\displaystyle+ 2gλβ2αβΔλβΣλβcλcλaβaβ+4gλβ2αβΔλβΣλβcλcλaβaβ\displaystyle\frac{2g^{2}_{\lambda\beta}\alpha_{\beta}}{\Delta_{\lambda\beta}\Sigma_{\lambda\beta}}c^{\dagger}_{\lambda}c^{\dagger}_{\lambda}a^{\dagger}_{\beta}a_{\beta}+\frac{4g^{2}_{\lambda\beta}\alpha_{\beta}}{\Delta_{\lambda\beta}\Sigma_{\lambda\beta}}c_{\lambda}c_{\lambda}a^{\dagger}_{\beta}a_{\beta}
+\displaystyle+ gλβ2αβΔλβΣλβ(2cλcλ+1)aβaβ\displaystyle\frac{g^{2}_{\lambda\beta}\alpha_{\beta}}{\Delta_{\lambda\beta}\Sigma_{\lambda\beta}}(2c^{\dagger}_{\lambda}c_{\lambda}+1)a_{\beta}a_{\beta}
+\displaystyle+ gλβ2αβΔλβΣλβ(2cλcλ+1)aβaβ\displaystyle\frac{g^{2}_{\lambda\beta}\alpha_{\beta}}{\Delta_{\lambda\beta}\Sigma_{\lambda\beta}}(2c^{\dagger}_{\lambda}c_{\lambda}+1)a^{\dagger}_{\beta}a^{\dagger}_{\beta}

Up to the second-order expanding terms, keeping the energy and particle number conservation terms, we can get the nonlinear term for qubit β\beta in the decoupled coordinate as

Hnl,β\displaystyle H^{\prime}_{nl,\beta} =\displaystyle= λ=a,b(gλβ2αβΣλβ2gλβ2αβΔλβ2)aβaβaβaβ\displaystyle\sum_{\lambda=a,b}\left(\frac{g^{2}_{\lambda\beta}\alpha_{\beta}}{\Sigma^{2}_{\lambda\beta}}-\frac{g^{2}_{\lambda\beta}\alpha_{\beta}}{\Delta^{2}_{\lambda\beta}}\right)a^{\dagger}_{\beta}a^{\dagger}_{\beta}a_{\beta}a_{\beta} (D.4)
+\displaystyle+ λ=a,b[2gλx2αβΔλβ2cλcλaβaβ+2gλβ2αβΣλβ2cλcλaβaβ]\displaystyle\sum_{\lambda=a,b}\left[\frac{2g^{2}_{\lambda x}\alpha_{\beta}}{\Delta^{2}_{\lambda\beta}}c^{\dagger}_{\lambda}c_{\lambda}a^{\dagger}_{\beta}a_{\beta}+\frac{2g^{2}_{\lambda\beta}\alpha_{\beta}}{\Sigma^{2}_{\lambda\beta}}c_{\lambda}c^{\dagger}_{\lambda}a^{\dagger}_{\beta}a_{\beta}\right]
+λ=a,b[gλβ2αβ2Δλβ2cλcλaβaβ+gλβ2αβ2Δλβ2cλcλaβaβ]\displaystyle+\sum_{\lambda=a,b}\left[\frac{g^{2}_{\lambda\beta}\alpha_{\beta}}{2\Delta^{2}_{\lambda\beta}}c^{\dagger}_{\lambda}c^{\dagger}_{\lambda}a_{\beta}a_{\beta}+\frac{g^{2}_{\lambda\beta}\alpha_{\beta}}{2\Delta^{2}_{\lambda\beta}}c_{\lambda}c_{\lambda}a^{\dagger}_{\beta}a^{\dagger}_{\beta}\right]
+λ=a,bgλβαβΔλβ(cλaβaβaβ+cλaβaβaβ).\displaystyle+\sum_{\lambda=a,b}\frac{g_{\lambda\beta}\alpha_{\beta}}{\Delta_{\lambda\beta}}\left(c^{\dagger}_{\lambda}a^{\dagger}_{\beta}a_{\beta}a_{\beta}+c_{\lambda}a^{\dagger}_{\beta}a^{\dagger}_{\beta}a_{\beta}\right).

In the right side of Eq.(D.4), the first line describes the self-kerr resonance, while the second line labels to the cross-kerr resonance. The third line describe the double virtual processes between one qubit and one resonator. The fourth line describes combined physical processes that the qubit and the resonator exchange a virtual photon, and the qubit simulatively participates the self-excitation and subsequent self-annihilation processes.

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